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We calculated the magnetic dipole and the electric quadrupole hyperfine interaction constants of 3s3p $^{3,1}P^o_1$ states and the isotope shift, including mass and field shift, factors for transitions from these two states to the ground…

Atomic Physics · Physics 2017-09-13 Tingxian Zhang , Luyou Xie , Jiguang Li , Zehuang Lu

We study atomic systems that are in the frequency range of optical atomic clocks and have enhanced sensitivity to potential time-variation of the fine structure constant, alpha. The high sensitivity is due to coherent contributions from…

Atomic Physics · Physics 2010-09-16 J. C. Berengut , V. A. Dzuba , V. V. Flambaum

We propose a novel class of atomic clocks based on highly charged ions. We consider highly-forbidden laser-accessible transitions within the $4f^{12}$ ground-state configurations of highly charged ions. Our evaluation of systematic effects…

Atomic Physics · Physics 2016-10-05 Andrei Derevianko , V. A. Dzuba , V. V. Flambaum

An ultrastable optical clock based on neutral atoms trapped in an optical lattice is proposed. Complete control over the light shift is achieved by employing the $5s^2 {}^1S_0 \to 5s5p {}^3P_0$ transition of ${}^{87}{\rm Sr}$ atoms as a…

Atomic Physics · Physics 2009-11-10 Hidetoshi Katori , Masao Takamoto , V. G. Pal'chikov , V. D. Ovsiannikov

We review a number of highly charged ions which have optical transitions suitable for building extremely accurate atomic clocks. This includes ions from Hf$^{12+}$ to U$^{34+}$, which have the $4f^{12}$ configuration of valence electrons,…

Atomic Physics · Physics 2015-06-23 V. A. Dzuba , V. V. Flambaum

We explore the potential of the electric quadrupole transitions $7s\,^2S_{1/2}$ - $6d\,^2D_{3/2}$, $6d\,^2D_{5/2}$ in radium isotopes as single-ion optical frequency standards. The frequency shifts of the clock transitions due to external…

A systematic study of Ca+ atomic properties is carried out using high-precision relativistic all-order method where all single, double, and partial triple excitations of the Dirac-Fock wave functions are included to all orders of…

Atomic Physics · Physics 2015-05-20 M. S. Safronova , U. I. Safronova

Highly charged ions of heavy actinides from uranium to einsteinium are studied theoretically to find optical transitions sensitive to the variation of the fine structure constant. A number of promising transitions have been found in ions…

Atomic Physics · Physics 2024-05-21 V. A. Dzuba , V. V. Flambaum

Vibrational overtones in deeply bound molecules are sensitive probes for variation of the proton-to-electron mass ratio $\mu$. In nonpolar molecules, these overtones may be driven as two-photon transitions. Here, we present procedures for…

Atomic Physics · Physics 2019-01-03 Ryan Carollo , Alexander Frenett , David Hanneke

Theories unifying gravity and other interactions suggest the possibility of spatial and temporal variation of physical ``constants''. Accuracy achieved for the atomic optical frequency standards (optical clocks) approaches the level when…

Atomic Physics · Physics 2009-02-05 V. A. Dzuba , V. V. Flambaum.

It is shown that the dynamic differential scalar polarisability of the $S_{1/2}-D_{5/2}$ transition in $^{138}$Ba$^+$ can be determined to an inaccuracy below $0.5\%$ across a wide wavelength range ($\lambda>700\,\mathrm{nm}$). This can be…

Atomic Physics · Physics 2019-10-30 M. D. Barrett , K. J. Arnold , M. S. Safronova

We report an observation of the weak $6^{1}$S$_{0}$-$6^3$P$_0$ transition in $^{171,173}$Yb as an important step to establish Yb as a primary candidate for future optical frequency standards, and to open up a new approach for qubits using…

Atomic Physics · Physics 2009-11-11 Tao Hong , Claire Cramer , Eryn Cook , Warren Nagourney , E. N. Fortson

We propose a new frequency standard based on a $4f^{14} 6s6p~ ^3\!P_0 - 4f^{13} 6s^2 5d ~(J=2)$ transition in neutral Yb. This transition has a potential for high stability and accuracy and the advantage of the highest sensitivity among…

Atomic Physics · Physics 2018-05-02 M. S. Safronova , S. G. Porsev , Christian Sanner , Jun Ye

State-of-the-art atomic clocks are based on the precise detection of the energy difference between two atomic levels, measured as a quantum phase accumulated in a given time interval. Optical-lattice clocks (OLCs) now operate at or near the…

The first three electronically excited states in the alkaline-earth-metal atoms magnesium, calcium, and strontium comprise the (nsnp) triplet P^o_J (J=0,1,2) fine-structure manifold. All three states are metastable and are of interest for…

Atomic Physics · Physics 2009-11-10 Robin Santra , Kevin V. Christ , Chris H. Greene

We consider a narrow magneto-dipole transition in the $^{169}$Tm atom at the wavelength of $1.14\,\mu$m as a candidate for a 2D optical lattice clock. Calculating dynamic polarizabilities of the two clock levels $[\text{Xe}]4f^{13}6s^2…

Active optical clock, a new conception of atomic clock, has been proposed recently. In this report, we propose a scheme of active optical clock based on four-level quantum system. The final accuracy and stability of two-level quantum system…

Atomic Physics · Physics 2014-04-18 Tonggang Zhang , Yanfei Wang , Xiaorun Zang , Wei Zhuang , Jingbiao Chen

We address the problem of the lattice Stark shifts in the Sr clock caused by the multipolar $M1$ and $E2$ atom-field interactions and by the term nonlinear in lattice intensity and determined by the hyperpolarizability. We have developed an…

Atomic Physics · Physics 2018-02-14 S. G. Porsev , M. S. Safronova , U. I. Safronova. , M. G. Kozlov

We present the experimental demonstration of non-destructive probing of the 1S0-3P0 clock transition probability in an optical lattice clock with 87Sr atoms. It is based on the phase shift induced by the atoms on a weak off-resonant laser…

Quantum Physics · Physics 2011-02-08 Jerome Lodewyck , Philip G. Westergaard , Pierre Lemonde

We experimentally investigate an optical frequency standard based on the $^2S_{1/2} (F=0)\to {}^2F_{7/2} (F=3)$ electric octupole (\textit{E}3) transition of a single trapped $^{171}$Yb$^+$ ion. For the spectroscopy of this strongly…

Atomic and Molecular Clusters · Physics 2016-02-15 N. Huntemann , C. Sanner , B. Lipphardt , Chr. Tamm , E. Peik