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We present a general theory for using an optically pumped diamond nitrogen-vacancy center as a tunable, non-equilibrium bath to control a variety of nuclear spin dynamics (such as dephasing, relaxation, squeezing, polarization, etc.) and…

Quantum Physics · Physics 2019-08-17 Ping Wang , Jiangfeng Du , Wen Yang

We suggest a new spin orientation mechanism for localized electrons: $dynamic~electron~spin~polarization~provided~by~nuclear~spin~fluctuations$. The angular momentum for the electrons is gained from the nuclear spin system via the hyperfine…

Mesoscale and Nanoscale Physics · Physics 2020-10-14 D. S. Smirnov , T. S. Shamirzaev , D. R. Yakovlev , M. Bayer

The spin of a confined electron, when oriented originally in some direction, will lose memory of that orientation after some time. Physical mechanisms leading to this relaxation of spin memory typically involve either coupling of the…

Mesoscale and Nanoscale Physics · Physics 2013-07-24 A. C. Johnson , J. R. Petta , J. M. Taylor , A. Yacoby , M. D. Lukin , C. M. Marcus , M. P. Hanson , A. C. Gossard

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

Coherent two-level systems, or qubits, based on electron spins in GaAs quantum dots are strongly coupled to the nuclear spins of the host lattice via the hyperfine interaction. Realizing nuclear spin control would likely improve electron…

Mesoscale and Nanoscale Physics · Physics 2010-06-15 D. J. Reilly , J. M. Taylor , J. R. Petta , C. M. Marcus , M. P. Hanson , A. C. Gossard

For coherent electron spins, hyperfine coupling to nuclei in the host material can either be a dominant source of unwanted spin decoherence or, if controlled effectively, a resource allowing storage and retrieval of quantum information. To…

Mesoscale and Nanoscale Physics · Physics 2013-05-28 H. O. H. Churchill , A. J. Bestwick , J. W. Harlow , F. Kuemmeth , D. Marcos , C. H. Stwertka , S. K. Watson , C. M. Marcus

Dephasing and relaxation of the nuclear spins coupled to the nitrogen-vacancy (NV) center during optical initialization and readout is an important issue for various applications of this hybrid quantum register. Here we present both an…

Quantum Physics · Physics 2016-07-15 Ping Wang , Wen Yang

Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 E. Evers , T. Kazimierczuk , F. Mertens , D. R. Yakovlev , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer , A. Greilich

We study a system in which electrons in a two-dimensional electron gas are confined by a nonhomogeneous nuclear spin polarization. The system consists of a heterostructure that has non-zero nuclei spins. We show that in this system…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yu. V. Pershin

Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…

Materials Science · Physics 2026-01-13 A. N. Anisimov , A. V. Poshakinskiy , G. V. Astakhov

The nuclear spin in the vicinity of a nitrogen-vacancy (NV) center possesses of long coherence time and convenient manipulation assisted by the strong hyperfine interaction with the NV center. It is suggested for the subsequent quantum…

Quantum Physics · Physics 2018-04-18 Yang-Yang Wang , Jing Qiu , Ying-Qi Chu , Mei Zhang , Jianming Cai , Qing Ai , Fu-Guo Deng

The concept of nuclear spin temperature has been a cornerstone of the theory of dynamic nuclear spin polarization by electrons in various semiconductor structures for decades. Still, it is not always applicable to strongly localized…

Mesoscale and Nanoscale Physics · Physics 2024-08-13 D. S. Smirnov , K. V. Kavokin

We study a mechanism by which nuclear hyperpolarization due to the polarization transfer from a microwave-pulse-controlled electron spin is suppressed. From analytical and numerical calculations of the unitary dynamics of multiple nuclear…

Quantum Physics · Physics 2024-03-12 Kento Sasaki , Eisuke Abe

Spin inertia measurements are a novel experimental tool to study long-time spin relaxation processes in semiconductor nanostructures. We develop a theory of the spin inertia effect for resident electrons and holes localized in quantum dots.…

Mesoscale and Nanoscale Physics · Physics 2019-12-23 Philipp Schering , Götz S. Uhrig , Dmitry S. Smirnov

Thermalization phenomena, while ubiquitous in quantum systems, have traditionally been viewed as obstacles to be mitigated. In this study, we demonstrate the ability, instead, to harness thermalization to dynamically engineer and stabilize…

Extensive work on single molecule magnets has identified a fundamental mode of relaxation arising from the nuclear-spin assisted quantum tunnelling of nearly independent and quasi-classical magnetic dipoles. Here we show that nuclear-spin…

Strongly Correlated Electrons · Physics 2019-03-28 C. Paulsen , S. R. Giblin , E. Lhotel , D. Prabhakaran , K. Matsuhira , G. Balakrishnan , S. T. Bramwell

Physical systems reach thermal equilibrium through energy exchange with their environment, and for spins in solids the relevant environment is almost always the host lattice in which they sit. However, recent studies motivated by…

Polarizing nuclear spins is of fundamental importance in biology, chemistry and physics. Methods for hyperpolarizing 13C nuclei from free electrons in bulk, usually demand operation at cryogenic temperatures. Room-temperature approaches…

We theoretically study the longitudinal relaxation of a nitrogen-vacancy (NV) center surrounded by a 13C nuclear spin bath in diamond. By incorporating electron spin in the cluster, we generalize the cluster-correlation expansion (CCE) to…

Quantum Physics · Physics 2020-01-22 Zhi-Sheng Yang , Yan-Xiang Wang , Ming-Jie Tao , Wen Yang , Mei Zhang , Qing Ai , Fu-Guo Deng

The long standing problem of inexplicably short spin relaxation in carbon nanotubes (CNTs) is examined. The curvature-mediated spin-orbital interaction is shown to induce fluctuating electron spin precession causing efficient relaxation in…

Materials Science · Physics 2015-05-18 Y. G. Semenov , J. M. Zavada , K. W. Kim