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Electron Spin Resonance (ESR) describes a suite of techniques for characterising electronic systems, with applications in physics, materials science, chemistry, and biology. However, the requirement for large electron spin ensembles in…

Quantum Physics · Physics 2015-03-04 L. T. Hall , P. Kehayias , D. A. Simpson , A. Jarmola , A. Stacey , D. Budker , L. C. L. Hollenberg

Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

Understanding fully the dynamics of coupled electron-nuclear spin systems, which are important for the development of long-lived qubits based on solid-state systems, remains a challenge. We show that in a singly charged semiconductor…

Mesoscale and Nanoscale Physics · Physics 2010-07-26 Wenxian Zhang , Jian-Liang Hu , Jun Zhuang , J. Q. You , Ren-Bao Liu

We analytically solve the {\it Non-Markovian} single electron spin dynamics due to hyperfine interaction with surrounding nuclei in a quantum dot. We use the equation-of-motion method assisted with a large field expansion, and find that…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Changxue Deng , Xuedong Hu

The interplay of optical driving and hyperfine interaction between an electron confined in a quantum dot and its surrounding nuclear spin environment produces a range of interesting physics such as mode-locking. In this work, we go beyond…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Arian Vezvaee , Gargee Sharma , Sophia E. Economou , Edwin Barnes

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

The main source of decoherence for an electron spin confined to a quantum dot is the hyperfine interaction with nuclear spins. To analyze this process theoretically we diagonalize the central spin Hamiltonian in the high magnetic B-field…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Oleksandr Tsyplyatyev , Daniel Loss

We report electronic control and measurement of an imbalance between spin-up and spin-down electrons in micron-scale open quantum dots. Spin injection and detection was achieved with quantum point contacts tuned to have spin-selective…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 E. J. Koop , B. J. van Wees , D. Reuter , A. D. Wieck , C. H. van der Wal

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

The periodic optical orientation of electron spins in (In,Ga)As/GaAs quantum dots leads to the formation of electron spin precession modes about an external magnetic field which are resonant with the pumping periodicity. As the electron…

Mesoscale and Nanoscale Physics · Physics 2019-08-15 E. Evers , V. V. Belykh , N. E. Kopteva , I. A. Yugova , A. Greilich , D. R. Yakovlev , D. Reuter , A. D. Wieck , M. Bayer

In this work, we devise a fast and effective nuclear spin hyperpolarization scheme, which is in principle magnetic field and temperature independent. We use this scheme to experimentally demonstrate polarizations of up to 66% for phosphorus…

Techniques for coherent control of electron spin-nuclear spin interactions in quantum dots can be directly applied in spintronics and in quantum information processing. In this work we study numerically the interaction of electron and…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 V. V. Dobrovitski , J. M. Taylor , M. D. Lukin

Superradiance of nuclear spins is considered, when the nuclei interact via hyperfine forces with electrons of a ferromagnet. The consideration is based on a microscopic model. If the sample, coupled with a resonant electric circuit,…

Condensed Matter · Physics 2007-05-23 V. I. Yukalov , E. P. Yukalova

We discuss the implications of a small indium content (3%) in a GaAs epilayer on the electron- and nuclear-spin relaxation due to enhanced quadrupolar effects induced by the strain. Using the weakly perturbative spin-noise spectroscopy, we…

Mesoscale and Nanoscale Physics · Physics 2022-07-27 C. Rittmann , M. Yu. Petrov , A. N. Kamenskii , K. V. Kavokin , A. Yu. Kuntsevich , Yu. P. Efimov , S. A. Eliseev , M. Bayer , A. Greilich

We present a methodology for probing the details of electronic susceptibility through minimally-invasive nuclear magnetic resonance techniques. Specifically, we classify electron-mediated long-range interactions in an ensemble of nuclear…

Strongly Correlated Electrons · Physics 2022-08-17 Stephen Carr , Charles Snider , D. E. Feldman , Chandrasekhar Ramanathan , J. B. Marston , V. F. Mitrović

The nitrogen-vacancy (NV) centre, as a promising candidate solid state system of quantum information processing, its electron spin coherence is influenced by the magnetic field fluctuations due to the local environment. In pure diamonds,…

Mesoscale and Nanoscale Physics · Physics 2011-04-08 Nan Zhao , Jian-Liang Hu , Sai-Wah Ho , Tsz-Kai Wen , R. B. Liu

Nuclear hyperpolarization is a known method to enhance the signal in nuclear magnetic resonance (NMR) by orders of magnitude. The present work addresses the $^{13}$C hyperpolarization in diamond micro- and nanoparticles, using the…

The sensitivity of Magnetic Resonance Imaging (MRI) depends strongly on nuclear spin polarisation and, motivated by this observation, dynamical nuclear spin polarisation has recently been applied to enhance MRI protocols (Kurhanewicz, J.,…

We present an experimental study of the dynamics underlying the buildup and decay of dynamical nuclear spin polarization in a single semiconductor quantum dot. Our experiment shows that the nuclei can be polarized on a time scale of a few…

Optics · Physics 2007-08-02 P. Maletinsky , A. Badolato , A. Imamoglu

Perovskite nanocrystals are a convenient model system for optical spin orientation and manipulation. However, its real potential might be underestimated due to the incomplete knowledge on spin relaxation times, which are obscured by the…