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We introduce chiral rotational spectroscopy: a new technique that enables the determination of the orientated optical activity pseudotensor components $B_{XX}$, $B_{YY}$ and $B_{ZZ}$ of chiral molecules, in a manner that reveals the…

Atomic and Molecular Clusters · Physics 2018-01-16 Robert P. Cameron , Jörg B. Götte , Stephen M. Barnett

Chiral phonons have attracted significant attention due to their potential applications in spintronics, superconductivity, and advanced materials, but their detection has predominantly relied on indirect photon-involved processes. Here, we…

Materials Science · Physics 2025-07-29 Tingting Wang , Jun Zhou , Qingyong Ren , Lifa Zhang

The notion that phonons can carry pseudo-angular momentum has become popular in the last decade, with recent research efforts highlighting phonon chirality, Berry curvature of phonon band structure, and the phonon Hall effect. When a phonon…

Two-dimensional (2D) materials may host circular phonons, considered as chiral if the presence of a substrate breaks mirror symmetry. In 2D transition metal dichalcogenide (TMDC) monolayers lacking inversion symmetry, phonons with a given…

Materials Science · Physics 2025-09-16 Banhi Chatterjee , Peter Kratzer

Circularly polarized lattice vibrations carry angular momentum and lead to magnetic responses in applied magnetic fields or when resonantly driven with ultrashort laser pulses. Recent measurements have found responses that are orders of…

Mesoscale and Nanoscale Physics · Physics 2024-09-05 Swati Chaudhary , Dominik M. Juraschek , Martin Rodriguez-Vega , Gregory A. Fiete

Lattice vibrations can carry angular momentum and magnetic moments under broken inversion or time-reversal symmetry, forming so-called chiral phonons. While such excitations have been explored in nonmagnetic systems via optical probes,…

The ability to control chirality and chiral phonons offers a route to manipulate the direction of spin and angular-momentum transport. In materials with rigid structural chirality, such as quartz, phonon chirality is fixed by the handedness…

In ionic materials, circularly polarized phonons carry orbital magnetic moments that arise from circular motions of the ions, and which interact with other magnetic moments or fields. Here, we calculate the orbital magnetic moments of…

Materials Science · Physics 2019-06-12 Dominik M. Juraschek , Nicola A. Spaldin

The elucidation of the mechanisms behind chiral-induced spin selectivity remains an outstanding scientific challenge. Here we consider the role of delocalised phonon modes in electron transport in chiral structures and demonstrate that spin…

Mesoscale and Nanoscale Physics · Physics 2023-01-12 Clemens Vittmann , James Lim , Dario Tamascelli , Susana F. Huelga , Martin B. Plenio

Lattice vibrations carrying angular momentum, known as chiral phonons, have emerged as a promising route to control and understand complex material properties, yet their deterministic manipulation remains largely unexplored. Here we…

Chirality is a fundamental concept in physics that underpins various phenomena in nonlinear optics, quantum physics, and topological photonics. Although the spin of a photon naturally brings chirality, orbital angular momentum can also…

Chiral phonons, originally identified in two-dimensional hexagonal lattices and later extended to kagome, square, and other lattices, have been extensively studied as manifestations of broken inversion and time-reversal symmetries in…

Statistical Mechanics · Physics 2025-11-03 Ravi Kiran , A. Taraphder

Chirality is a fundamental symmetry concept describing discrete states, i.e., left-handed, right-handed, or achiral, and existing at disparate scales and in many categories of scientific fields. Even though symmetry breaking is…

Ferrochiral materials with an achiral-to-chiral phase transition and switchable chirality have unique application opportunities, enabling control of the angular momentum of circularly polarized lattice vibrations (chiral phonons) and…

Materials Science · Physics 2025-07-24 C. R. Zeiger , R. S. Dragland , R. Sjökvist , R. Beanland , D. Meier , T. Grande , M. S. Senn , O. G. Grendal

Chiral functionalities exhibited by systems lacking any mirror symmetry encompass natural optical activity, magnetochiral effect, diagonal current-induced magnetization, chirality-selective spin-polarized current of charged electrons or…

Materials Science · Physics 2024-10-01 Sang-Wook Cheongand Fei-Ting Huang

Topology and chirality of fermionic quasiparticles have enabled exciting discoveries, including quantum anomalous Hall liquids and topological superconductivity. Recently, topological and chiral phonons emerge as new and fast-evolving…

Materials Science · Physics 2025-04-16 Tiantian Zhang , Shuichi Murakami , Hu Miao

The direct, ultrafast excitation of polar phonons with electromagnetic radiation is a potent strategy for controlling the properties of a wide range of materials, particularly in the context of influencing their magnetic behavior. Here, we…

Mesoscale and Nanoscale Physics · Physics 2024-05-01 R. Merlin

We propose a mechanism to obtain chiral phonon-like excitations from the bond-dependent magnetoelastic couplings in the absence of out-of-plane magnetization and magnetic fields. By mapping the hybrid excitation to its phononic analog, we…

Mesoscale and Nanoscale Physics · Physics 2025-01-03 Bowen Ma , Z. D. Wang , Gang V. Chen

In continuum mechanics, the non-centrosymmetric micropolar theory is usually used to capture the chirality inherent in materials. However when reduced to a two dimensional (2D) isotropic problem, the resulting model becomes non-chiral.…

Materials Science · Physics 2015-06-04 X. N. Liu , G. L. Huang , G. K. Hu

We propose a method for detecting single chiral phonons that will enable their use as dark-matter detectors. We suggest metal--organic frameworks (MOFs) as detector materials, as their flexibility yields low-energy chiral phonons with…

High Energy Physics - Phenomenology · Physics 2023-12-20 Carl P. Romao , Riccardo Catena , Nicola A. Spaldin , Marek Matas