Related papers: Cross-phase modulation in the two dimensional spec…
We show that two-photon coherent control in a $V$-shape three-level system projects one-photon coherent transient in a simple two-level system. Higher order chirps of a shaped laser pulse play the roles of time and linear chirp in…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
This theoretical paper investigates the formation of ground state molecules from ultracold cesium atoms in a two-color scheme. Following previous work on photoassociation with chirped picosecond pulses [Luc-Koenig et al., Phys. Rev. A {\bf…
Level-crossing spectroscopy involves lifting the degeneracy of an excited state and using the interference of two nearly degenerate levels to measure the excited state lifetime. Here we use the idea of interference between different…
A new difference-frequency method based on electro-optic phase modulators and two free-running lasers is reported to perform THz dual-comb spectroscopy.
We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection this delay line allows for recording of 6 ps decay traces…
The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond…
The paper describes the design of broadband chirp excitation pulses in NMR. We first develop a three stage model for understanding chirp excitation in NMR. We then show how a chirp $\pi$ pulse can be used to refocus the phase of the chirp…
Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…
We demonstrate experimentally a scheme to measure small temporal delays, much smaller than the pulse width, between optical pulses. Specifically, we observe an interference effect, based on the concepts of quantum weak measurements and weak…
Recent work applying multidimentional coherent electronic spectroscopy at dilute samples in the gas phase is reviewed. The development of refined phase-cycling approaches with improved sensitivity has opened-up new opportunities to probe…
We consider the interaction between distinct superradiance (SR) systems and use the dressed state formalism to solve the case of two interacting two-atom SR samples at resonance. We show that the ensuing entanglement modifies the transition…
In this letter, we propose dual-mode chirp spread spectrum (DM-CSS) modulation for low-power wide-area networks. DM-CSS is capable of achieving a higher spectral efficiency (SE) relative to its counterparts, such as Long Range (LoRa)…
Spectral analyses of energetic particle (EP) driven bursts of MHD fluctuations in magnetically confined plasmas often exhibit multiple simultaneous chirps. While the superposition of oscillations at multiple frequencies necessarily causes…
We explore theoretically the feasibility of using frequency conversion by sum- or difference-frequency generation, enabled by three- wave-mixing, for selectively multiplexing orthogonal input waveforms that overlap in time and frequency.…
We show that the modulation of the phases of the laser beams of ultra-short pulses leads to modulation of the two photon fluorescence intensity. The phase modulation technique when used in multi-photon microscopy can improve the signal to…
In this work we extend low frequency impulsive stimulated Raman microspectroscopy to the pre-electronic resonance regime. We use a broadband two color collinear pump probe scheme which can be readily extended to imaging. We discuss the…
The single-particle density of states and the tunneling conductance are studied for a two-dimensional BCS-like Hamiltonian with a d_{x^2-y^2}-gap and phase fluctuations. The latter are treated by a classical Monte Carlo simulation of an XY…
A new technique for obtaining switched wave packets using spectrally truncated chirped laser pulses is demonstrated experimentally and numerically by one-dimensional alignment of both linear and asymmetric top molecules. Using a simple…
Light travel time changes due to gravitational waves may be detected within the next decade through precision timing of millisecond pulsars. Removal of frequency-dependent interstellar medium (ISM) delays due to dispersion and scattering is…