Related papers: Chiral phonons probed by X rays
The interplay between different degrees of freedom in condensed matter systems engenders a rich variety of emergent phenomena. In particular, fermions with non-trivial quantum geometry can generate Chern-Simons (CS)-like terms in effective…
Coupling between light and material excitations underlies a wide range of optical phenomena. Polaritons are eigenstates of a coupled system with hybridized wave function. Owing to their hybrid composition, polaritons exhibit at the same…
We have developed a microscopic theory on phonon energy dispersion in chiral crystals within a harmonic approximation. One of the main issues is about the splitting of sound velocity of acoustic phonons with opposite ``crystal'' angular…
Hexagonal two-dimensional materials with broken inversion symmetry (as BN or transition metal dichalcodenides) are known to sustain chiral phonons with finite angular momentum, adding a further useful degree of freedom to the extraordinary…
Valley degrees of freedom in transition-metal dichalcogenides influence thoroughly electron-phonon coupling and its nonequilibrium dynamics. We conducted a first-principles study of the quantum kinetics of chiral phonons following…
This article reviews recent theoretical developments in the ab initio study of polarons in materials. The polaron is an emergent quasiparticle that arises from the interaction between electrons and phonons in solids, and consists of an…
Chiral symmetry breaking of phonons plays an essential role in emergent quantum phenomena owing to its strong coupling to spin degree of freedom. However, direct experimental evidence of the chiral phonon-spin coupling is lacking. In this…
We propose a macroscopic theory of optical phonons, Fr{\"o}hlich polarons, and exciton-polarons in two-dimensional (2D) polar crystalline monolayers. Our theory extends the classical macroscopic formulation of the electron-phonon problem in…
Chiral phonons offer a route to transfer angular momentum without relying on magnetic order, but their electronic response in metals remains poorly understood from perspectives beyond spin-based scenarios. Using first-principles…
The control and detection of crystallographic chirality is an important and challenging scientific problem. Chirality has wide ranging implications from medical physics to cosmology including an intimate but subtle connection in magnetic…
Chirality and topology are fundamental and ubiquitous in nature. Symmetry has proven to be a powerful tool for predicting topological phonons. However, to date, topological phonon emergent particles (EMPs) have not been systematically…
Condensed-matter and other engineered systems, such as cold atoms, photonic, or phononic metamaterials, have proven to be versatile platforms for the observation of low-energy counterparts of elementary particles from relativistic field…
Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…
Immersing a mobile impurity in a quantum many-body environment can reveal fundamental properties of the background medium, hence providing a powerful probe of quantum matter. This approach is particularly intriguing when considering media…
Time-reversal symmetry (TRS) is pivotal for materials optical, magnetic, topological, and transport properties. Chiral phonons, characterized by atoms rotating unidirectionally around their equilibrium positions, generate dynamic lattice…
Metasurfaces, the two-dimensional analogues of metamaterials, are ideal platforms for sensing molecular chirality at the nanoscale, e.g. of inclusions of natural optically active molecules, as they offer large accessible areas (they are…
Chiral structures that produce asymmetric spin-phonon coupling can theoretically generate spin-phonon polarons -- quasiparticles exhibiting non-degenerate spin states with phonon displacements. These quasiparticles are speculated to be the…
Organic/inorganic interfaces formed by monolayer substrates and conjugated molecular adsorbates are attractive material platforms leveraging the modularity of organic compounds together with the long-range phenomena typical of condensed…
Unlike the chirality of electrons, the intrinsic chirality of phonons has only surfaced in recent years. Here we report on the effects of the interaction between electrons and chiral phonons in two-dimensional materials by using a…
In crystals with broken time-reversal symmetry, zone-center phonons can acquire a finite angular momentum via velocity-dependent forces on the nuclei. Despite having the same order of magnitude as the electron spin angular momentum, the…