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Here, we report on the nonlinear ionization of argon atoms in the short wavelength regime using ultraintense x rays from the European XFEL. After sequential multiphoton ionization, high charge states are obtained. For photon energies that…

We propose a new scheme to control the shape of the Autler-Townes (AT) doublet in the photoelectron spectrum from atomic resonance-enhanced multiphoton ionization (REMPI). The scheme is based on the interference of two AT doublets created…

Atomic Physics · Physics 2025-07-01 T. Bayer , K. Eickhoff , D. Köhnke , M. Wollenhaupt

We study time-delays in atomic multiphoton ionization (MPI) using the phase-sensitive detection of photoelectron vortices. Photoelectron vortices are created by MPI with counter-rotating circularly polarized (CRCP) ultrashort double pulse…

Atomic Physics · Physics 2025-01-13 D. Köhnke , T. Bayer , M. Wollenhaupt

Resonance-enhanced multiphoton ionization (REMPI) in potassium atom is investigated within the strong coupling regime using photoelectron momentum imaging techniques. The kinetic energy distribution of the ionized electrons reveals the…

Atomic Physics · Physics 2025-03-10 Wankai Li , Yixuan Wang , Xing Li , Tao Yang , Dongdong Zhang , Dajun Ding

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

We study resonant two-color two-photon ionization of Helium via the 1s3p 1P1 state. The first color is the 15th harmonic of a tunable titanium sapphire laser, while the second color is the fundamental laser radiation. Our method uses…

Photoelectron circular dichroism (PECD) is a highly sensitive enantiospecific spectroscopy for studying chiral molecules in the gas phase using either single-photon ionization or multiphoton ionization. In the short pulse limit investigated…

The spectrum of electronic states at 30000--33000 cm$^{-1}$ in hafnium fluoride has been studied using (1+1) resonance-enhanced multi-photon ionization (REMPI) and (1+1$'$) REMPI. Six $\Omega' = 3/2$ and ten $\Pi_{1/2}$ vibronic bands have…

In optical detection of ultrasound, resonators with high Q-factors are often used to maximize sensitivity. However, in order to perform parallel interrogation, conventional interferometric techniques require an overlap between the resonator…

Optics · Physics 2019-01-27 Yoav Hazan , Amir Rosenthal

Laser induced plasmas have found numerous applications including plasma-assisted combustion, combustion diagnostics, laser induced breakdown spectroscopy, light detection and ranging techniques (LIDAR), microwave guiding, reconfigurable…

Plasma Physics · Physics 2017-10-11 A. Sharma , M. N. Slipchenko , M. N. Shneider , X. Wang , K. A. Rahman , A. Shashurin

We photoionize nitrogen molecules with a train of extreme ultraviolet attosecond pulses together with a weak infrared field. We measure the phase of the two-color two-photon ionization transition (molecular phase) for different states of…

We theoretically study multiphoton ionization of the Ca atom irradiated by the second (photon energy 3.1 eV) and third (photon energy 4.65 eV) harmonics of Ti:sapphire laser pulses (photon energy 1.55 eV). Because of the dense energy level…

Atomic Physics · Physics 2013-03-07 Gabriela Buica , Takashi Nakajima

The intermediate state dependence of photoelectron circular dichroism (PECD) in resonance-enhanced multi-photon ionization of fenchone in the gas phase is experimentally studied. By scanning the excitation wavelength from 359 to 431 nm we…

We report the first observation of free-electron angular momentum wave packets generated by atomic multiphoton ionization with bichromatic three-dimensional (3D) polarization-tailored ultrashort laser fields. These fields, created by the…

Atomic Physics · Physics 2025-11-25 Darius Köhnke , Hans-Christian Ahlswede , Tim Bayer , Matthias Wollenhaupt

We theoretically study multiphoton ionization through the triplet states of Mg by linearly polarized (LP) and circularly polarized (CP) fs laser pulses. After the construction of the atomic basis using the frozen-core Hartree-Fock potential…

Atomic Physics · Physics 2013-03-07 Gabriela Buica , Takashi Nakajima

The ability to prepare molecular ions in selected quantum states enables studies in areas such as chemistry, metrology, spectroscopy, quantum information, and precision measurements. Here, we demonstrate $(2+1)$ resonance-enhanced…

Using a linear optical elements and post-selection, we construct an entangled polarization state of three photons in the same spatial mode. This state is analogous to a ``photon-number path entangled state'' and can be used for…

Quantum Physics · Physics 2009-11-10 M. W. Mitchell , J. S. Lundeen , A. M. Steinberg

We present ionization probability and line shape calculations for the two-step 3-photon ionization process, $1S \stackrel{2\hbar \omega}{\longrightarrow}2S \stackrel{\hbar \omega}{\longrightarrow}\epsilon P $, of the ground state of…

Atomic Physics · Physics 2016-08-15 V Yakhontov , R. Santra , K. Jungmann

We measure the photoelectron energy spectra from strong-field ionization of Kr in a two-color laser pulse consisting of a strong 400-nm field and a weak 800-nm field. The intensities of the main above-threshold ionization (ATI) and sideband…

Atomic Physics · Physics 2019-12-11 Yudi Feng , Min Li , Siqiang Luo , Kun Liu , Baojie Du , Yueming Zhou , Peixiang Lu

We present a joint experimental and theoretical study on strong-field photo-ionization of sodium atoms using chirped femtosecond laser pulses. By tuning the chirp parameter, selectivity among the population in the highly excited states 5p,…

Atomic Physics · Physics 2015-05-28 M Krug , T Bayer , M Wollenhaupt , C Sarpe-Tudoran , T Baumert , S S Ivanov , N V Vitanov
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