Related papers: Cross-phase modulation in the two dimensional spec…
Nonlinear terahertz (THz) spectroscopy relies on the interaction of matter with few-cycle THz pulses of electric field amplitudes up to megavolts/centimeter (MV/cm). In condensed-phase molecular systems, both resonant interactions with…
We present the first fully ab initio calculations for attosecond transient absorption spectroscopy of atomic krypton with overlapping pump and probe pulses. Within the time-dependent configuration interaction singles (TDCIS) approach, we…
We present a simple approach to predict the main features of optical spectra affected by self-phase modulation (SPM), which is based on regarding the spectrum modification as an interference effect. A two-wave interference model is found…
We present a study of the effects of dispersion on the properties of photon pairs generated by type-II, collinear spontaneous parametric downconversion. Specifically, we take into consideration the effects of a chirped pump, as well as of…
The consistent quantum theory of self-phase modulation (SPM) and cross-phase modulation (XPM) for ultrashort light pulses (USP) in medium with electronic Kerr-nonlinearity are developed. The approach makes use of momentum operator of…
In an ultrafast optical-pump terahertz-probe measurement, the photoinduced material response can be modulated on a timescale shorter than the extent of the THz pulse. In this situation, the measured time-frequency response deviates from a…
Broadband energy-time entanglement can be used to enhance the rate of two-photon absorption (TPA) by combining a precise two-photon resonance with a very short coincidence time. Because of this short coincidence time, broadband TPA is not…
The effect of ordering field phase fluctuations on the normal and superconducting properties of a simple 2D model with a local four-fermion attraction is studied. Neglecting the coupling between the spin and charge degrees of freedom an…
We evaluate the advantages of performing cross-phase modulation (XPM) on a very-far-off-resonance atomic system. We consider a ladder system with a weak (few-photon level) control coherent field imparting a conditional nonlinear phase shift…
Two-dimensional (2D) spectroscopy combines high temporal and spectral resolution, allowing the observation of ultrafast energy transfer and the separation of homogeneous and inhomogeneous broadening. Typically, 2D spectroscopy is dominated…
Atomically thin two-dimensional (2D) semiconductors are extensively investigated for opto-electronic applications that require strong light-matter interactions. In view of such applications, it is essential to understand how…
Magnetic- and electric-dipole two-photon absorption (MED-TPA), recently introduced as a new spectroscopic technique for studying transitions between states of opposite parities, is investigated from a theoretical point of view. A new…
Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…
For decades since the development of phase-contrast optical microscopy, an analogous approach has been sought for maximizing the image contrast of weakly-scattering objects in transmission electron microscopy (TEM). The recent development…
A 2-D spatio-temporal analysis of terahertz generation by optical rectification of tilted-pulse-fronts is presented. Closed form expressions of terahertz transients and spectra in two spatial dimensions are furnished in the undepleted…
Pump-probe spectroscopy is a powerful tool to study ultrafast exciton dynamics, revealing the underlying complex interactions on the electronic scale. Despite significant advances in experimental techniques, developing a comprehensive and…
Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…
Triple sum-frequency (TSF) spectroscopy measures multidimensional spectra by resonantly exciting multiple quantum coherences of vibrational and electronic states. In this work we demonstrate pump-TSF-probe spectroscopy in which a pump…
Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…
The creation of high-quality cluster states in superconducting microwave circuits is a relevant ingredient in continuous-variable quantum computing. Although large-scale cluster states have been established in optical systems, dissipation…