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Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

To better understand the many effects of temperature on the optical properties of metals, we experimentally and theoretically quantify the electron vs. phonon contributions to the thermoreflectance spectra of gold. We perform a series of…

Materials Science · Physics 2021-10-26 Kexin Liu , Xinping Shi , Frank Angeles , Ramya Mohan , Jon Gorchon , Sinisa Coh , Richard B. Wilson

We show a marked reduction in the emission from nitrogen-vacancy (NV) color centers in single crystal diamond due to exposure of the diamond to hydrogen plasmas ranging from 700{\deg}C to 1000{\deg}C. Significant fluorescence reduction was…

The negatively charged Nitrogen-Vacancy (NV-) center in diamond is one of the most versatile and robust quantum sensors suitable for quantum technologies, including magnetic field and temperature sensors. For precision sensing applications,…

Spectral diffusion is the phenomenon of random jumps in the emission wavelength of narrow lines. This phenomenon is a major hurdle for applications of solid state quantum emitters like quantum dots, molecules or diamond defect centers in an…

As promising quantum sensors, nitrogen-vacancy (NV) centers in diamond have been widely used in frontier studies in condensed matter physics, material sciences, and life sciences. In practical applications, weak laser excitation is…

Nitrogen-vacancy (NV-) color centers in diamond were created by implantation of 7 keV 15N (I = 1/2) ions into type IIa diamond. Optically detected magnetic resonance was employed to measure the hyperfine coupling of the NV- centers. The…

Optical coating, an integral part of many optical systems, is prone to damage from environmental exposure and laser irradiation. This underscores the need for reliable and sensitive coating diagnostics. We introduce second harmonic…

We demonstrate precise control over the zero-phonon optical transition energies of individual nitrogen-vacancy (NV) centers in diamond by applying multiaxis electric fields, via the dc Stark effect. The Stark shifts display surprising…

Mesoscale and Nanoscale Physics · Physics 2015-03-19 L. C. Bassett , F. J. Heremans , C. G. Yale , B. B. Buckley , D. D. Awschalom

We present an analytical theory of second harmonic generation (SHG) in hybrid structures combining a nonlinear 2D crystal with a dielectric metasurface waveguide. The theory describes the excitation spectrum and enhancement of SHG at both…

Optics · Physics 2025-11-07 Egor S. Vyatkin , Sergey A. Tarasenko

By employing a pump-probe technique for enhanced spectral mapping of the dynamics in nonlinear frequency conversion, we demonstrate that photo-induced second-harmonic generation (SHG) in silicon nitride (Si3N4) microresonators can persist…

The temperature evolution of the resonant Raman scattering from high-quality bilayer 2H-MoS$_{2}$ encapsulated in hexagonal BN flakes is presented. The observed resonant Raman scattering spectrum as initiated by the laser energy of 1.96 eV,…

Giant second-harmonic generation (SHG) in the terahertz (THz) frequency range is observed in a thin film of an s-wave superconductor NbN, where the time-reversal ($\mathcal{T}$-) and space-inversion ($\mathcal{P}$-) symmetries are…

Superconductivity · Physics 2020-08-31 Sachiko Nakamura , Kota Katsumi , Hirotaka Terai , Ryo Shimano

Incipient ferroelectric KTaO3 with off-center Li impurity of the critical concentration of 2.8 mol% was investigated in order to clarify the dipole glass state under electric field. Using optical second-harmonic generation (SHG) microscope,…

Materials Science · Physics 2009-11-11 Hiroko Yokota , Taeko Ohyama , Yoshiaki Uesu

Spectroscopy of the centrosymmetric magnetic semiconductors EuTe and EuSe reveals spin-induced optical second harmonic generation (SHG) in the band gap vicinity at 2.1-2.4eV. The magnetic field and temperature dependence demonstrates that…

We performed high-temperature luminescence studies of silicon-vacancy color centers obtained by ion implantation in single crystal diamond. We observed reduction of the integrated fluorescence upon increasing temperature, ascribable to a…

Nitrogen-vacancy (NV) centers in diamond have shown promise as inherently localized electric-field sensors, capable of detecting individual charges with nanometer resolution. Working with NV ensembles, we demonstrate that a detailed…

Quantum Physics · Physics 2021-09-28 M. Block , B. Kobrin , A. Jarmola , S. Hsieh , C. Zu , N. L. Figueroa , V. M. Acosta , J. Minguzzi , J. R. Maze , D. Budker , N. Y. Yao

We report polarization of a dense nuclear-spin ensemble in diamond and its dependence on magnetic field and temperature. The polarization method is based on the transfer of electron spin polarization of negatively charged nitrogen vacancy…

Quantum Physics · Physics 2013-04-01 Ran Fischer , Andrey Jarmola , Pauli Kehayias , Dmitry Budker

The nitrogen-vacancy (NV) color center in diamond has demonstrated great promise in a wide range of quantum sensing. Recently, there have been a series of proposals and experiments using NV centers to detect spin noise of quantum materials…

Mesoscale and Nanoscale Physics · Physics 2023-04-14 Jacob Henshaw , Pauli Kehayias , Luca Basso , Michael Jaris , Rong Cong , Michael Titze , Tzu-Ming Lu , Michael P. Lilly , Andrew M. Mounce

Lead sulfide is an important semiconductor that has found technological applications for over a century. Raman spectroscopy, a standard tool for the investigation and characterization of semiconductors, has limited application to this…

Materials Science · Physics 2015-05-13 P. G. Etchegoin , M. Cardona , R. Lauck , R. J. H. Clark , J. Serrano , A. H. Romero