Related papers: Field-free molecular alignment by the optimized tw…
Combining the features of molecular wires and femtosecond laser pulses gives the unique opportunity to optically switch electron currents in molecular devices with very high speed. Based on a weak-coupling approximation between wire and…
To solve the time-dependent Schr\"odinger equation in spatially inhomogeneous pulses of electromagnetic radiation, we propose an iterative semi-classical complex trajectory approach. In numerical applications, we validate this method…
Strong optical laser fields modify the way x rays interact with matter. This allows us to use x rays to gain deeper insight into strong-field processes. Alternatively, optical lasers may be utilized to control the propagation of x rays…
A strong inhomogeneous static electric field is used to spatially disperse a rotationally cold supersonic beam of 2,6-difluoroiodobenzene molecules according to their rotational quantum state. The molecules in the lowest lying rotational…
Machine learning for predicting control landscape maps of full quantum molecular dynamics is examined through a case study of the laser-induced three-dimensional (3D) alignment of asymmetric top molecules, an essential technique for…
The Schrodinger equation for an electron near an azimuthally symmetric curved surface $\Sigma$ in the presence of an arbitrary uniform magnetic field $\mathbf B$ is developed. A thin layer quantization procedure is implemented to bring the…
A symmetry analysis is presented for the three-dimensional nonrelativistic motion of charged particles in arbitrary stationary electromagnetic fields. The general form of the Lie point symmetries is found along with the fields that respect…
We study the resonances of $2\times 2$ systems of one dimensional Schr\"odinger operators which are related to the mathematical theory of molecular predissociation. We determine the precise positions of the resonances with real parts below…
The Schr\"odinger equation for a charged particle in the field of a nonrelativistic electric quadrupole in two dimensions is known to be separable in spherical coordinates. We investigate the occurrence of bound states of negative energy…
In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…
We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…
We demonstrate the control of electron-electron correlation in frustrated double ionization (FDI) of the two-electron triatomic molecule D$_{3}^{+}$ when driven by two orthogonally polarized two-color laser fields. We employ a…
We analyze the imprint of nodal planes in high-order harmonic spectra from aligned diatomic molecules in intense laser fields whose components exhibit orthogonal polarizations. We show that the typical suppression in the spectra associated…
We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…
We report the first observation of free-electron angular momentum wave packets generated by atomic multiphoton ionization with bichromatic three-dimensional (3D) polarization-tailored ultrashort laser fields. These fields, created by the…
Several families of nonlinear field equations are known to possess space- localized singularity-free solutions which describe fields with finite Hermitian norms. This paper studies the interaction of such fields with given electromagnetic…
Spectra of circularly polarized harmonics is calculated by numerically solving the Time-Dependent Schr\"{o}dinger Equation for a 2D model of Ne atom using circularly polarized fundamental with counter-rotating second harmonic laser fields.…
We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…
Oriented external electric fields are ubiquitous in chemistry; however, the effects of fields applied in different directions on molecular systems remain underexplored. A major challenge is that an applied field exerts a torque on a…
We present a new dimensional scaling transformation of the Schrodinger equation for the two electron bond. This yields, for the first time, a good description of the two electron bond via D-scaling. There also emerges, in the large-D limit,…