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We study the excitation of asymmetric-top (including chiral) molecules by two-color femtosecond laser pulses. In the cases of non-chiral asymmetric-top molecules excited by an orthogonally polarized two-color pulse, we demonstrate,…

Optics · Physics 2021-09-16 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

A nonlocal quantum model is presented for calculating the atomic dielectric response to a strong laser electric field. By replacing the Coulomb potential with a nonlocal potential in the Schrodinger equation, a 3+1D calculation of the…

Atomic Physics · Physics 2015-06-18 T. C. Rensink , T. M. Antonsen , J. P. Palastro , D. Gordon

We investigate the full control over the orientation of a non-symmetric molecule by using moderate and weak electric fields. Quantum Optimal Control techniques allow us to orient any axis of 6-chloropyridazine-3-carbonitrile, which is taken…

Quantum Physics · Physics 2023-11-21 Rosario González-Férez , Juan J. Omiste

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer

Coherent control of chaotic molecular systems, using laser-assisted alignment of sulphur dioxide (SO$_2$) molecules in the presence of a static electric field as an example, is considered. Conditions for which the classical version of this…

Chemical Physics · Physics 2017-04-26 Johannes Floß , Paul Brumer

In this paper, we studied the optimal alignment and anti-alignment of O2 molecules by femtosecond laser pulse under different input energy. The results show that there is an energy limit in molecular alignment. The optimal molecular…

Optics · Physics 2023-03-16 Yue-Xun Li , Tao Du

The alternative to dynamic alignment explanation of experimental results on spatial-asymmetric dissociation of molecules in a laser field is proposed. The concept of geometrical alignment is sufficient for explanation of these results. In…

Optics · Physics 2007-05-23 V. A. Kuz'menko

We present a general mathematical procedure to handle interactions described by a Morse potential in the presence of a strong harmonic excitation. We account for permanent and field-induced terms and their gradients in the dipole moment…

Atomic Physics · Physics 2023-07-19 Sándor Varró , Szabolcs Hack , Gábor Paragi , Péter Földi , Imre F. Barna , Attila Czirják

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

We present an algebraic method for treating molecular vibrations in the Morse potential perturbed by an external laser field. By the help of a complete and normalizable basis we transform the Schr\"{o}dinger equation into a system of…

Quantum Physics · Physics 2009-11-07 Balazs Molnar , Peter Foldi , Mihaly G. Benedict , Ferenc Bartha

Globally optimal solution describing a phase conjugated field of Raman scattering on the resonant $B\gets X$ transition of iodine $I_2$ is studied. Maximum optical coherence is found as a top eigenvalue problem. A reversibility theorem has…

Optics · Physics 2009-09-29 V. M. Akulin , V. A. Dubovitskii , A. M. Dykhne , A. G. Rudavets

By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…

Atomic Physics · Physics 2008-04-04 Toru Morishita , Anh-Thu Le , Zhangjin Chen , C. D. Lin

We consider deflection of rotating symmetric molecules by inhomogeneous optical and static electric fields, compare results with the case of linear molecules, and find new singularities in the distribution of the scattering angle.…

Chemical Physics · Physics 2015-05-28 Erez Gershnabel , Ilya Sh. Averbukh

We extend the superconductor's free energy to include an interaction of the order parameter with the curvature of space-time. This interaction leads to geometry dependent coherence length and Ginzburg-Landau parameter which suggests that…

General Physics · Physics 2017-06-29 Victor Atanasov

We solve the three-dimensional time-dependent Schr\"{o}dinger equation for a few-cycle circularly polarized femtosecond laser pulse interacting with an oriented target exemplified by an Argon atom, initially in a $3\text{p}_{x}$ or…

Atomic Physics · Physics 2015-05-18 C. P. J. Martiny , M. Abu-samha , L. B. Madsen

We investigate the orientation dependence of high-order harmonic generation (HHG) from H$_2^+$ with different internuclear distances irradiated by intense laser fields both numerically and analytically. The calculated molecular HHG spectra…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jie Liu , Bambi Hu

We investigate the photoelectron angular emission distributions obtained by strong field dissociative ionization of H$_2$ using cold target recoil ion momentum spectroscopy. In case of employing laser light with an ellipticity close to 0.9…

Collective coherent scattering of laser light by an ensemble of polarizable point particles creates long range interactions, whose properties can be tailored by choice of injected laser powers, frequencies and polarizations. We use a…

Quantum Physics · Physics 2015-06-17 Stefan Ostermann , Matthias Sonnleitner , Helmut Ritsch

We present a numerical method for investigating the non-perturbative quantum mechanical interaction of light with atoms in two dimensions, without a basis expansion. This enables us to investigate intense laser-atom interactions with light…

Quantum Physics · Physics 2009-10-30 M. Protopapas , D. G. Lappas , P. L. Knight
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