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We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…

We report an experiment to measure the femtosecond electric field of the signal emitted from an optical third-order nonlinear interaction in carbon dioxide molecules. Using degenerate four-wave mixing with femtosecond near infrared laser…

Quantum Physics · Physics 2022-10-05 Francis Walz , Siddhant Pandey , Liang Z. Tan , Niranjan Shivaram

We introduce and implement an interferometric technique based on chirped femtosecond laser pulses and nonlinear optics. The interference manifests as a high-visibility (> 85%) phase-insensitive dip in the intensity of an optical beam when…

Quantum Physics · Physics 2008-11-07 R. Kaltenbaek , J. Lavoie , D. N. Biggerstaff , K. J. Resch

Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field's oscillation period. However, synthesizing such a gate pulse is…

Spectro-temporal shaping of high-power femtosecond ultraviolet (UV) pulses remains a key challenge in ultrafast optics. Tailoring high-energy, ultrashort UV pulses underpins applications in ultrafast dynamics, high-precision spectroscopy,…

We describe an experiment to measure the emitted real-time electric field from an ultrafast third-order nonlinear optical interaction in molecules, using a phase-tracked spectral interferometry scheme. By combining a software lock-in…

Optics · Physics 2025-03-11 Siddhant Pandey , Francis Walz , Niranjan Shivaram

This article describes an interferometric method, called "Chirped Heterodyne Interferometry for Measuring Pulses" (CHIMP), for the complete characterization of highly (monotonically) chirped ultrabroadband optical pulses. CHIMP provides the…

Optics · Physics 2016-12-28 Adam S Wyatt , Pedro Oliveira , Ian O Musgrave

The recent introduction of coherent optical communications has created a compelling need for ultra-fast phase-sensitive measurement techniques operating at milliwatt peak power levels and in time scales ranging from sub-picoseconds to…

Laser frequency combs, which are composed of a series of equally-spaced coherent frequency components, have triggered revolutionary progress for precision spectroscopy and optical metrology. Length/distance is of fundamental importance in…

Optics · Physics 2024-02-27 Mingyang Xu , Hanzhong Wu , Jiawen Zhi , Yang Liu , Jie Zhang , Zehuang Lu , Chenggang Shao

Single-shot supercontinuum spectral interferometry (SSSI) is an optical technique that can measure ultrafast transients in the complex index of refraction. This method uses chirped supercontinuum reference/probe pulses that need to be…

Instrumentation and Detectors · Physics 2018-06-05 DinhDuy Tran Vu , Dogeun Jang , Ki-Yong Kim

Advances in the amplification and manipulation of ultrashort laser pulses has led to revolutions in several areas. Examples include chirped pulse amplification for generating high peak-power lasers, power-scalable amplification techniques,…

Optics · Physics 2016-08-24 C. R. Phillips , B. W. Mayer , L. Gallmann , U. Keller

We report a new version of spectral phase interferometry for direct electric field reconstruction (SPIDER), which enables consistency checking through the simultaneous acquisition of multiple shears and offers a simple and precise…

Optics · Physics 2019-03-27 Tobias Witting , Dane R. Austin , Ian A. Walmsley

Chirped-pulse interferometry (CPI) is a classical low-coherence interferometry technique with automatic dispersion cancellation and improved resolution over white-light interference. Previous work has shown that CPI with linearly-chirped…

Quantum Physics · Physics 2025-05-09 Madeleine Bérubé , Michael D. Mazurek , Kevin J. Resch

We describe an all-fiber nonlinear interferometer based on four-wave mixing in highly nonlinear fiber. Our configuration realizes phase-sensitive interference with 97% peak visibility and >90% visibility over a broad 554 GHz optical band.…

Instrumentation and Detectors · Physics 2018-08-28 Joseph M. Lukens , Raphael C. Pooser , Nicholas A. Peters

The success of non-linear optics relies largely on pulse-to-pulse consistency. In contrast, covariance based techniques used in photoionization electron spectroscopy and mass spectrometry have shown that wealth of information can be…

We show the existence of nonlinear resonant states in a higher-order nonlinear Schr\"odinger model that appertains to the wave propagation in femtosecond fiber optics, under certain parametric regime. These nonlinear resonant states are…

Pattern Formation and Solitons · Physics 2020-12-30 Shailza Pathania , Amit Goyal , Thokala Soloman Raju , C. N. Kumar

Measuring the phase of light is fundamental to optical imaging, sensing, and signal processing applications. Conventional optical phase measurements rely on multipath configurations, bulky interferometric setups, and computationally…

In this article, we report classical sensing with undetected light using octave spanning stimulated four-wave mixing from a plasmonic metasurface. The bidirectional nonlinear scattering due to inherent reflections from such thin nonlinear…

Chirped-pulse interferometry is a new interferometric technique encapsulating the advantages of the quantum Hong-Ou-Mandel interferometer without the drawbacks of using entangled photons. Both interferometers can exhibit even-order…

Quantum Physics · Physics 2009-09-07 Kevin J. Resch , Rainer Kaltenbaek , Jonathan Lavoie , Devon N. Biggerstaff

The combination of electronic sources operating at high frequencies and modern microwave instrumentation has enabled the recent development of chirped-pulse spectrometers for the millimetre and THz bands. This type of instrument can operate…

Instrumentation and Detectors · Physics 2018-10-12 Francis Hindle , Cédric Bray , Daniele Fontanari , Meriem Mouelhi , Arnaud Cuisset , Gael Mouret , Robin Bocquet
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