English

Resonant two-photon ionization of helium atoms studied by attosecond interferometry

Atomic Physics 2022-06-30 v1

Abstract

We study resonant two-photon ionization of helium atoms via the 1s3p1s3p, 1s4p1s4p and 1s5p11s5p^1P1_1 states using the 15th^\mathrm{th} harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the ionization. The phase of the photoelectron wavepackets is measured by an attosecond interferometric technique, using the 17th^\mathrm{th} harmonic. We perform experiments with angular resolution using a velocity map imaging spectrometer and with high energy resolution using a magnetic bottle electron spectrometer. Our results are compared to calculations using the two-photon random phase approximation with exchange to account for electron correlation effects. We give an interpretation for the multiple π\pi-rad phase jumps observed, both at and away from resonance, as well as their dependence on the emission angle.

Keywords

Cite

@article{arxiv.2206.14299,
  title  = {Resonant two-photon ionization of helium atoms studied by attosecond interferometry},
  author = {Lana Neoričić and David Busto and Hugo Laurell and Robin Weissenbilder and Mattias Ammitzböll and Sizuo Luo and Jasper Peschel and Hampus Wikmark and Jan Lahl and Sylvain Maclot and Richard James Squibb and Shiyang Zhong and Per Eng-Johnsson and Cord Louis Arnold and Raimund Feifel and Mathieu Gisselbrecht and Eva Lindroth and Anne L'Huillier},
  journal= {arXiv preprint arXiv:2206.14299},
  year   = {2022}
}