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We present theory and calculations for coherent high-fidelity quantum control of many-particle states in semiconductor quantum wells. We show that coupling a two-electron double quantum dot to a terahertz optical source enables targeted…

Mesoscale and Nanoscale Physics · Physics 2013-02-04 E. Rasanen , T. Blasi , M. F. Borunda , E. J. Heller

Strong spin-orbit coupling in transition metal dichalcogenide (TMDC) monolayers results in spin resolvable band structures about the $K$ and $K'$ valleys such that the eigenbasis of a 2D quantum dot (QD) in a TMDC monolayer in zero field is…

Mesoscale and Nanoscale Physics · Physics 2018-04-25 Matthew Brooks , Guido Burkard

We theoretically investigated the coupling between the exciton internal and center-of-mass motions in monolayer transition metal dichalcogenides subjected to a periodic electrostatic potential. The coupling leads to the emergence of…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Fujia Lu , Qianying Hu , Yang Xu , Hongyi Yu

Present proposals for the realisation of entangled photon pair sources using the radiative decay of the biexciton in semiconductor quantum dots are limited by the need to enforce degeneracy of the two intermediate, single exciton states. We…

The equilibrium and non-equilibrium optical properties of single-layer transition metal dichalcogenides (TMDs) are determined by strongly bound excitons. Exciton relaxation dynamics in TMDs have been extensively studied by time-domain…

Electron spins in silicon quantum dots are excellent qubits because they have long coherence times, high gate fidelities, and are compatible with advanced semiconductor manufacturing techniques. The valley degree of freedom, which results…

Mesoscale and Nanoscale Physics · Physics 2023-03-27 Xinxin Cai , Elliot J. Connors , John M. Nichol

Layered transition metal dichalcogenides (TMDCs) host a variety of strongly bound exciton complexes that control the optical properties in these materials. Apart from spin and valley, layer index provides an additional degree of freedom in…

Mesoscale and Nanoscale Physics · Physics 2019-05-08 Sarthak Das , Garima Gupta , Kausik Majumdar

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

While conventional semiconductor technology relies on the manipulation of electrical charge for the implementation of computational logic, additional degrees of freedom such as spin and valley offer alternative avenues for the encoding of…

The concept of valleytronics has recently gained considerable research attention due to its intriguing physical phenomena and practical applications in optoelectronics and quantum information. In this study, by employing GW-BSE calculations…

Materials Science · Physics 2024-01-22 Vo Khuong Dien , Pham Thi Bich Thao , Nguyen Thi Han , Nguyen Thanh Tien

Fabricating van der Waals (vdW) bilayer heterostructures (BL-HS) by stacking the same or different two-dimensional (2D) layers, offers a unique physical system with rich electronic and optical properties. Twist-angle between component…

Mesoscale and Nanoscale Physics · Physics 2020-12-17 Kha Tran , Junho Choi , Akshay Singh

Electron transfer to an individual quantum dot promotes the formation of charged excitons with enhanced recombination pathways and reduced lifetimes. Excitons with only one or two extra charges have been observed and exploited for very…

Current semiconductor qubits rely either on the spin or on the charge degree of freedom to encode quantum information. By contrast, in bilayer graphene the valley degree of freedom, stemming from the crystal lattice symmetry, is a robust…

We show that inversion symmetry breaking together with spin-orbit coupling leads to coupled spin and valley physics in monolayers of MoS2 and other group-VI dichalcogenides, making possible controls of spin and valley in these 2D materials.…

Mesoscale and Nanoscale Physics · Physics 2012-05-09 Di Xiao , Gui-Bin Liu , Wanxiang Feng , Xiaodong Xu , Wang Yao

Two-dimensional (2D) van-der-Waals materials are a promising platform for exciton state engineering. In this paper, we study the properties of excitons in 2D group VI transition-metal dichalcogenide (TMD) semiconductors that are modified by…

Strongly Correlated Electrons · Physics 2026-05-08 Jose M. Torres-Lopez , Sudipta Kundu , Felipe H. da Jornada , Tony Heinz , Allan H. MacDonald

Excitons and their complexes govern optical-related behaviors in semiconductors. Here, using angle-resolved photoemission spectroscopy (ARPES), we have elucidated the light-matter interaction mediated by quasi-steady excitonic complexes…

Strongly Correlated Electrons · Physics 2025-12-03 Shangkun Mo , Hao Zhong , Keming Zhao , Yunfei Bai , Dingkun Qin , Chunlong Wu , Qiang Wan , Renzhe Li , Cao Peng , Xingzhe Wang , Enting Li , Sheng Meng , Nan Xu

Identifying multi-exciton states generated from singlet fission is key to understanding the carrier multiplication process, which presents a strategy for improving the efficiency of photovoltaics and bio-imaging. Broadband optically…

Mesoscale and Nanoscale Physics · Physics 2024-06-14 Yan Sun , M. Monteverde , V. Derkach , J. E. Anthony , A. D. Chepelianskii

Coupling between exciton states across the Brillouin zone in monolayer transition metal dichalcogenides can lead to ultrafast valley depolarization. Using time- and angle-resolved photoemission, we present momentum- and energy-resolved…

We show how the optical properties of a single semiconductor quantum dot can be controlled with a small dc voltage applied to a gate electrode. We find that the transmission spectrum of the neutral exciton exhibits two narrow lines with…

Mesoscale and Nanoscale Physics · Physics 2012-09-18 A. Högele , S. Seidl , M. Kroner , K. Karrai , R. J. Warburton , B. D. Gerardot , P. M. Petroff

Monolayer transition metal dichalcogenides feature tightly bound bright excitons at the degenerate valleys, where electron-hole Coulomb exchange interaction strongly couples the valley pseudospin to the momentum of exciton. Placed on…

Mesoscale and Nanoscale Physics · Physics 2022-06-01 Xu-Chen Yang , Hongyi Yu , Wang Yao
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