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In this work, we experimentally manipulate the spectrum and phase of a biphoton wave packet in a two-dimensional frequency space. The spectrum is shaped by adjusting the temperature of the crystal, and the phase is controlled by tilting the…

Quantum Physics · Physics 2018-08-14 Rui-Bo Jin , Ryoji Shiina , Ryosuke Shimizu

We demonstrate a new technique for saturated-absorption spectroscopy using co-propagating beams that does not have the problem of crossover resonances. The pump beam is locked to a transition and its absorption signal is monitored while the…

Atomic Physics · Physics 2009-11-10 Ayan Banerjee , Vasant Natarajan

We have previously demonstrated that in the context of two-dimensional (2D) coherent electronic spectroscopy measured by phase modulation and phase-sensitive detection, an \emph{incoherent} nonlinear response, due to pairs of…

The recently proposed affine frequency division multiplexing (AFDM) modulation has been considered as a promising technology for narrowband doubly-dispersive channels. However, the time-scaling effects, i.e., pulse widening and pulse…

Performance · Computer Science 2025-07-08 Xiangxiang Li , Haiyan Wang , Yao Ge , Xiaohong Shen , Yong Liang Guan , Miaowen Wen , Chau Yuen

Understanding optical responses of topological matter is a central problem for enabling optoelectronic applications based on topological physics, which is of fundamental concern for photocurrents control and spectroscopy. Currently, schemes…

Other Condensed Matter · Physics 2026-04-24 Osamah Sufyan , Ofer Neufeld

Pump-probe microscopy enables label-free imaging of structural and chemical features of samples. However, signals in pump-probe microscopy are typically small and often must be measured in the presence of large backgrounds. As a result,…

We investigate the precision of estimating the interaction strength between a two-level system (TLS) and a single-photon pulse when the latter is subject to chirping. We consider linear, quadratic, and sinusoidal temporal phases applied to…

Quantum Physics · Physics 2024-11-07 Elnaz Darsheshdar , Aiman Khan , Francesco Albarelli , Animesh Datta

Transient absorption (TA) is the most widespread method to follow ultrafast dynamics in molecules and materials. The related method of TA anisotropy (TAA) reports on the ultrafast reorientation dynamics of transition dipole moments,…

We vary the time-frequency mode structure of ultrafast pulse-pumped modulational instability (MI) twin beams in an argon-filled hollow-core kagom\'e-style PCF by adjusting the pressure, pump pulse chirp, fiber length and parametric gain.…

Quantum Physics · Physics 2017-05-10 Martin A. Finger , Nicolas Y. Joly , Philip St. J. Russell , Maria V. Chekhova

The Coulomb drag is a many-body effect observed in proximized low-dimensional systems. It appears as emergence of voltage in one of them upon passage of bias current in another. The magnitude of drag voltage can be strongly affected by…

Mesoscale and Nanoscale Physics · Physics 2024-11-22 Ilya Safonov , Aleksandr S. Petrov , Dmitry Svintsov

Ultrachirped pulses for which the frequency chirp is of the order of the transition frequency of a two-level atom are examined. When the chirp is large enough, the resonance may be crossed twice, for positive and negative quadrature…

Quantum Physics · Physics 2011-11-08 S. Ibáñez , A. Peralta Conde , D. Guéry-Odelin , J. G. Muga

A chirped-pulse interleaving method is reported for generation of dual optical frequency combs based on electro-optic phase modulators (EOM) in a free-running all-fiber based system. Methods are discussed to easily modify the linear chirp…

Single-shot supercontinuum spectral interferometry (SSSI) is an optical technique that can measure ultrafast transients in the complex index of refraction. This method uses chirped supercontinuum reference/probe pulses that need to be…

Instrumentation and Detectors · Physics 2018-06-05 DinhDuy Tran Vu , Dogeun Jang , Ki-Yong Kim

Phase-sensitive pump-probe hyperspectral imaging is a precise technique for absolute two-beam measurements of the optical Kerr coefficient ($n_2$). The irradiance profile is characterized and background effects are rejected by rastering the…

Optics · Physics 2026-04-14 J. K. Wahlstrand , C. D. Cruz

Scanning tunneling spectroscopy of the high-Tc superconductor Bi2Sr2CaCu2O8+d reveals weak, incommensurate, spatial modulations in the tunneling conductance. Images of these energy-dependent modulations are Fourier analyzed to yield the…

Superconductivity · Physics 2009-11-07 J. E. Hoffman , K. McElroy , D. -H. Lee , K. M Lang , H. Eisaki , S. Uchida , J. C. Davis

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

The effect of the pulse-shape on pump-probe spectroscopies is examined for the simplest model of noninteracting fermions on an infinite-dimensional hypercubic lattice. The probe-modified density of states follows the time evolution of the…

Strongly Correlated Electrons · Physics 2018-09-27 A. M. Shvaika , O. P. Matveev , T. P. Devereaux , J. K. Freericks

Breaking the symmetry in a coupled wave system can result in unusual amplification behavior. In the case of difference parametric amplification the resonant pump frequency is equal to the difference, instead of the sum, frequency of the…

Quantum Physics · Physics 2021-05-17 Wayne Cheng-Wei Huang , Herman Batelaan

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

Atomic Physics · Physics 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

Two-dimensional (2D) fluorescence-excitation (2D-FLEX) spectroscopy is a recently proposed nonlinear femtosecond technique for the detection of photoinduced dynamics. The method records a time-resolved fluorescence signal in its excitation-…

Chemical Physics · Physics 2024-06-24 Sebastian V. Pios , Maxim F. Gelin , Luis Vasquez , Jürgen Hauer , Lipeng Chen