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The sharp optical resonances of NV- centers in diamond at cryogenic temperatures offer powerful new capabilities for material characterization, but extracting the most detailed information typically requires careful calibration of…

Materials Science · Physics 2025-11-06 Jason Shao , Richard Monge , Tom Delord , Carlos A. Meriles

The advancement of quantum optical science and technology with solid-state emitters such as nitrogen-vacancy (NV) centers in diamond critically relies on the coherence of the emitters' optical transitions. A widely employed strategy to…

In this work, we explore the ability of plasma assisted chemical vapor deposition (PACVD) operating under high power densities to produce thin high-quality diamond layers with a controlled doping with negatively-charged nitrogen-vacancy…

Materials Science · Physics 2015-04-09 A. Tallaire , M. Lesik , V. Jacques , S. Pezzagna , V. Mille , O. Brinza , J. Meijer , B. Abel , J. -F. Roch , A. Gicquel , J. Achard

The ultrathin one-dimensional sp3 diamond nanothreads (NTHs), as successfully synthesised recently, have greatly augmented the interests from the carbon community. In principle, there can exist different stable NTH structures. In this work,…

Materials Science · Physics 2018-03-20 Haifei Zhan , Gang Zhang , John M. Bell , Yuantong Gu

We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…

We demonstrate the cooling of a microwave mode at 2872 MHz through its interaction with optically spin-polarized NV$^-$ centers in diamond at zero applied magnetic field, removing thermal photons from the mode. By photo-exciting (pumping) a…

Quantum Physics · Physics 2022-03-08 Wern Ng , Hao Wu , Mark Oxborrow

Second harmonic generation (SHG) is a coherent nonlinear phenomenon that plays an important role in laser color conversion. Lithium niobate (LN), which features both a large band gap and outstanding second-order nonlinearities, acts as an…

Temperature dependence of Fano resonance, recently discovered in infra-red (IR spectra of nanodiamonds synthesized from chloroadamantane at high static pressures, is investigated. For the first time, marked variations of the resonance…

Mesoscale and Nanoscale Physics · Physics 2022-08-10 A. A. Shiryaev , E. A. Ekimov , V. Yu. Prokof'ev , M. V. Kondrin

We report depth-resolved photoluminescence measurements of nitrogen-vacancy (NV$^-$) centers formed along the tracks of swift heavy ions (SHIs) in type Ib synthetic single crystal diamonds that had been doped with 100 ppm nitrogen during…

The nonlinear frequency conversion of low-temporal-coherent light holds a variety of applications and has attracted considerable interest. However, its physical mechanism remains relatively unexplored, and the conversion efficiency and…

Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…

An optical Second-Harmonic Generation (SHG) allows to probe various structural and symmetry-related properties of materials, since it is sensitive to the inversion symmetry breaking in the system. Here, we investigate the SHG response from…

Mesoscale and Nanoscale Physics · Physics 2019-05-08 M. Vandelli , M. I. Katsnelson , E. A. Stepanov

We investigate ultrafast harmonic generation (HG) in Si:B, driven by intense pump pulses with fields reaching ~100 kV/cm and a carrier frequency of 300 GHz, at 4 K and 300 K, both experimentally and theoretically. We report several novel…

Recent numerical studies on glassy systems provide evidences for a population of non-Goldstone modes (NGMs) in the low-frequency spectrum of the vibrational density of states $D(\omega)$. Similarly to Goldstone modes (GMs), i. e., phonons…

Disordered Systems and Neural Networks · Physics 2019-11-26 Matteo Paoluzzi , Luca Angelani , Giorgio Parisi , Giancarlo Ruocco

Optical second harmonic generation (SHG) is studied from multilayer graphene films in the presence of DC electric current flowing in the sample plane. Graphene layers are manufactured by chemical vapour deposition (CVD) technique and…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Anton Y. Bykov , Tatiana V. Murzina , Maxim G. Rybin , Elena D. Obraztsova

Optical second-harmonic-generation(SHG) observations and precise X-ray diffraction experiments have been performed on quantum paraelectrics KTaO3 (KTO) and relaxor K(1-x)LixTaO3 with x=3% (KLT-3) and 7% (KLT-7). It is found in KLT-3 and…

Materials Science · Physics 2009-11-11 Hiroko Yokota , Yoshiaki Uesu , Charlotte Malibert , Jean-Michel Kiat

We use second and third harmonic generation microscopy to investigate the nonlinear optical response of GaAs nanocavities embedded in a gold film and compare them to bare GaAs nanocavities. Our results reveal that the surrounding metallic…

Second-order nonlinear optical interactions such as sum- and difference-frequency generation are widely used for bioimaging and as selective probes of interfacial environments. However, inefficient nonlinear optical conversion often leads…

Optics · Physics 2015-05-07 Aaron J. Goodman , William A. Tisdale

We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…

Mesoscale and Nanoscale Physics · Physics 2017-04-13 Peter R. Wiecha , Arnaud Arbouet , Houssem Kallel , Priyanka Periwal , Thierry Baron , Vincent Paillard

We report an experimental design where the position and resonance frequency of the Nitrogen Vacancy (NV) in a diamond are correlated with the room temperature. A simple model trained on the interpolated correlation data predicts both…

Quantum Physics · Physics 2026-01-06 Manpreet Singh Jattana , Thomas Lippert