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The current family of experimentally realized two-dimensional magnetic materials consist of 3$d$ transition metals with very weak spin-orbit coupling. In contrast, we report a new platform in a chemically bonded and layered 4$d$ oxide, with…

Diverse interlayer tunability of physical properties of two-dimensional layers mostly lies in the covalent-like quasi-bonding that is significant in electronic structures but rather weak for energetics. Such characteristics result in…

Materials Science · Physics 2019-04-03 Peiheng Jiang , Cong Wang , Dachuan Chen , Zhicheng Zhong , Zhe Yuan , Zhong-Yi Lu , Wei Ji

In all van der Waals layered antiferromagnetic semiconductors investigated so far a negative magnetoresistance has been observed in vertical transport measurements, with characteristic trends that do not depend on applied bias. Here we…

Mesoscale and Nanoscale Physics · Physics 2024-10-24 Xiaohanwen Lin , Fan WU , Nicolas Ubrig , Menghan Liao , Fengrui Yao , Ignacio Gutiérrez-Lezama , Alberto F. Morpurgo

Altermagnets constitute a novel, third fundamental class of collinear magnetic ordered materials, alongside with ferro- and antiferromagnets. They share with conventional antiferromagnets the feature of a vanishing net magnetization. At the…

Surface reconstruction plays a vital role in determining the surface electronic structure and chemistry of semiconductors and metal oxides. However, it has been commonly believed that surface reconstruction does not occur in van der Waals…

Materials Science · Physics 2023-09-19 Sung-Hoon Lee , Doohee Cho

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

Materials Science · Physics 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

Among two-dimensional magnetic materials, CrSBr has attracted considerable attention owing to its coexistence of ferromagnetic and antiferromagnetic ordering, which depends sensitively on crystallographic orientation. An additional…

Materials Science · Physics 2026-05-26 Naresh Shyaga , Pankaj Bhardwaj , Rajib Sarkar , Jagadish Rajendran , Abhiram Soori , Dhavala Suri

Motivated by the recent experimental developments in van der Waals heterostructures, we investigate the emergent magnetism in Mott insulator - semimetal moir\'e superlattices by deriving effective spin models and exploring their phase…

Strongly Correlated Electrons · Physics 2024-11-05 M. A. Keskiner , Pouyan Ghaemi , M. Ö. Oktel , Onur Erten

The recent discovery of ferromagnetism in 2D van der Waals (vdw) crystals has generated widespread interest, owing to their potential for fundamental and applied research. Advancing the understanding and applications of vdw magnets requires…

The behavior of 2-dimensional (2D) van der Waals (vdW) layered magnetic materials in the 2D limit of the few-layer thickness is an important fundamental issue for the understanding of the magnetic ordering in lower dimensions. The…

Materials Science · Physics 2020-12-02 Soo Yeon Lim , Kangwon Kim , Sungmin Lee , Je-Geun Park , Hyeonsik Cheong

Van der Waals (vdW) layered materials have rather weaker interlayer bonding than the intra-layer bonding, therefore the exfoliation along the stacking direction enables the achievement of monolayer or few layers vdW materials with emerging…

The effect of strain on the magnetic order and band structure of single-layer CrAsS$_4$ has been investigated by first-principles calculations based on density functional theory. We found that single-layer CrAsS$_4$ was an antiferromagnetic…

Materials Science · Physics 2021-10-01 Tengfei Hu , Wenhui Wan , Yanfeng Ge , Yong Liu

Antiferromagnets have garnered significant attention due to their negligible stray field and ultrafast magnetic dynamics, which are promising for high-density and ultrafast spintronic applications. Their dual functionality as both spin…

In this article we review recent work on van der Waals (vdW) systems in which at least one of the components has strong spin-orbit coupling. We focus on a selection of vdW heterostructures to exemplify the type of interesting electronic…

Mesoscale and Nanoscale Physics · Physics 2020-06-04 Enrico Rossi , Christopher Triola

Van der Waals heterostructures (vdWHs) composed of transition-metal dichalcogenides (TMDs) and layered magnetic semiconductors offer great opportunities to manipulate exciton and valley properties of TMDs. Here, we present…

We study the electronic properties of the heterobilayer of vanadium and iron oxychlorides, VOCl and FeOCl, two layered air stable van der Waals insulating oxides with different types of antiferromagnetic order in bulk: VOCl monolayers are…

Mesoscale and Nanoscale Physics · Physics 2021-04-19 F. Mahrouche , K. Rezouali , Z. C. Wang , J. Fernández-Rossier , A. Molina-Sánchez

Altermagnets (AMs) are a recently identified class of unconventional collinear compensated antiferromagnets that exhibit momentum-dependent spin splitting despite having zero net magnetization. This unconventional magnetic order gives rise…

Materials Science · Physics 2025-11-24 Bo Zhao , Fu Li , Wei Ren , Hao Wang , Hongbin Zhang

Although the magnetic order is suppressed by a strong magnetic frustration, it is maintained but appears in complex order forms such as a cycloid or spin density wave in weakly frustrated systems. Herein, we report a weakly…

Combining first-principles calculations and tight-binding Hamiltonians, we study the stack-dependent behaviour of electronic and topological properties of layered antiferromagnet MnBi$_2$Te$_4$. Lateral shift of top septuple-layer greatly…

Materials Science · Physics 2025-03-05 Jiaheng Li , Quansheng Wu , Hongming Weng

Two-dimensional (2D) Van der Waals compounds exhibit interesting electronic and magnetic properties due to complex intra-layer and inter-layer interactions, which are of immense importance in realizing exotic physics as well as advanced…

Strongly Correlated Electrons · Physics 2025-01-22 Smita Gohil , Saswata Halder , Karthik K Iyer , Shankar Ghosh , A. Thamizhavel , Kalobaran Maiti
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