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The mixed rare-earth orthochromite Nd$_{0.5}$Dy$_{0.5}$CrO$_{3}$ has a N\'eel temperature ($T_\mathrm{{N}}$) of ${\sim}$ 175\,K, resulting in the G-type antiferromagnetic ordering of Cr$^{3+}$ spins. The inverse susceptibility shows a…

The quantum dimer magnet, with antiferromagnetic intradimer and interdimer Heisenberg exchange between spin-1/2 moments, is known to host an up/down - down/up singlet ground state when the intradimer exchange is dominant. Rare-earth-based…

Strongly Correlated Electrons · Physics 2025-09-10 A. Brassington , Q. Ma , G. Duan , S. Calder , A. I. Kolesnikov , K. M. Taddei , G. Sala , E. S. Choi , H. Wang , W. Xie , B. A. Frandsen , N. Li , X. F. Sun , C. Liu , R. Yu , H. D. Zhou , A. A. Aczel

Motivated by the recent experimental progress on the strong spin-orbit-coupled rare earth triangular antiferromagnet, we analyze the highly anisotropic spin model that describes the interaction between the spin-orbit-entangled Kramers'…

Strongly Correlated Electrons · Physics 2016-07-13 Yao-Dong Li , Xiaoqun Wang , Gang Chen

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$\frac{1}{2}$ state due to the combined effect of crystal electric field and spin…

Strongly Correlated Electrons · Physics 2020-04-22 K. M. Ranjith , Ph. Schlender , Th. Doert , M. Baenitz

As a hallmark of electronic correlation, spin-charge interplay underlies many emergent phenomena in doped Mott insulators, such as high-temperature superconductivity, whereas the half-filled parent state is usually electronically frozen…

Magnetism of Cu$_2$(OH)$_3$Br single crystals based on a triangular lattice is studied by means of magnetic susceptibility, pulsed-field magnetization, and specific heat measurements. There are two inequivalent Cu$^{2+}$ sites in an…

Strongly Correlated Electrons · Physics 2019-09-04 Z Y Zhao , H L Che , R Chen , J F Wang , X F Sun , Z Z He

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

We report studies of the magnetic properties of a staggered stacked triangular lattice Ba$_2$MnTeO$_6$ using magnetic susceptibility, specific heat, neutron powder diffraction and inelastic neutron scattering measurements, as well as first…

We report on high-field electron spin resonance (ESR) studies of magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuBr$_4$. Frequency-field diagrams of ESR excitations are measured for different orientations of…

Motivated by experiments on the double perovskites La2ZnIrO6 and La2MgIrO6, we study the magnetism of spin-orbit coupled j=1/2 iridium moments on the three-dimensional, geometrically frustrated, face-centered cubic lattice. The…

Strongly Correlated Electrons · Physics 2015-09-30 A. M. Cook , S. Matern , C. Hickey , A. A. Aczel , A. Paramekanti

We report magnetic susceptibility, specific heat and muon spin relaxation (muSR) experiments on the triangular antiferromagnet La2Ca2MnO7 which develops a genuine two-dimensional, three-sublattice \sqrt{3} \times \sqrt{3} magnetic order…

Strongly Correlated Electrons · Physics 2015-07-08 P. Dalmas de Réotier , C. Marin , A. Yaouanc , T. Douce , A. Sikora , A. Amato , C. Baines

A detailed zero and transverse field (ZF&TF) muon spin rotation (muSR) investigation of magnetism and the magneto-electric coupling in Cu2OSeO3 is reported. An internal magnetic field B_int(T=0) = 85.37(25) mT was found, in agreement with a…

Strongly Correlated Electrons · Physics 2015-05-28 A. Maisuradze , Z. Guguchia , B. Graneli , H. M. Ronnow , H. Berger , H. Keller

Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…

Two triangular lattice antiferromagnets Sr$_3$Co(Nb,Ta)$_2$O$_9$ with an effective $j_{\rm eff}=1/2$ of Co$^{2+}$ are synthesized and their magnetic properties are investigated via magnetization and heat capacity measurements. The leading…

Strongly Correlated Electrons · Physics 2023-08-09 Surender Lal , Sebin J Sebastian , S. S. Islam , M. P. Saravanan , M. Uhlarz , Y. Skourski , R. Nath

Spin-1/2 Heisenberg antiferromagnetic frustrated spin chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is…

We report $^{75}$As nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) studies on the superconductor Rb$_{2}$Cr$_{3}$As$_{3}$ with a quasi one-dimensional crystal structure. Below $T\sim$ 100 K, the spin-lattice…

Superconductivity · Physics 2015-10-07 J. Yang , Z. T. Tang , G. H. Cao , Guo-qing Zheng

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

We performed high-field magnetization, magnetocaloric effect (MCE), and NMR measurements on the Ising triangular-lattice antiferromagnet Rb$_2$Co(SeO$_3$)$_2$. The observations of the 1/3-magnetization plateau, the split NMR lines, and the…

Dynamical correlations of Jeff = 1/2 isospins in the paramagnetic state of spin-orbital Mott insu- lator Sr2IrO4 was revealed by resonant magnetic x-ray diffuse scattering. We found two-dimensional antiferromagnetic fluctuation with a large…

Strongly Correlated Electrons · Physics 2015-06-04 S. Fujiyama , H. Ohsumi , T. Komesu , J. Matsuno , B. J. Kim , M. Takata , T. Arima , H. Takagi