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Integration of 2D semiconductors with photonic crystal slabs provides an attractive approach to achieve strong light--matter coupling and exciton-polariton formation in a planar chip-compatible geometry. However, for the development of…

When light is absorbed by a semiconductor, photoexcited charge carriers enhance the absorption of far-infrared radiation due to intraband transitions. We observe the opposite behavior in monolayer graphene, a zero-gap semiconductor with…

Mesoscale and Nanoscale Physics · Physics 2013-04-02 A. J. Frenzel , C. H. Lui , W. Fang , N. L. Nair , P. K. Herring , P. Jarillo-Herrero , J. Kong , N. Gedik

Trions are excitonic species with a positive or negative charge, and thus, unlike neutral excitons, the flow of trions can generate a net detectable charge current. Trions under favourable doping conditions can be created in a coherent…

Applied Physics · Physics 2020-03-24 Sarthak Das , Sangeeth Kallatt , Nithin Abraham , Kausik Majumdar

Organic semiconducting polymers are currently of broad interest as potential low-cost materials for photovoltaic and light-emitting display applications. I will give an overview of our work in developing a consistent quantum dynamical…

Materials Science · Physics 2007-05-23 Eric R. Bittner , John Glen S. Ramon

Semiconducting 2D materials, such as molybdenum disulfide (MoS2) and other members of the transition metal dichalcogenide family, have emerged as promising materials for applications in high performance nanoelectronics that exhibit…

Applied Physics · Physics 2019-05-24 David Maeso , Andres Castellanos-Gomez , Nicolas Agraït , Gabino Rubio-Bollinger

Light emission in atomically thin heterostructures is known to depend on the type of materials, number and stacking sequence of the constituent layers. Here we show that the thickness of a two-dimensional substrate can be crucial in…

We present first-principles calculations of many-electron effects on the optical response of graphene, bilayer graphene, and graphite employing the GW-Bethe Salpeter equation approach. We find that resonant excitons are formed in these…

Materials Science · Physics 2009-10-31 Li Yang , Jack Deslippe , Cheol-Hwan Park , Marvin L. Cohen , Steven G. Louie

We study spatial photoluminescence characteristics of neutral and charged excitons across extended monolayer MoS$_2$ synthesized by chemical vapor deposition. Using two-dimensional hyperspectral photoluminescence mapping at cryogenic…

Mesoscale and Nanoscale Physics · Physics 2019-02-20 Andre Neumann , Jessica Lindlau , Manuel Nutz , Aditya D. Mohite , Hisato Yamaguchi , Alexander Högele

A self-consistent scheme for the calculations of the interacting groundstate and the near bandgap optical spectra of mono- and multilayer transition-metal-dichalcogenide systems is presented. The approach combines a dielectric model for the…

Mesoscale and Nanoscale Physics · Physics 2018-01-24 Lars Meckbach , Tineke Stroucken , Stephan W. Koch

We theoretically study nonlinear optics of excitons under intense THz irradiation. In particular, the linear near infrared absorption and resonantly enhanced nonlinear sideband generation are described. We predict a rich structure in the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Kristinn Johnsen , Antti-Pekka Jauho

Strong optical nonlinearities play a central role in realizing quantum photonic technologies. In solid state systems, exciton-polaritons, which result from the hybridization of material excitations and cavity photons, are an attractive…

The recent advent of two-dimensional monolayer materials with tunable optoelectronic properties and high carrier mobility offers renewed opportunities for efficient, ultra-thin excitonic solar cells alternative to those based on conjugated…

Mesoscale and Nanoscale Physics · Physics 2012-06-26 Marco Bernardi , Maurizia Palummo , Jeffrey C. Grossman

We propose an equivalent circuit representation of the photogenerated charge separation and propagation in dye sensitized polycrystalline semiconductor in contact with a redox electrolyte. The suggested equivalent circuit for this type of…

Materials Science · Physics 2007-05-23 B. Vainas

Recent experiments on microwave-irradiated high-mobility two-dimensional electron systems revealed a novel photoresistivity peak in the vicinity of the second cyclotron resonance harmonic. Here we report on the nonlinear transport…

Mesoscale and Nanoscale Physics · Physics 2011-05-10 A. T. Hatke , M. A. Zudov , L. N. Pfeiffer , K. W. West

The new generation of two-dimensional (2D) materials has shown a broad range of applications for optical and electronic devices. Understanding the properties of these materials when integrated with the more traditional three-dimensional…

Controlling the flow of charge neutral interlayer exciton (IX) quasiparticles can potentially lead to low loss excitonic circuits. Here, we report unidirectional transport of IXs along nanoscale electrostatically defined channels in an…

Nonlinear interactions between excitons strongly coupled to light are key for accessing quantum many-body phenomena in polariton systems. Atomically-thin two-dimensional semiconductors provide an attractive platform for strong light-matter…

Quantum interference between one- and two-photon absorption pathways allows coherent control of interband transitions in unbiased bulk semiconductors; carrier population, carrier spin polarization, photocurrent injection, and spin current…

Other Condensed Matter · Physics 2007-05-23 R. D. R. Bhat , J. E. Sipe

Optical excitation serves as a powerful approach to control the electronic structure of layered Van der Waals materials via many-body screening effects, induced by photoexcited free carriers, or via light-driven coherence, such as optical…

Time-dependent current of the electrons excited in the conduction band after ultrafast interband photogeneration is studied theoretically. The transient photocurrent is calculated for the nonlinear regime of response to a stationary…

Materials Science · Physics 2009-11-11 O. E. Raichev , F. T. Vasko