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We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

Quantum Physics · Physics 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

Frequency-bin entangled photons can be efficiently produced on-chip which offers a scalable, robust and low-footprint platform for quantum communication, particularly well-suited for resource-constrained settings such as mobile or…

We report measurements of time-frequency entangled photon pairs and heralded single photons at 1550~nm wavelengths generated using a microring resonator pumped optically by a diode laser. Along with a high spectral brightness of pair…

Quantum Physics · Physics 2018-02-14 Chaoxuan Ma , Xiaoxi Wang , Vikas Anant , Andrew D. Beyer , Matthew D. Shaw , Shayan Mookherjea

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or…

Particle entanglement is a fundamental resource upon which are based many quantum technologies. However, the up-to-now best sources of entangled photons rely on parametric down-conversion processes, which are optimal only at certain…

Entangled photons, generated by spontaneous parametric down-conversion from a second-order nonlinear crystal, present a rich potential for imaging and image-processing applications. Since this source is an example of a three-wave mixing…

Quantum Physics · Physics 2015-06-26 Ayman F. Abouraddy , Bahaa E. A. Saleh , Alexander V. Sergienko , Malvin C. Teich

Photon entanglement is an important state of light that is at the basis of many protocols in photonic quantum technologies, from quantum computing, to simulation and sensing. The capability to generate entangled photons in integrated…

Entangling independent photons is not only of fundamental interest but also of crucial importance for quantum information science. Two-photon interference is a major method to entangle independent identical photons. If two photons are…

Quantum Physics · Physics 2015-01-27 Tian-Ming Zhao , Han Zhang , Jian Yang , Zi-Ru Sang , Xiao Jiang , Xiao-Hui Bao , Jian-Wei Pan

Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that…

Quantum Physics · Physics 2021-08-25 Stefan Lerch , André Stefanov

We present an experimental demonstration of the full control of the frequency correlations of entangled photon pairs. The joint spectrum of photon pairs is continuously varied from photons that exhibit anticorrelation in frequency to…

Quantum Physics · Physics 2009-08-14 M. Hendrych , M. Mičuda , A. Valencia , J. P. Torres

The generation of entangled photon pairs by parametric down--conversion from solid state CW lasers with small coherence time is theoretically and experimentally analyzed. We consider a compact and low-cost setup based on a two-crystal…

Quantum Physics · Physics 2009-04-16 Simone Cialdi , Fabrizio Castelli , Matteo G. A. Paris

Pairs of photons entangled in their time-frequency degree of freedom are of great interest in quantum optics research and applications, due to their relative ease of generation and their high capacity for encoding information. Here we…

Quantum Physics · Physics 2022-02-23 Sofiane Merkouche , Valérian Thiel , Brian J. Smith

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

Quantum Physics · Physics 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

The non-classical spectral and temporal features of entangled photons offer new possibilities to investigate the interactions of excitons in photosynthetic complexes, and to target the excitation of specific states. Simulations of…

Quantum Physics · Physics 2012-11-05 Frank Schlawin , Konstantin Dorfman , Benjamin P. Fingerhut , Shaul Mukamel

A monochromatic laser pumping a parametric down conversion crystal generates frequency entangled photon pairs. We study this experimentally by addressing such frequency entangled photons at telecommunication wavelengths (around 1550 nm)…

Quantum Physics · Physics 2015-05-14 L. Olislager , J. Cussey , A. T. Nguyen , Ph. Emplit , S. Massar , J. -M. Merolla , K. Phan Huy

We introduce a scalable photonic platform that enables efficient generation of entangled photon pairs from a semiconductor quantum dot. Our system, which is based on a self-aligned quantum dot-micro-cavity structure, erases the need for…

Entangled photons have the remarkable ability to be more sensitive to signal and less sensitive to noise than classical light. Joint photons can sample an object collectively, resulting in faster phase accumulation and higher spatial…

Optics · Physics 2015-09-04 Chien-Hung Lu , Matthew Reichert , Xiaohang Sun , Jason W. Fleischer

We present a technique to completely characterise the spectral-temporal wave function of a broadband photon pair using spectral-shearing interferometry. Our method is fully self-referencing and is generalisable across a wide range of…

Quantum Physics · Physics 2018-09-12 Alex O. C. Davis , Valerian Thiel , Brian J. Smith

We propose a method to produce pure single photons with an arbitrary designed temporal shape in a heralded, lossless and scalable way. As the indispensable resource, the method uses pairs of time-energy entangled photons. To accomplish the…

Quantum Physics · Physics 2017-10-18 Valentin Averchenko , Denis Sych , Gerd Leuchs

We extend entangled coincidence (ghost) imaging to fluorescent samples. Given the entangled photon correlation, one photon of the pair carries information on where the other photon has been absorbed and has produced fluorescence in a…

Quantum Physics · Physics 2009-11-13 Giuliano Scarcelli , Seok Hyun Yun