Related papers: Solid-state heteronuclear multiple-quantum spectro…
Manipulation of spin states at the single-atom scale underlies spin-based quantum information processing and spintronic devices. Such applications require protection of the spin states against quantum decoherence due to interactions with…
Nonlinear manipulation of nuclear and electron spins is the basis for all advanced methods in magnetic resonance including multidimensional nuclear magnetic and electron spin resonance spectroscopies, magnetic resonance imaging, and in…
Solid-state electronic spin systems such as nitrogen-vacancy (NV) color centers in diamond are promising for applications of quantum information, sensing, and metrology. However, a key challenge for such solid-state systems is to realize a…
New evidence is presented in favor of irreversible decoherence as the mechanism which leads an initial out-of-equilibrium state to quasi-equilibrium in nematic liquid crystals. The NMR experiment combines the Jeener-Broekaert sequence with…
We explore how to encode more than a qubit in vanadyl porphyrin molecules hosting a electronic spin 1/2 coupled to a nuclear spin 7/2. The spin Hamiltonian and its parameters, as well as the spin dynamics, have been determined via a…
Coherent time is a characteristic time in the extreme nonlinear optics regime and thus generally introduced as the dephasing time in the simulations of the solid-state high-harmonic generation. This characteristic time linked with the…
The measurement of single quanta in a collection of coherently interacting objects is transformative in the investigations of emergent quantum phenomena. An isolated nuclear-spin ensemble is a remarkable platform owing to its coherence, but…
An all-optical measurement of high-order fractional molecular echoes is demonstrated by using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser pulses, the signatures of full and high order fractional (1/2…
Nuclear magnetic resonance (NMR) spectroscopy usually requires high magnetic fields to create spectral resolution among different proton species. At low fields, chemical shift dispersion is insufficient to separate the species, and the…
We report the first experimental observation of frequency shift in high order harmonic generation (HHG) from isotopic molecules H2 and D2 . It is found that harmonics generated from the isotopic molecules exhibit obvious spectral red shift…
We study the spectra of heavy-light and heavy-heavy mesons containing charm quarks, including higher spin states. We use two sets of $N_f = 2 + 1$ gauge configurations, one set from QCDSF using the SLiNC action, and the other configurations…
Highest resolution laser spectroscopy has generally been limited to single trapped ion systems due to rapid decoherence which plagues neutral atom ensembles. Here, precision spectroscopy of ultracold neutral atoms confined in a trapping…
Magnetic spin resonance is a key non-invasive sensing and imaging technique across the life-, material- and fundamental sciences with further medical and commercial applications. Recent advances using paramagnetic color centers enable…
A correlation between the symmetry of NMR spectra, including higher-order spectra, and the properties of the spin system has been established. It is shown that for a spectrum to be symmetric about the mid-resonance frequency ({\nu}0), two…
We demonstrate strong adiabatic laser alignment and mixed-field orientation at kHz repetition rates. We observe degrees of alignment as large as cos\Theta=0.94 at 1 kHz operation for iodobenzene. The experimental setup consist of a kHz…
We introduce and demonstrate a new approach to measuring coherent electron wave packets using high-harmonic spectroscopy. By preparing a molecule in a coherent superposition of electronic states, we show that electronic coherence opens…
We study in theory the generation and detection of electron spin coherence in nonlinear optical spectroscopy of semiconductor quantum dots doped with single electrons. In third-order differential transmission spectra, the inverse width of…
We study the ability to implement unitary maps on states of the $I=9/2$ nuclear spin in \textsuperscript{87}Sr, a $d=10$ dimensional (qudecimal) Hilbert space, using quantum optimal control. Through a combination of nuclear spin-resonance…
Harnessing dipolar spin environments as controllable quantum resources is a central challenge in solid-state quantum technologies. Here, we report the observation of a coherent mesoscopic spin state in a disordered ensemble of…
It is showed on the basis of the multiple-quantum operator algebra space formalism that ultra-broadband heteronuclear Hartmann-Hahn polarization transfer could be achieved by the amplitude- and frequency-modulation quasi-adiabatic…