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We explore a pure optical method for enantioselective orientation of chiral molecules by means of laser fields with twisted polarization. Several field implementations are considered, including a pair of delayed cross-polarized laser…

Chemical Physics · Physics 2018-03-23 I. Tutunnikov , E. Gershnabel , S. Gold , I. Sh. Averbukh

We have investigated the angle-resolved ATI spectrum of oriented molecules in the IR+XUV co-rotating circular laser fields. According to the different roles of IR and XUV laser in the ionization process, we purposefully adjust the photon…

Atomic Physics · Physics 2024-01-15 Yu-Hong Li , Facheng Jin , Yujun Yang , Fei Li , Ying-Chun Guo , Zhi-Yi Wei , Jing Chen , Xiaojun Liu , Bingbing Wang

Electron quantum path interferences in strongly laser-driven aligned molecules and their dependence on the molecular alignment is an essential open problem in strong-field molecular physics. Here, we demonstrate an approach which provides…

Electrons colliding with spatially fixed ions in strong laser fields are investigated by solving the time-dependent Schr\"odinger equation. Considering first simple one-dimensional model systems, the mechanisms and energy spectra of fast…

Atomic Physics · Physics 2015-10-28 S. Bauch , M. Bonitz

We present a combined theoretical and experimental work investigating the angle-resolved phases of the photoionization process driven by a two-color field consisting of an attosecond pulse train and an infrared pulse in an ensemble of…

We give a framework for molecular multiphoton excitation process induced by an optimally designed electric field. The molecule is initially prepared in a coherent superposition state of two of its eigenfunctions. The relative phase of the…

Chemical Physics · Physics 2009-11-10 Bijoy K Dey

We present a theoretical study of the wave packet dynamics of the H$_2^+$ molecular ion in plasmon-enhanced laser fields. Such fields may be produced, for instance, when metallic nano-structures are illuminated by a laser pulse of moderated…

Atomic Physics · Physics 2016-07-08 I. Yavuz , M. F. Ciappina , A. Chacón , Z. Altun , M. Lewenstein

We discuss double ionization of atoms in strong laser pulses using a reduced dimensionality model. Following the insights obtained from an analysis of the classical mechanics of the process, we confine each electron to move along the lines…

Atomic Physics · Physics 2008-08-06 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

Non Born-Oppenheimer quantum dynamics of H$_{2}^{+}$ excited by shaped one-cycle laser pulses linearly polarized along the molecular axis have been studied by the numerical solution of the time-dependent Schr\"odinger equation within a…

Atomic and Molecular Clusters · Physics 2017-08-02 Guennaddi K. Paramonov , Oliver Kühn , Andre D. Bandrauk

We present a method for retrieving of single-active electron potential in an atom or molecule from a given momentum distribution of photoelectrons ionized by a strong laser field. In this method the potential varying within certain limits…

Atomic Physics · Physics 2021-07-07 N. I. Shvetsov-Shilovski

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

Quantum Physics · Physics 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

The impact of nonadiabatic laser-induced molecular alignment on filamentation is numerically studied. Weak and strong field model of impulsive molecular alignment are compared in the context of nonlinear pulse propagation. It is shown that…

Optics · Physics 2014-12-03 N. Berti , P. Béjot , J. -P. Wolf , O. Faucher

The method of zero range potential (ZRP) for one-electron problems is reviewed. In the absence of an external electromagnetic field, the notion of a ZRP is introduced from different points of view and for an arbitrary dimension of space.…

Atomic Physics · Physics 2009-07-14 Denys I. Bondar , Ryan Murray , Misha Yu. Ivanov

We extend our finite difference time domain method for numerical solution of the Schrodinger equation to cases where eigenfunctions are complex-valued. Illustrative numerical results for an electron in two dimensions, subject to a confining…

Computational Physics · Physics 2008-07-05 I. Wayan Sudiarta , D. J. Wallace Geldart

We investigate theoretically the Casimir-Polder potential of an atom which is driven by a laser field close to a surface. This problem is addressed in the framework of macroscopic quantum electrodynamics using the Green's tensor formalism…

Quantum Physics · Physics 2018-08-29 Sebastian Fuchs , Robert Bennett , Stefan Yoshi Buhmann

The ionization probability of N$_2$, O$_2$, and CO$_2$ in intense laser fields is studied theoretically as a function of the alignment angle by solving the time-dependent Schr\"odinger equation numerically assuming only the…

Atomic Physics · Physics 2015-05-18 Simon Petretti , Yulian V. Vanne , Alejandro Saenz , Alberto Castro , Piero Decleva

The lack of a direct map between control fields and desired control objectives poses a significant challenge in applying quantum control theory to quantum technologies. Here, we propose an analytical framework to precisely control a limited…

Quantum Physics · Physics 2025-03-05 Qian-Qian Hong , Daoyi Dong , Niels E. Henriksen , Franco Nori , Jun He , Chuan-Cun Shu

We investigate the formation and control of stationary optical patterns in a cold Rydberg atomic gas via double electromagnetically induced transparency. We show that, through the modulational instability of plane-wave state of a laser…

Quantum Gases · Physics 2021-07-21 Zeyun Shi , Guoxiang Huang

The strong coupling between intense laser fields and valence electrons in molecules causes a distortion of the potential energy hypersurfaces which determine the motion of nuclei in a molecule and influences possible reaction pathways. The…

We theoretically and numerically analyze x-ray scattering from asymmetric-top molecules three-dimensionally aligned using elliptically polarized laser light. A rigid-rotor model is assumed. The principal axes of the polarizability tensor…

Atomic Physics · Physics 2010-05-07 Stefan Pabst , Phay J. Ho , Robin Santra