English

Spin-Dependent Momentum Conservation of Electron-Phonon Scattering in Chirality-Induced Spin Selectivity

Mesoscale and Nanoscale Physics 2023-01-12 v1 Chemical Physics Quantum Physics

Abstract

The elucidation of the mechanisms behind chiral-induced spin selectivity remains an outstanding scientific challenge. Here we consider the role of delocalised phonon modes in electron transport in chiral structures and demonstrate that spin selectivity can originate from spin-dependent energy and momentum conservation in electron-phonon scattering events. While this mechanism is robust to the specifical nature of the vibrational modes, the degree of spin polarization depends on environmental factors, such as external driving fields, temperatures and phonon relaxation rates. This dependence is used to present experimentally testable predictions of our model.

Keywords

Cite

@article{arxiv.2209.05323,
  title  = {Spin-Dependent Momentum Conservation of Electron-Phonon Scattering in Chirality-Induced Spin Selectivity},
  author = {Clemens Vittmann and James Lim and Dario Tamascelli and Susana F. Huelga and Martin B. Plenio},
  journal= {arXiv preprint arXiv:2209.05323},
  year   = {2023}
}