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The physical properties of two-dimensional van der Waals (2D vdW) crystals depend sensitively on the interlayer coupling, which is intimately connected to the stacking arrangement and the interlayer spacing. For example, simply changing the…

Recently discovered ferromagnetism of the layered van der Waals material VI$_3$ attracts much research attention. Despite substantial progress,in the following important aspects no consensus has been reached: (i) a possible deviation of the…

Materials Science · Physics 2021-07-07 L. M. Sandratskii , K. Carva

Interfaces between twisted 2D materials host a wealth of physical phenomena originating from the long-scale periodicity associated with the resulting moire structure. Besides twisting, an alternative route to create structures with…

Electric-field switching of magnetic order is of significant physical interest and holds great potential for spintronic applications. However, it has rarely been reported in two-dimensional (2D) van der Waals (vdW) magnets due to the…

Materials Science · Physics 2025-02-06 Chengxi Huang , Jinzhe Han , Jing Wang , Jintao Jiang , Ziyang Qu , Fang Wu , Ang Li , Yi Wan , Kaiyou Wang , Erjun Kan

We show that anisotropic energy of a 2D antiferromagnet is greatly enhanced via stacking on a magnetic substrate layer, arising from the sublattice-dependent interlayer magnetic interaction that defines an effective anisotropic energy.…

Mesoscale and Nanoscale Physics · Physics 2022-08-16 Feiping Xiao , Qingjun Tong

Magnetic van der Waals heterostructures provide a unique platform to study magnetism and spintronics device concepts in the two-dimensional limit. Here, we report studies of exchange bias from the van der Waals antiferromagnet CrSBr acting…

Van der Waals (vdW) ferromagnetic materials are rapidly establishing themselves as effective building blocks for next generation spintronic devices. When layered with non-magnetic vdW materials, such as graphene and/or topological…

We investigate the ultrafast magnetization dynamics of semiconducting antiferromagnetic CrSBr using real-time time-dependent density functional theory. In zero magnetic field, laser excitation modifies only the magnetization along the easy…

Materials Science · Physics 2026-03-16 Ali Kefayati , Yafei Ren

Unusual magnetic properties of Van der Waals type antiferromagnetic semiconductors make them highly attractive for spintronics and optoelectronics. A link between the magnetic and optical properties of those materials, required for…

The optical properties of the layered magnet CrSBr are dominated by intralayer excitons: the antiferromagnetic order between the layers makes layer-to-layer charge hopping, and therefore interlayer excitons, spin-forbidden. An external…

In conventional ferroelectric materials, polarization is an intrinsic property limited by bulk crystallographic structure and symmetry. Recently, it has been demonstrated that polar order can also be accessed using inherently non-polar van…

Van der Waals (vdW) heterostructures have attracted great interest because of their rich material combinations.The discovery of two-dimensional magnets has provided a new platform for magnetic vdW heterointerfaces; however, research on…

The recent isolation of two-dimensional (2D) magnets offers tantalizing opportunities for spintronics and magnonics at the limit of miniaturization. One of the key advantages of atomically-thin materials is their outstanding deformation…

Materials Science · Physics 2022-11-23 Dorye L. Esteras , Andrey Rybakov , Alberto M. Ruiz , José J. Baldoví

Following the discovery of graphene, interest in van der Waals (vdW) materials has surged; however, advancing physics beyond graphene requires quantum vdW materials platforms that host versatile, strongly interacting many-body states. Here,…

We show how van der Waals (vdW) forces outcompete covalent and ionic forces to control ferroelectric ordering in CuInP2S6 nanoflakes as well as in CuInP2S6 and CuBiP2Se6 crystals. While the self-assembly of these 2D layered materials is…

Materials Science · Physics 2018-05-31 Jeffrey R. Reimers , Sherif Abdulkader Tawfik , Michael J. Ford

Strategies such as chemical substitution, strain engineering and van der Waals stacking offer powerful means to control magnetism in 2D materials, enabling the emergence of novel quantum phenomena. Here, we investigate the magnetic…

Materials Science · Physics 2024-12-30 Alberto M. Ruiz , José J. Baldoví

Recent advancements in 2D materials have revealed the potential of van der Waals magnets, and specifically of their magnetic anisotropy that allows applications down to the 2D limit. Among these materials, CrSBr has emerged as a promising…

Magnetic semiconductors are a powerful platform for understanding, utilizing and tuning the interplay between magnetic order and electronic transport. Compared to bulk crystals, two-dimensional magnetic semiconductors have greater…

We predict that antiferromagnetic bilayers formed from van der Waals (vdW) materials, like bilayer CrI$_3$, have a strong magnetoelectric response that can be detected by measuring the gate voltage dependence of Faraday or Kerr rotation…

Mesoscale and Nanoscale Physics · Physics 2021-03-15 Chao Lei , Bheema Lingam Chittari , Kentaro Nomura , Nepal Banerjee , Jeil Jung , Allan H. MacDonald

The recent discovery of magnetism in atomically thin layers of van der Waals (vdW) crystals has created new opportunities for exploring magnetic phenomena in the two-dimensional (2D) limit. In most 2D magnets studied to date the c-axis is…