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Magnetic Properties of an Effective Spin-$\frac{1}{2}$ Triangular-Lattice Compound LiYbS$_2$

Strongly Correlated Electrons 2020-04-22 v1 Materials Science

Abstract

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS2_2. At low temperatures, it features an effective spin-12\frac{1}{2} state due to the combined effect of crystal electric field and spin orbit coupling. Magnetic susceptibility measurements and 7^7Li nuclear magnetic resonance experiments reveal the absence of magnetic long range ordering down to 2~K, which suggests a possible quantum spin liquid ground state. A dominant antiferromagnetic nearest neighbour exchange interaction J/kBJ/k_{\rm B}\simeq 5.3~K could be extracted form the magnetic susceptibility. The NMR linewidth analysis yields the coupling constant between the Li nuclei and Yb3+^{3+} ions which was found to be purely dipolar in nature.

Keywords

Cite

@article{arxiv.2003.00566,
  title  = {Magnetic Properties of an Effective Spin-$\frac{1}{2}$ Triangular-Lattice Compound LiYbS$_2$},
  author = {K. M. Ranjith and Ph. Schlender and Th. Doert and M. Baenitz},
  journal= {arXiv preprint arXiv:2003.00566},
  year   = {2020}
}

Comments

(accepted)