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We report the observation of superconductivity in infinite-layer Ca-doped LaNiO$_2$ (La$_{1-x}$Ca$_x$NiO$_2$) thin films and construct their phase diagram. Unlike the metal-insulator transition in Nd- and Pr-based nickelates, the undoped…

Superconductivity · Physics 2022-02-25 S. W. Zeng , C. J. Li , L. E. Chow , Y. Cao , Z. T. Zhang , C. S. Tang , X. M. Yin , Z. S. Lim , J. X. Hu , P. Yang , A. Ariando

The recent discovery of compressed superconductivity at 80~K in La$_3$Ni$_2$O$_7$-$\delta$ has brought nickelates into the family of unconventional high-temperature superconductors. However, due to the challenges of directly probing the…

Superconductivity · Physics 2025-09-17 Jianning Guo , Yuzhi Chen , Yulong Wang , Hualei Sun , Deyuan Hu , Meng Wang , Xiaoli Huang , Tian Cui

The discovery of high-Tc superconductivity around 80K in bilayer nickelate La3Ni2O7 under high pressure has expanded the family of high-Tc superconductors above the nitrogen boiling temperature. Recent studies have further shown that…

Superconductivity · Physics 2025-02-04 H C Regan B. Bhatta , Xiaoliang Zhang , Yong Zhong , Chunjing Jia

The discovery of superconductivity in a $d^{9-{\delta}}$ nickelate has inspired disparate theoretical perspectives regarding the essential physics of this class of materials. A key issue is the magnitude of the magnetic superexchange, which…

The pairing mechanism in cuprates remains as one of the most challenging issues in the field of condensed matter physics. The unique 3d9 electron orbital of the Cu2+ ionic states in cuprates is supposed to be the major player for the…

Superconductivity · Physics 2020-12-01 Qiangqiang Gu , Yueying Li , Siyuan Wan , Huazhou Li , Wei Guo , Huan Yang , Qing Li , Xiyu Zhu , Xiaoqing Pan , Yuefeng Nie , Hai-Hu Wen

The series of nickel-oxide compounds LaNiO$_3$ (formal Ni$(d^7)$), La$_2$NiO$_4$ (formal Ni$(d^8)$) and LaNiO$_2$ (formal Ni$(d^9)$) is investigated by first-principles many-body, using a combination of density functional theory,…

Strongly Correlated Electrons · Physics 2022-04-07 Frank Lechermann

The discovery of superconductivity in Sr-doped NdNiO$_{2}$ is a crucial breakthrough in the long pursuit for nickel oxide materials with electronic and magnetic properties similar to those of the cuprates. NdNiO$_2$ is the infinite-layer…

Superconductivity · Physics 2020-08-05 Emilian M. Nica , Jyoti Krishna , Rong Yu , Qimiao Si , Antia S. Botana , Onur Erten

Behaviours of hydrogen, such as fluidity and metallicity, are crucial for our understanding of planetary interiors and the emerging field of high-temperature superconducting hydrides. These behaviours were discovered in complex phase…

To investigate the detailed magnetic properties of a recently discovered superconducting nickelate Nd6Ni5O12, we performed the first-principles electronic structure calculation based on density functional theory. The band dispersion,…

Superconductivity · Physics 2024-10-02 Terri Yoon , Myung Joon Han

Several reports about infinite-layer nickelate thin films suggest that the superconducting critical temperature versus chemical doping phase diagram has a dome-like shape, similar to cuprates. Here, we demonstrate a highly reproducible…

After being expected as a promising analogue to cuprates for decades, superconductivity was recently discovered in infinite-layer nickelates, providing new opportunities to explore mechanisms of high-temperature superconductivity. However,…

The discovery of superconductivity in hole-doped infinite layer nickelates, RNiO2 (R = Nd, Pr, La) has garnered sustained interest in the field. A definitive picture of low-energy many-body states has not yet emerged. We provide new…

Strongly Correlated Electrons · Physics 2023-03-28 Gheorghe Lucian Pascut , Lucian Cosovanu , Kristjan Haule , Khandker F. Quader

In addition to the pressurized high-temperature superconductivity, bilayer and trilayer nickelate superconductors Lan+1NinO3n+1 (n = 2 and 3) exhibit many intriguing properties at ambient pressure, such as orbital-dependent electronic…

The striking discovery of high-temperature superconductivity (HTSC) of 80 K in a bilayer nickelate La$_3$Ni$_2$O$_7$ under a moderately high pressure of about 14 GPa ignited a new wave of studying HTSC in nickelates. The properties of the…

Recently, superconductivity with a $T_c$ up to 78 K has been reported in bulk samples of the bilayer nickelate La$_3$Ni$_2$O$_7$ at pressures above 14 GPa. Important theoretical tasks are the formulation of relevant low-energy models and…

Strongly Correlated Electrons · Physics 2023-11-17 Viktor Christiansson , Francesco Petocchi , Philipp Werner

We demonstrate in this paper that the recently discovered infinite-layer (IL) nickelates have much in common with a class of materials known as electrides. Oxide based electrides are compounds in which topotactic removal of loosely bound…

Superconductivity · Physics 2023-11-30 Kateryna Foyevtsova , Ilya Elfimov , George A. Sawatzky

To understand the superconductivity recently discovered in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, we carried out LDA+DMFT (local density approximation plus dynamical mean-field theory) and magnetic force response calculations. The on-site correlation…

Superconductivity · Physics 2020-02-25 Siheon Ryee , Hongkee Yoon , Taek Jung Kim , Min Yong Jeong , Myung Joon Han

The discovery of superconductivity in infinite-layer nickelates establishes a new category of unconventional superconductors that share structural and electronic similarities with cuprates. Despite exciting advances, such as the…

The discovery of superconductivity with Tc ~ 80 K in the nickelate Ruddlesden-Popper bilayer La3Ni2O7 at high pressure has opened a new platform for unconventional superconductivity, followed by the subsequent observation of…

Superconductivity · Physics 2026-04-22 Yang Zhang , Ling-Fang Lin , Thomas A. Maier , Elbio Dagotto

Superconducting states onsetting at moderately high temperatures have been observed in epitaxially-stabilized RENiO2-based thin films. However, recently it has also been reported that superconductivity at high temperatures is observed in…

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