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Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…

Optics · Physics 2021-07-07 Szilard Szoke , Manni He , Bryce P. Hickam , Scott K. Cushing

Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…

The investigation of fluorescence lifetime became an important tool in biology and medical science. So far, established methods of fluorescence lifetime measurements require the illumination of the investigated probes with pulsed or…

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of…

Quantum Physics · Physics 2022-05-31 Bryce P. Hickam , Manni He , Nathan Harper , Szilard Szoke , Scott Cushing

A quantum system composed of two or more subsystems can be in an entangled state, i.e. a state in which the properties of the global system are well defined but the properties of each subsystem are not. Entanglement is at the heart of…

Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission…

Quantum Physics · Physics 2020-08-10 Akihito Ishizaki

A pulsed source of entangled photons is desirable for some applications. Yet, such a source has intrinsic problems arising from the simultaneous arrival of the signal and noise photons to the detectors. These problems are analyzed and…

Optics · Physics 2015-06-18 Mónica B. Agüero , Alejandro A. Hnilo , Marcelo G. Kovalsky

Single photon avalanche diode arrays can provide both the spatial and temporal information of each detected photon. We present here the characterization of entangled light with a sensor specifically designed for quantum imaging…

Entangled photons can be used to make measurements with an accuracy beyond that possible with classical light. While most implementations of quantum metrology have used states made up of a single colour of photons, we show that entangled…

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

Fluorescence excitation by absorption of entangled photon pairs offers benefits compared to classical imaging techniques, such as the attainment of higher signal levels at low excitation power while simultaneously mitigating photo-toxicity.…

Quantum Physics · Physics 2023-11-02 Tobias Bernd Gäbler , Patrick Hendra , Nitish Jain , Markus Gräfe

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

Interaction of light with media often occurs with a femtosecond response time. Its measurement by conventional techniques requires the use of femtosecond lasers and sophisticated time-gated optical detection1-3. Here we demonstrate that by…

We consider ramifications of the use of high speed light modulators to questions of correlation and measurement of time-energy entangled photons. Using phase modulators, we find that temporal modulation of one photon of an entangled pair,…

Quantum Physics · Physics 2009-11-13 S. E. Harris

In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…

Quantum Physics · Physics 2026-04-24 Arunangshu Debnath , Shaul Mukamel

Quantum light is increasingly recognized as a promising resource for developing optical measurement techniques. Particular attention has been paid to enhancing the precision of the measurements beyond classical techniques by using…

Chemical Physics · Physics 2023-10-03 Yuta Fujihashi , Kuniyuki Miwa , Masahiro Higashi , Akihito Ishizaki

Entangled photons have attracted increasing interest as resources for developing time-resolved spectroscopic techniques. Theoretical studies suggest that their non-classical correlations enable time-resolved spectroscopy with monochromatic…

Chemical Physics · Physics 2025-12-01 Yuta Fujihashi , Akihito Ishizaki

Invariant entangled states remain unchanged under simultaneous identical unitary transformations of all their subsystems. We experimentally generate and characterize such invariant two-, four-, and six-photon polarization entangled states.…

Quantum Physics · Physics 2015-05-13 Magnus Radmark , Marcin Wiesniak , Marek Zukowski , Mohamed Bourennane

Entangled photon pairs form the foundation for many applications in the realm of quantum communication. For fiber-optic transfer of entangled photon pairs, time-bin encoding can potentially offer an improved stability compared to…

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