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Extreme ultraviolet pulses as generated by high harmonic generation (HHG) are a powerful tool for both time-resolved spectroscopy and coherent diffractive imaging. However, the integration of spectroscopy and microscopy to harness the…

Existing super-resolution methods of optical imaging hold a solid place as an application in natural sciences, but many new developments allow for beating the diffraction limit in a more subtle way. One of the recently explored strategies…

Quantum Physics · Physics 2022-02-08 Mateusz Mazelanik , Adam Leszczyński , Michał Parniak

When multifrequency Raman scattering is driven in the transient regime by two chirped pump pulses, the resulting anti-Stokes orders exhibit asymmetric spectral broadening toward lower frequencies, leading to a characteristic double-peaked…

We present an optical method to measure radio-frequency electro-optic phase modulation profiles by employing spectrum-to-time mapping realized by highly chirped optical pulses. We directly characterize temporal phase modulation profiles of…

Instrumentation and Detectors · Physics 2017-11-23 Michał Jachura , Jan Szczepanek , Wojciech Wasilewski , Michal Karpinski

Exploiting the correspondence between Wigner distribution function and a frequency-resolved optical gating (FROG) measurement, we experimentally demonstrate existence of the chessboard-like interference patterns with a time-bandwidth…

Quantum Physics · Physics 2016-06-01 Ludmila Praxmeyer , Chih-Cheng Chen , Popo Yang , Shang-Da Yang , Ray-Kuang Lee

We introduce a self-referenced method for quantum-state tomography of light based on photon-number-resolved double-slit interferometry. Two identical copies of the unknown quantum field illuminate laterally displaced slits, guaranteeing…

Optics · Physics 2025-12-10 Matan Even Tzur

Sum-frequency generation (SFG) spectroscopy provides a versatile method for the investigation of non-centrosymmetric media and interfaces. Here, using tunable picosecond infrared (IR) pulses from a free-electron laser, the nonlinear optical…

Materials Science · Physics 2023-08-01 Riko Kiessling , Martin Wolf , Alexander Paarmann

The resolution limits of classical spectroscopy can be surpassed by quantum-inspired methods leveraging the information contained in the phase of the complex electromagnetic field. Their counterpart in spatial imaging has been widely…

Optics · Physics 2024-09-02 Michał Lipka , Michał Parniak

A Python package for the calculation of spectrograms with optimized time and frequency resolution for application in the analysis of numerical simulations on ultrashort pulse propagation is presented. Gabor's uncertainty principle prevents…

Computational Physics · Physics 2018-09-05 O. Melchert , B. Roth , U. Morgner , A. Demircan

The wave nature of light is revealed by diffraction from physical structures. We report a time-domain version of the classic Young's double-slit experiment: a beam of light twice gated in time produces an interference in the frequency…

We present a common pulse retrieval algorithm (COPRA) that can be used for a broad category of ultrashort laser pulse measurement schemes including frequency-resolved optical gating (FROG), interferometric FROG, dispersion scan, time domain…

Instrumentation and Detectors · Physics 2019-04-16 Nils C. Geib , Matthias Zilk , Thomas Pertsch , Falk Eilenberger

Fourier transform spectroscopy (FTS) has been widely used in a variety of fields in research, industry, and medicine due to its high signal-to-noise ratio, simultaneous acquisition of signals in a broad spectrum, and versatility for…

Interferometric imaging is a well established method to image phase objects by mixing the image wavefront with a reference one on a CCD camera. It has also been applied to fast transient phenomena, mostly through the analysis of single…

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

While frequency-resolved optical gating (FROG) is widely used in characterizing the ultrafast pulse in optics, analytic signals are often considered in time-frequency analysis and signal processing, especially when extracting instantaneous…

Signal Processing · Electrical Eng. & Systems 2021-03-17 Youfa Li , Yaoshuai Ma , Deguang Han

Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…

Quantum Physics · Physics 2017-08-22 Kochise Bennett , Jeremy Rouxel , Shaul Mukamel

Femtosecond interferometry combined with acousto-optical phase modulation is an effective approach to implement various types of coherent nonlinear and multidimensional spectroscopy schemes. The high sensitivity of this method has recently…

Atomic Physics · Physics 2025-02-24 Friedemann Landmesser , Nicolai Gölz , Ulrich Bangert , Tobias Sixt , Lukas Bruder

The precise temporal characterization of laser pulses is crucial for ultrashort applications in biology, chemistry, and physics. Especially in femto- and attosecond science, diverse laser pulse sources in different spectral regimes from the…

Dual-comb spectroscopy can provide broad spectral bandwidth and high spectral resolution in a short acquisition time, enabling time-resolved measurements. Specifically, spectroscopy in the mid-infrared wavelength range is of particular…