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We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

The crystallographic, magnetic, and transport properties of the van der Waals bonded, layered compound CrTe3 have been investigated on single crystal and polycrystalline materials. The crystal structure contains layers made up of lozenge…

Strongly Correlated Electrons · Physics 2017-04-19 Michael A. McGuire , V. Ovidiu Garlea , Santosh KC , Valentino R. Cooper , Jiaqiang Yan , Huibo Cao , Brian C. Sales

Interlayer magnetic interactions play a pivotal role in determining the magnetic arrangement within van der Waals (vdW) magnets, and the remarkable tunability of these interactions through applied pressure further enhances their…

Materials Science · Physics 2024-04-16 Qiye Liu , Wenjie Su , Yue Gu , Xi Zhang , Xiuquan Xia , Le Wang , Ke Xiao , Xiaodong Cui , Xiaolong Zou , Bin Xi , Jia-Wei Mei , Jun-Feng Dai

In the rich phases of van der Waals (vdW) materials featuring intertwined electronic order and collective phenomena, characterizing elementary dynamics that entail the low-energy Hamiltonian and electronic degrees of freedom is of paramount…

Layered van der Waals antiferromagnet CrSBr supports strong light--matter coupling and formation of magnetically tunable exciton-polaritons, yet active magnetic control over polariton propagation direction has remained elusive. Here, we…

How a certain ground state of complex physical systems emerges, especially in two-dimensional materials, is a fundamental question in condensed-matter physics. A particularly interesting case is systems belonging to the class of XY…

Mesoscale and Nanoscale Physics · Physics 2019-01-31 Kangwon Kim , Soo Yeon Lim , Jae-Ung Lee , Sungmin Lee , Tae Yun Kim , Kisoo Park , Gun Sang Jeon , Cheol-Hwan Park , Je-Geun Park , Hyeonsik Cheong

Chromium triiodide, CrI$_3$, is emerging as a promising magnetic two-dimensional semiconductor where spins are ferromagnetically aligned within a single layer. Potential applications in spintronics arise from an antiferromagnetic ordering…

In twisted two-dimensional (2D) magnets, the stacking dependence of the magnetic exchange interaction can lead to regions of ferromagnetic and antiferromagnetic interlayer order, separated by non-collinear, skyrmion-like spin textures.…

Nonlinear magnetoconductivity (NLMC) is a nonreciprocal transport response arising in non-centrosymmetric materials. However, this ordinary NLMC signal vanishes at zero magnetic field, limiting its potential for applications. Here, we…

CrSBr is an air-stable 2D van der Waals semiconducting magnet with great technological promise, but its atomic-scale magnetic interactions -- crucial information for high-frequency switching -- are poorly understood. We present an…

Materials Science · Physics 2022-07-18 A. Scheie , M. Ziebel , D. G. Chica , Y. J. Bae , Xiaoping Wang , A. I. Kolesnikov , Xiaoyang Zhu , X. Roy

The recently discovered van der Waals material CeSiI exhibits both heavy fermion behavior and spiral order with strong magnetic anisotropy which makes it a potential host for topological spin textures such as skyrmions through electrical…

Mesoscale and Nanoscale Physics · Physics 2024-10-10 Aayush Vijayvargia , Hao Zhang , Kipton Barros , Shi-Zeng Lin , Onur Erten

We report measurements of antiferromagnetic resonances in the van der Waals easy-axis antiferromagnet CrSBr. The interlayer exchange field and magnetocrystalline anisotropy fields are comparable to laboratory magnetic fields, allowing a…

We report a La2CuO4-like interlayer antiferromagnetic order in Sr2IrO4 films with large orthorhombic distortion (> 1.5%). The biaxial lattice strain in epitaxial heterostructures of Sr2IrO4/Ca3Ru2O7 lowers the crystal symmetry of Sr2IrO4…

Strongly Correlated Electrons · Physics 2022-03-23 S. Shrestha , M. Krautloher , M. Zhu , J. Kim , J. Hwang , J. Kim , J. -W. Kim , B. Keimer , A. Seo

The $R\mathrm{Te}_3$ ($R = \text{rare earth}$) family of layered van der Waals (vdW) compounds hosts coexisting magnetic and charge density wave (CDW) orders, yet the interplay between these degrees of freedom remains little explored.…

The growing interest in 2D van der Waals (vdW) magnetic materials stems from their unique properties and potential applications in spintronics, magnonics and quantum information technologies. Among them, CrSBr is a semiconductor that stands…

Materials Science · Physics 2024-12-24 Sourav Dey , Dorye L. Esteras , José J. Baldoví

We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

Van der Waals (vdW) Dirac magnon system CrI$_3$, a potential host of topological edge magnons, orders ferromagnetically (FM) (T$_C=61$ K) in the bulk, but antiferromagnetic (AFM) order has been observed in nanometer thick flakes, attributed…

Materials Science · Physics 2024-05-14 John A. Schneeloch , Luke Daemen , Despina Louca

Interlayer coupling is of vital importance for manipulating physical properties, e.g. electronic bandgap, in two-dimensional materials. However, tuning magnetic proper-ties in these materials is yet to be addressed. Here, we found a striped…

Materials Science · Physics 2018-06-20 Cong Wang , Xieyu Zhou , Yuhao Pan , Jingsi Qiao , Xianghua Kong , Chao-Cheng Kaun , Wei Ji

We use a data-driven approach to study the magnetic and thermodynamic properties of van der Waals (vdW) layered materials. We investigate monolayers of the form A$_2$B$_2$X$_6$, based on the known material Cr$_2$Ge$_2$Te$_6$, using density…

Materials Science · Physics 2018-06-22 Trevor David Rhone , Wei Chen , Shaan Desai , Amir Yacoby , Efthimios Kaxiras

Layered van-der-Waals 2D magnetic materials are of great interest in fundamental condensed-matter physics research, as well as for potential applications in spintronics and device physics. We present neutron powder diffraction data using…