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Donor-acceptor (D-A) type copolymers show great potential for the application in the active layer of organic solar cells. Nevertheless the nature of the excited states, the coupling mechanism and the relaxation pathways following…

Electron-beam-induced luminescence typically relies on direct excitation by high energy primary electrons. Here, we explore properties of an alternative excitation approach where cathodoluminescence (CL) is driven by substrate-generated…

Optics · Physics 2026-04-01 Sven Ebel , N. Asger Mortensen , Sergii Morozov

To explore nontrivial photoinduced modulations of charge correlations, we theoretically study photoinduced dynamics in quarter-filled extended Hubbard models with competing intersite repulsive interactions on triangular lattices with…

Strongly Correlated Electrons · Physics 2017-01-27 Kenji Yonemitsu

Active fluids refer to the fluids that contain self-propelled particles such as bacteria or micro-algae, whose properties differ fundamentally from the passive fluids. Such particles often exhibit an intermittent motion, with high-motility…

Biological Physics · Physics 2020-03-05 Thomas Vourc'h , Julien Léopoldès , Hassan Peerhossaini

The current understanding of charge transfer dynamics in Charge-Coupled Devices (CCDs) is that charge is moved so quickly from one phase to the next in a clocking sequence and with a density so low that trapping of charge in the inter-phase…

Instrumentation and Methods for Astrophysics · Physics 2018-01-04 Jesper Skottfelt , David J. Hall , Ben Dryer , Nathan Bush , Jason Gow , Andrew Holland

We present the first time-dependent density-functional theory (TDDFT) calculation on a light harvesting triad carotenoid-diaryl-porphyrin-C60. Besides the numerical challenge that the ab initio study of the electronic structure of such a…

Materials Science · Physics 2009-03-13 N. Spallanzani , C. A. Rozzi , D. Varsano , T. Baruah , M. R. Pederson , F. Manghi , A. Rubio

We investigate the optical excitation spectra and the photoluminescence depolarization dynamics in bilayer WS$_2$. A different understanding of the optical excitation spectra in the recent photoluminescence experimentby Zhu {\em et al.}…

Mesoscale and Nanoscale Physics · Physics 2014-07-25 T. Yu , M. W. Wu

We have evaluated excitation energy transfer rates in photosyntetic complexes using the exact HEOM method and various approximate methods frequently used in the literature, namely, the F\"orster method, the Redfield method, the modified…

Chemical Physics · Physics 2014-05-19 Simon Jesenko , Marko Žnidarič

We studied the recombination dynamics of charge carriers in organic bulk heterojunction solar cells made of the blend system poly(2,5-bis(3-dodecyl thiophen-2-yl) thieno[2,3-b]thiophene) (pBTCT-C12):[6,6]-phenyl-C61-butyric acid methyl…

Ultrafast photoinduced dynamics of electronic excitation in molecular dimers is drastically affected by the dynamic reorganization of inter- and intra- molecular nuclear configuration modeled by a quantized nuclear degree of freedom [Cina…

Mathematical Physics · Physics 2009-11-10 Dmitri S. Kilin , Yuri V. Pereversev , Oleg V. Prezhdo

Energy transfer in the photosynthetic complex of the Green Sulfur Bacteria known as the Fenna-Matthews-Olson (FMO) complex is studied theoretically taking all three subunits (monomers) of the FMO trimer and the recently found eighth…

Quantum Physics · Physics 2012-02-07 G. Ritschel , J. Roden , W. T. Strunz , A. Aspuru-Guzik , A. Eisfeld

Photosynthesis, the process by which energy from sunlight drives cellular metabolism, relies on a unique organization of light-harvesting and reaction center complexes. Recently, the organization of light-harvesting LH2 complexes and…

Biological Physics · Physics 2011-11-02 Elad Harel

Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 K. Beltako , F. Michelini , N. Cavassilas , L. Raymond

Apparent recombination orders exceeding the value of two expected for bimolecular recombination have been reported for organic solar cells in various publications. Two prominent explanations are bimolecular losses with a carrier…

Soft Condensed Matter · Physics 2012-08-23 D. Rauh , C. Deibel , V. Dyakonov

We calculate the bulk photovoltaic response of the ferroelectrics BaTiO$_3$ and PbTiO$_3$ from first principles by applying "shift current" theory to the electronic structure from density functional theory. The first principles results for…

Materials Science · Physics 2015-06-04 Steve M. Young , Andrew M. Rappe

Diffusion-driven processes are important phenomena of materials science in the field of energy conversion and transmission. During the conversion from chemical energy to electrical energy, the species diffusion is generally linked to the…

Applied Physics · Physics 2021-02-23 Jay Santoki

Hybrid interfaces formed by inorganic semiconductors and organic molecules are intriguing materials for opto-electronics. Interfacial charge transfer is primarily responsible for their peculiar electronic structure and optical response.…

Materials Science · Physics 2020-04-15 Matheus Jacobs , Jannis Krumland , Ana M. Valencia , Haiyuan Wang , Mariana Rossi , Caterina Cocchi

We investigate the quantum dynamics of energy and charge transfer in a wheel-shaped artificial photosynthetic antenna-reaction center complex.This complex consists of six light-harvesting chromophores and an electron-acceptor fullerene. To…

Biological Physics · Physics 2015-05-28 Pulak Kumar Ghosh , Anatoly Yu. Smirnov , Franco Nori

The realm of latent heat storage has witnessed emergence of optical charging as a promising route of solar thermal latent heat storage. However, it is still in its initial stages of development and warrants further investigations to take it…

Applied Physics · Physics 2023-12-13 Domala Sai Suhas , Vikrant Khullar

Two distinct approaches, the Frenkel-Dirac time-dependent variation and the Haken-Strobl model, are adopted to study energy transfer dynamics in single-ring and double-ring light-harvesting systems in purple bacteria. It is found that…

Chemical Physics · Physics 2015-06-05 Jun Ye , Kewei Sun , Yang Zhao , Yunjin Yu , Chee Kong Lee , Jianshu Cao
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