Related papers: Asymmetric double-pulse interferometric frequency-…
Two-color side-view probing of light-matter interaction from minute focal volume of a tightly focused fs-laser pump pulse reveals charge dynamics with high 0.9 micrometers optical resolution and approximately ~20 fs temporal resolution in…
Time-resolved atom interferometry, as employed in applications such as gravitational wave detection and searches for ultra-light dark matter, requires precise control over systematic effects. In this work, we investigate phase noise arising…
Interferometric measurements of high-harmonics induced by multiple laser fields in an emerging field of research that promises optimized yield of harmonics, and time and space-resolved nonlinear spectroscopy. Most of the measurements have…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…
The periodicity inherent to any interferometric signal entails a fundamental trade-off between sensitivity and dynamic range of interferometry-based sensors. Here we develop a methodology for significantly extending the dynamic range of…
We present an alternative approach to pump-probe spectroscopy for measuring fast charge dynamics with an atomic force microscope (AFM). Our approach is based on coherent multifrequency lock-in measurement of the intermodulation between a…
In this paper we present proof of principle experiments of an optical gating concept for free electrons. We demonstrate a temporal resolution of 1.2+-0.3 fs via energy and transverse momentum modulation as a function of time. The scheme is…
Precise measurement of multi-parameters of ultrafast lasers is vital both in scientific investigations and technical applications, such as, optical field manipulation, pulse shaping, sample characteristics test, and biomedical imaging.…
This letter presents a dual quadrature phasemeter, an implementation of a phase-locked loop designed to track the phase of homodyne and heterodyne inter-satellite laser links. The dual quadrature phasemeters use dual quadrature optical…
We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…
The near-field diffraction of fs and sub-fs light pulses by nm-size slit-type apertures and its implication for near-field scanning optical microscopy (NSOM) is analyzed. The amplitude distributions of the diffracted wave-packets having the…
Much work over the last 25 years has demonstrated that the interface-specific, alloptical technique, vibrational sum frequency generation (v-SFG) spectroscopy, is often uniquely capable of characterizing the structure and dynamics of…
Characterizing quantum states of the electromagnetic field at microwave frequencies requires fast and sensitive detectors that can simultaneously probe the field time-dependent amplitude and its quantum fluctuations. In this work, we…
Multi-photon dressing and interference in atomic systems is a key to several cutting edge technologies like Rydberg atom radio frequency sensors, clocks and magnetometers because it enables the engineering of atomic properties. Rydberg atom…
Sub-cycle optical pulse is of great importance for ultrafast science and technology. While a narrower pulse can offer a higher temporal resolution, so far the pulse width has not reached the limit of half an optical cycle. Here we propose…
We develop the two-electron attosecond streak camera under realistic conditions using a quasi-classical model. We assume extreme ultra-violet (XUV) attosecond pulses with a full width at half maximum (FWHM) of 24 attoseconds, centered at…
We present a rapid-scanning approach to fluorescence-detected two-dimensional electronic spectroscopy that combines acousto-optic phase-modulation with digital lock-in detection. The approach shifts the signal detection window to suppress…
Transparent conducting oxides (TCO) such as indium-tin-oxide (ITO) exhibit strong optical nonlinearity in the frequency range where their permittivities are near zero. We leverage this nonlinear optical response to realize a sub-picosecond…
The attosecond high harmonic pulses obtained from a long Ar-filled gas cell were characterized by two techniques - the reconstruction of attosecond beating by interference of two-photon transition (RABITT) and frequency-resolved optical…
We investigate the system of a heavy impurity immersed in a degenerated Fermi gas, where the impurity's internal degree of freedom (pseudospin) is manipulated by a series of radiofrequency (RF) pulses at several different times. Applying…