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We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…

Atomic Physics · Physics 2019-05-15 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

We demonstrate fluorescence generation through a sequential multiphoton process with real intermediary states. Our findings suggest new directions for optical control of previously unexplored molecular excitation pathways.

Optics · Physics 2025-02-03 J. David Wong-Campos , Mackenzie Dion

Quantum coherence plays a fundamental role in the study and control of ultrafast dynamics in matter. In the case of photoionization, entanglement of the photoelectron with the ion is a well known source of decoherence when only one of the…

We investigate photoisomerization (PI), the shape change of a molecule upon photoabsorption, in a dissipative environment using a simple spin-boson model. We identify two classes of environment depending on whether it "entangles" with the…

Materials Science · Physics 2007-05-23 Chang-Qin Wu , Jian-Xin Li , Dung-Hai Lee

We propose an interferometry experiment for the detection of axion-like particles (ALPs). As in ordinary photon-regeneration (light shining through a wall) experiments, a laser beam traverses a region permeated by a magnetic field, where…

High Energy Physics - Phenomenology · Physics 2018-08-28 H. Tam , Q. Yang

Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…

Atomic Physics · Physics 2021-06-30 Saad Mehmood , Eva Lindroth , Luca Argenti

Second-harmonic and sum-frequency mixing phenomena associated with 3D-localized photonic modes are studied in InP-based planar photonic crystal microcavities excited by short-pulse radiation near 1550 nm. Three-missing-hole microcavities…

Using the photon-ion merged-beams technique at the PETRA\,III synchrotron light source, we have measured cross sections for double and up to tenfold photoionization of La$^{+}$ ions by a single photon in the energy range 820--1400~eV, where…

Sulfur difluoride radicals in their ground state have been produced by a "laser-free" pulsed dc discharge of the SF$_{6}$/Ar gas mixtures in a supersonic molecular beam and detected by mass-selective resonance-enhanced multilphoton…

Chemical Physics · Physics 2008-08-11 Qun Zhang , Xiaoguo Zhou , Quanxin Li , Shuqin Yu , Xingxiao Ma

We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…

Optics · Physics 2019-05-01 Tsogvoo Khos-Ochir , Kim Myung-Whun , Purevdorj Munkhbaatar

We consider the decoherence of photons suffering in phase-damping channels. By exploring the evolutions of single-photon polarization states and two-photon polarization-entangled states, we find that different frequency spectrum envelopes…

Quantum Physics · Physics 2008-10-08 Yan-Xiao Gong , Yong-Sheng Zhang , Yu-Li Dong , Xiao-Ling Niu , Yun-Feng Huang , Guang-Can Guo

Pre-plasma conditions strongly influence laser-plasma interactions in the multi-petawatt (MPW) regime, increasing the need for reliable early-time plasma evolution diagnostics. Among available pre-plasma diagnostics, interferometry remains…

We study nondipole effects in multiphoton ionization of a two-dimensional hydrogen-like atom by a flat-top laser pulse of varied intensity. For this purpose, we solve numerically a two-dimensional Schr\"odinger equation treating a…

Atomic Physics · Physics 2024-12-25 J. Z. Kamiński , K. Krajewska

Within the scope of the relativistic quantum theory for electron-laser interaction in a medium and using the resonant approximation for the two degenerated states of an electron in a monochromatic radiation field [1] a nonperturbative…

Quantum Physics · Physics 2007-05-23 H. K. Avetissian , A. L. Khachatryan , G. F. Mkrtchian

Magnetic particle imaging (MPI) is a non-invasive, non-ionizing imaging technique for the visualization and quantification of magnetic nanoparticles (MNPs). The technique is especially suitable for cell imaging as it offers zero background…

Interferometric imaging is a well established method to image phase objects by mixing the image wavefront with a reference one on a CCD camera. It has also been applied to fast transient phenomena, mostly through the analysis of single…

We analyse recently measured nonlinear photoemission spectra from Ag surfaces that reveal resonances whose energies do not scale with the applied photon energy but stay pinned to multiples of bulk plasmon energy $\hbar\omega_p$ above the…

Materials Science · Physics 2021-05-05 Dino Novko , Vito Despoja , Marcel Reutzel , Andi Li , Hrvoje Petek , Branko Gumhalter

We demonstrate that important information about linear optical circuits can be obtained through the phase shift induced by integrated optical resonators. As a proof of principle, the phase of an unbalanced Mach-Zehnder interferometer is…

Optics · Physics 2016-11-03 Menno Poot , Hong X. Tang

The introduction of mid-IR optical parametric chirped pulse amplifiers (OPCPAs) has catalyzed interest in multi-millijoule, infrared femtosecond pulse-based filamentation. As tunneling ionization is a fundamental first stage in these…

We describe a method of selective generation and study of polarization moments of up to the highest rank $\kappa=2F$ possible for a quantum state with total angular momentum $F$. The technique is based on nonlinear magneto-optical rotation…

Atomic Physics · Physics 2009-11-10 V. V. Yashchuk , D. Budker , W. Gawlik , D. F. Kimball , Yu. P. Malakyan , S. M. Rochester