The properties of rare-earth elements diluted in non-magnetic crystals make them a promising candidate for a quantum memory due to their limited Hilbert space. The control and readout of the qubit states require a highly sensitive measurement and large coupling of the spin ensemble with the electro-magnetic mode of a superconducting resonator. We report sensitive detection of forbidden transitions of electronuclear states from the minority species of 155Gd and 157Gd isotopes which opens the possibility of connecting quantum states with very different spin projections. Cavity perturbation measurements seen in the reflected signal allows the detection of about 7.6×107 spins and the measurement of spin decoherence rate and spin-photon coupling strength.
@article{arxiv.2203.11304,
title = {On-Chip Detection of Electronuclear Transitions in the $^{155,157}$Gd Multilevel Spin System},
author = {G. Franco-Rivera and J. Cochran and L. Chen and S. Bertaina and I. Chiorescu},
journal= {arXiv preprint arXiv:2203.11304},
year = {2022}
}