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A model for charge transport in undoped, photo-excited semiconductor superlattices, which includes the dependence of the electron-hole recombination on the electric field and on the photo-excitation intensity through the field-dependent…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 J. I. Arana , L. L. Bonilla , H. T. Grahn

We present combined experimental and theoretical study of photo-induced current in molecular junctions consisting of monolayers of nitroazobenzene oligomers chemisorbed on carbon surfaces and illuminated by UV-Vis light through a…

Mesoscale and Nanoscale Physics · Physics 2019-03-22 Kuniyuki Miwa , Amin Morteza Najarian , Richard L. McCreery , Michael Galperin

Studies of excitonic transport in transition metal dichalcogenide monolayers have attracted increasing interest in recent years in order to develop nano-optoelectronic devices made with 2D materials. These studies began with low to moderate…

We investigate the optoelectronic properties of single indium arsenide nanowires, which are grown vertically on p-doped silicon substrates. We apply a scanning photocurrent microscopy to study the optoelectronic properties of the single…

Understanding the ultrafast coupling and relaxation mechanisms between valleys in transition metal dichalcogenide semiconductors is of crucial interest for future valleytronic devices. Recent ultrafast pump-probe experiments showed an…

We reveal stacking-induced strong coupling between atomic motion and interlayer excitons through photocurrent measurements of WSe$_2$/MoSe$_2$ heterojunction photodiodes. Strong coupling manifests as pronounced periodic sidebands in the…

We address the role of excitonic coulping on the nature of photoexcitations in the conjugated polymer regioregular poly(3-hexylthiophene). By means of temperature-dependent absorption and photoluminescence spectroscopy, we show that optical…

Materials Science · Physics 2007-05-23 Jenny Clark , Carlos Silva , Richard H. Friend , Frank C. Spano

In the realm of two-dimensional materials magnetic and transport properties of a unique representative $-$ Fe$_3$GeTe$_2$ $-$ attract ever increasing attention. Here, we use a developed first-principles method for calculating laser-induced…

Mesoscale and Nanoscale Physics · Physics 2021-12-22 M. Merte , F. Freimuth , T. Adamantopoulos , D. Go , T. G. Saunderson , M. Kläui , L. Plucinski , O. Gomonay , S. Blügel , Y. Mokrousov

The requirements for broadband photodetection are becoming exceedingly demanding in hyperspectral imaging. Whilst intrinsic photoconductor arrays based on mercury cadmium telluride represent the most sensitive and suitable technology, their…

Nonlinear optical properties, such as bulk photovoltaic effects, possess great potential in energy harvesting, photodetection, rectification, etc. To enable efficient light-current conversion, materials with strong photo-responsivity are…

Materials Science · Physics 2021-03-02 Haowei Xu , Hua Wang , Jian Zhou , Yunfan Guo , Jing Kong , Ju Li

Graphene/silicon (G/Si) heterojunction based devices have been demonstrated as high responsivity photodetectors that are potentially compatible with semiconductor technology. Such G/Si Schottky junction diodes are typically in parallel with…

The quantum-dynamical mechanism of photoinduced subpicosecond exciton dissociation and the concomitant formation of a charge-separated state at a TFB:F8BT polymer heterojunction is elucidated. The analysis is based upon a two-state vibronic…

Materials Science · Physics 2009-11-11 Hiroyuki Tamura , Eric R. Bittner , Irene Burghardt

To add to the rapidly progressing field of ultrafast photocurrent, we propose a universal method to generate photocurrent in normal and topological materials using a pair of multicycle linearly polarized laser pulses. The interplay of the…

Mesoscale and Nanoscale Physics · Physics 2024-03-20 Amar Bharti , Gopal Dixit

Theory of optical absorption of linearly and circularly polarized light in surface and edge states in topological insulators is developed for a nonlinear in light intensity regime. The absorbance for surface states and the absorption width…

Mesoscale and Nanoscale Physics · Physics 2022-03-30 N. V. Leppenen , L. E. Golub

Monolayer transition metal dichalcogenide (TMD) semiconductors such as MoSe$_2$ host strongly bound excitons which are known to exhibit a strong resonant third-order nonlinear response. Although there have been numerous studies of the…

Ultrafast charge separation after photoexcitation is a common phenomenon in various van-der-Waals (vdW) heterostructures with great relevance for future applications in light harvesting and detection. Theoretical understanding of this…

Mixed-dimensional van der Waals heterojunctions comprising polymer and twodimensional (2D) semiconductors have many characteristics of an ideal charge separation interface for optoelectronic and photonic applications. However, the…

Materials Science · Physics 2018-05-25 Chengmei Zhong , Vinod K. Sangwan , Chen Wang , Hadallia Bergeron , Mark C. Hersam , Emily A. Weiss

Monolayer transition metal dichalcogenide semiconductors host strongly bound two-dimensional excitonic complexes, and form an excellent platform for probing many-body physics through manipulation of Coulomb interaction. Quantum confined…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Nithin Abraham , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

A new phototransistor based on the mechanically-exfoliated single-layer MoS2 nanosheet is fabricated and its light-induced electric properties are investigated in details. Photocurrent generated from the phototransistor is solely determined…

Materials Science · Physics 2013-10-31 Zongyou Yin , Hai Li , Hong Li , Lin Jiang , Yumeng Shi , Yinghui Sun , Gang Lu , Qing Zhang , Xiaodong Chen , Hua Zhang

Excitons play a key role in the linear optical response of 2D materials. However, their significance in the highly nonlinear optical response to intense mid-infrared light has often been overlooked. Using hBN as a prototypical example, we…

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