Related papers: Solid-state heteronuclear multiple-quantum spectro…
Magnetic resonance spectroscopy is universally regarded as one of the most important tools in chemical and bio-medical research. However, sensitivity limitations typically restrict imaging resolution to length scales greater than 10 \mu m.…
The properties of rare-earth elements diluted in non-magnetic crystals make them a promising candidate for a quantum memory due to their limited Hilbert space. The control and readout of the qubit states require a highly sensitive…
Rotational states of ultracold polar molecules possess long radiative lifetimes, microwave-domain coupling, and tunable dipolar interactions. The availability of numerous rotational states has inspired many proposed applications, including…
We analyze the gravitational wave signals with a model-independent time-frequency analysis, which is improved from the Hilbert-Huang transform (HHT) and optimized for characterizing the frequency variability on the time-frequency map.…
We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum…
Recently, Pang et al reported a novel polarization transfer scheme applicable to three-spin systems, whereby a rotating-frame NMR analogue of the cross effect could transfer polarization between; e.g., two 13Cs and an 15N in a single…
Diatomic polar molecules are one of the most promising platforms of quantum computing due to their rich internal states and large electric dipole moments. Here, we propose entangling rotational states of adjacent polar molecules via a…
We experimentally investigate a superconducting circuit composed of two flux qubits ultrastrongly coupled to a common LC resonator. Owing to the large anharmonicity of the flux qubits, the system can be described well by a generalized Dicke…
In quantum dots made from materials with nonzero nuclear spins, hyperfine coupling creates a fluctuating effective Zeeman field (Overhauser field) felt by electrons, which can be a dominant source of spin qubit decoherence. We characterize…
The redshifted cosmic 21 cm line signal of neutral hydrogen provides the possibility to constrain the matter power spectrum. Cross correlating temperature maps at different frequencies (corresponding to different redshifts along the line of…
We report the first study of the micro-SQUID response of a molecular system to electromagnetic radiation. The advantages of our micro-SQUID technique in respect to pulsed electron paramagnetic resonance (EPR) techniques consist in the…
We experimentally study a homodyne detection technique for the characterization of a quadrature squeezed field where the correlated bands, here created by four-wave mixing in a hot atomic vapor, are separated by a large frequency gap of…
Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…
Purpose: Inhomogeneous magnetization transfer (ihMT) effect reflects dipolar order with a dipolar relaxation time ($T_{1D}$), specific to motion-restricted macromolecules. We aim to quantify $T_{1D}$ using spin-lock MRI technique. Methods:…
We have realized a hybrid solid-state quantum device in which a single-electron semiconductor double quantum dot is dipole coupled to a superconducting microwave frequency transmission line resonator. The dipolar interaction between the two…
Two dimensional nuclear magnetic resonance (NMR) spectroscopy is one of the major tools for analysing the chemical structure of organic molecules and proteins. Despite its power, this technique requires long measurement times, which,…
Using a 1GW-1ps pump laser pulse in high gain parametric down-conversion allows us to detect sub-shot-noise spatial quantum correlation with up to one hundred photoelectrons per mode, by means of a high efficiency CCD. The statistics is…
We have observed multi-photon resonances in a system with a spin 3/2 irradiated simultaneously by a multiple pulse radiofrequency sequence and a low frequency field swept in the range 0-80 kHz. The used excitation scheme allowed us to…
We report the first study of time-resolved high-harmonic spectroscopy (TR-HHS) of a bond-making chemical reaction. We investigate the transient change of the high harmonic signal from 1,3-cyclohexadiene (CHD), which undergoes ring-opening…
The optical theorem relates the total scattering cross-section of a given structure with its forward scattering, but does not impose any restrictions on other directions. Strong backward-forward asymmetry in scattering could be achieved by…