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The phasing problem of heterodyne-detected nonlinear spectroscopy states that the relative time delay between the exciting pulses and a local oscillator must be known with subcycle precision to separate absorptive and dispersive…

We report a novel experimental technique to investigate ultrafast dynamics in photoexcited molecules by probing the third-order nonlinear optical susceptibility. A non-colinear 3-pulse scheme is developed to probe the ultrafast dynamics of…

Cascaded nonlinearities have attracted much interest, but ultrafast applications have been seriously hampered by the simultaneous requirements of being near phase-matching and having ultrafast femtosecond response times. Here we show that…

Optics · Physics 2012-10-24 B. B. Zhou , A. Chong , F. W. Wise , M. Bache

Multi user orthogonal chirp spread spectrum (OCSS) can improve the spectral inefficiency of chirp spread spectrum (CSS) but is only feasible with perfect synchronism and without any channel dispersion. Asynchronism, channel dispersion, or…

Signal Processing · Electrical Eng. & Systems 2021-02-16 Nozhan Hosseini , David W. Matolak

In Impulsive Stimulated Raman Scattering vibrational oscillations, coherently stimulated by a femtosecond Raman pulse, are real time monitored and read out as intensity modulations in the transmission of a temporally delayed probe pulse.…

Chemical Physics · Physics 2019-11-28 Giovanni Batignani , Carino Ferrante , Giuseppe Fumero , Tullio Scopigno

Despite the multitude of available methods, the characterisation of ultrafast pulses remains a challenging endeavour, especially at the single-photon level. We introduce a pulse characterisation scheme that maps the magnitude of its…

We present a method for a complete characterization of a femtosecond ultraviolet pulse when a fundamental near-infrared beam is also available. Our approach relies on generation of second harmonic from the pre-characterized fundamental,…

Optics · Physics 2009-07-09 Marcin Kacprowicz , Wojciech Wasilewski , Konrad Banaszek

Specific features of nonlinear interference processes at quantum transitions in near- and fully-resonant optically-dense Doppler-broadened medium are studied. The feasibility of overcoming of the fundamental limitation on a…

Quantum Physics · Physics 2009-11-11 A. K. Popov , S. A. Myslivets , Thomas F. George

We report time resolved studies and measurement of all the components of the third-order nonlinear optical susceptibility of CS2 at 515 nm using degenerate four wave mixing. The use of a pulse of width 450 fs, which is comparable to the…

Optics · Physics 2022-03-08 Prajal Chettri , Shailesh Srivastava

By means of a metal opto-acoustic transducer we generate quasi-longitudinal and quasi-transverse picosecond strain pulses in a (311)-GaAs substrate and monitor their propagation by picosecond acoustic interferometry. By probing at the…

A finite element method simulation of a carbon fibre reinforced polymer block is used to analyse the nonlinearities arising from a contacting delamination gap inside the material. The ultrasonic signal is amplified and nonlinearities are…

Computational Engineering, Finance, and Science · Computer Science 2017-02-24 Martin Lints , Andrus Salupere , Serge Dos Santos

We present an optical method to measure radio-frequency electro-optic phase modulation profiles by employing spectrum-to-time mapping realized by highly chirped optical pulses. We directly characterize temporal phase modulation profiles of…

Instrumentation and Detectors · Physics 2017-11-23 Michał Jachura , Jan Szczepanek , Wojciech Wasilewski , Michal Karpinski

(Abridged) We revisit the problem of parameter estimation of gravitational-wave chirp signals from inspiralling non-spinning compact binaries in the light of the recent extension of the post-Newtonian (PN) phasing formula to order $(v/c)^7$…

General Relativity and Quantum Cosmology · Physics 2014-11-17 K. G. Arun , Bala R Iyer , B. S. Sathyaprakash , Pranesh A. Sundararajan

A novel characterization method to measure the pulse duration of ultrafast near-IR pulses is introduced, which uses simple tabletop optics, is relatively inexpensive, and is expected to work in a broad wavelength range. Our diagnostic tool…

Optics · Physics 2023-10-18 Rafeeq Syed , Cornelis J. G. J. Uiterwaal

We introduce the first method to enable an optical amplification of a coherent Raman spectroscopy signal called radio frequency Doppler Raman spectroscopy. Doppler Raman measurements amplify the optical signals in coherent Raman…

High-energy femtosecond laser pulses in the mid-infrared (MIR) wavelength range are essential for a wide range of applications from strong-field physics to selectively pump and probe low energy excitations in condensed matter and molecular…

Interferometers measure a wide variety of dynamic processes by converting a phase change into an intensity change. Nonlinear interferometers, making use of nonlinear media in lieu of beamsplitters, promise substantial improvement in the…

Quantum Physics · Physics 2016-11-16 Joseph M. Lukens , Nicholas A. Peters , Raphael C. Pooser

We study the effect of the chirped laser pulse on the transmission and associated ion acceleration by the sub-wavelength target. In the chirped laser pulses, the pulse frequency has a temporal variation about its fundamental frequency,…

Plasma Physics · Physics 2018-11-06 Shivani Choudhary , Amol R. Holkundkar

Ultra-intense laser-matter interaction experiments (>10$^{18}$ W/cm$^{2}$) with dense targets are highly sensitive to the effect of laser "noise" (in the form of pre-pulses) preceding the main ultra-intense pulse. These system-dependent…

Instrumentation and Detectors · Physics 2015-06-22 S. Feister , J. A. Nees , J. T. Morrison , K. D. Frische , C. Orban , E. A. Chowdhury , W. M. Roquemore

Conoscopic interferometry is a promising detection technique for ultrafast acoustics. By focusing a probe beam through a birefringent crystal before passing it through a polarizer, conoscopic interferences sculpt the spatial profile of the…

Applied Physics · Physics 2022-11-08 Martin Robin , Ruben Guis , Mustafa Umit Arabul , Zili Zhou , Nitesh Pandey , Gerard J. Verbiest