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We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

Coherent spin resonance techniques, such as nuclear and electron spin resonance spectroscopy, have revolutionized non-invasive imaging by providing spectrally resolved information about spin dynamics. Motivated by the recent emergence of…

Quantum Physics · Physics 2026-02-25 Santiago Beltrán-Romero , Stefan Löffler , Dennis Rätzel , Philipp Haslinger

NMR experiments, indispensable to chemists in many areas of research, are often run with generic, unoptimised experimental parameters. This approach makes robust and automated acquisition on different samples and instruments extremely…

Systems and Control · Electrical Eng. & Systems 2021-08-17 Jonathan R. J. Yong , Mohammadali Foroozandeh

We demonstrate a new method for electrical manipulation of nuclear spins utilizing dynamic nuclear polarization induced by quantum Hall effect breakdown. Nuclear spins are polarized and detected through the hyperfine interaction between a…

Mesoscale and Nanoscale Physics · Physics 2009-04-17 Minoru Kawamura , Hiroyuki Takahashi , Yoshiaki Hashimoto , Shingo Katsumoto , Tomoki Machida

Rapid injection of spin polarization into an ensemble of nuclear spins is a problem of broad interest, spanning dynamic nuclear polarization (DNP) to quantum information science. We report on a strategy to boost the spin injection rate by…

Color centers that enable nuclear-spin control without RF fields offer a powerful route towards simplified and scalable quantum devices. Such capabilities are especially valuable for quantum sensing and computing platforms that already find…

Hyperpolarization methods in magnetic resonance overcome sensitivity limitations, especially for low-{\gamma} nuclei such as 13C and 15N. Signal Amplification By Reversible Exchange (SABRE) and extended SABRE (X-SABRE) are efficient and…

Chemical Physics · Physics 2022-04-06 Jacob R. Lindale , Shannon L. Eriksson , Warren S. Warren

By leveraging the hyperfine interaction between the rotational and nuclear spin degrees of freedom, we demonstrate extensive magnetic control over the electric dipole moments, electric dipolar interactions, and ac Stark shifts of…

Atomic Physics · Physics 2024-01-11 Rebekah Hermsmeier , Ana Maria Rey , Timur V. Tscherbul

In heavy atoms and ions, nuclear structure effects are significantly enhanced due to the overlap of the electron wave functions with the nucleus. This overlap rapidly increases with the nuclear charge $Z$. We study the energy level shifts…

Atomic Physics · Physics 2021-03-17 V. V. Flambaum , I. B. Samsonov , H. B. Tran Tan , A. V. Viatkina

Spatially nonhomogeneously spin polarized nuclei are proposed as a new mechanism to monitor electron states in a nanostructure, or as a means to createn and, if necessary, reshape such nanostructures in the course of the experiment. We…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 V. Fleurov , V. A. Ivanov , F. M. Peeters , I. D. Vagner

Quantum sensing based on nitrogen-vacancy (NV) centers in diamond has been developed as a powerful tool for microscopic magnetic resonance. However, the reported sensor-to-sample distance is limited within tens of nanometers because the…

Here, we demonstrate the radiative polarization of high-energy electron beams in collisions with ultrashort pulsed bi-chromatic laser fields. Employing a Boltzmann kinetic approach for the electron distribution allows us to simulate the…

Plasma Physics · Physics 2019-12-06 Daniel Seipt , Dario Del Sorbo , Christopher P. Ridgers , Alec G. R. Thomas

Nanoscale nuclear magnetic resonance (NMR) signals can be measured through hyperfine interaction to paramagnetic electron sensor spins. A heterodyne approach is widely used to overcome the electron spin lifetime limit in spectral…

Electric control of spins has been a longstanding goal in the field of solid state physics due to the potential for increased efficiency in information processing. This efficiency can be optimized by transferring spintronics to the atomic…

Mesoscale and Nanoscale Physics · Physics 2023-11-30 Piotr Kot , Maneesha Ismail , Robert Drost , Janis Siebrecht , Haonan Huang , Christian R. Ast

From the study of long-range-interacting systems to the simulation of gauge fields, open-shell Lanthanide atoms with their large magnetic moment and narrow optical transitions open novel directions in the field of ultracold quantum gases.…

Magnetosensitive spin-correlated radical-pairs (SCRPs) offer a promising platform for noise-robust quantum metrology. However, unavoidable interradical interactions, such as electron-electron dipolar and exchange couplings, alongside…

Quantum Physics · Physics 2026-02-25 Luke D. Smith , Farhan T. Chowdhury , Jonas Glatthard , Daniel R. Kattnig

In quantum information science and sensing, electron spins are often purified into a specific polarisation through an optical-spin interface, a process known as optically-detected magnetic resonance (ODMR). Diamond-NV centres and transition…

Chemical Physics · Physics 2024-11-22 Yong Rui Poh , Joel Yuen-Zhou

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle…

Stochasticity effects in the spin (de)polarization of an ultrarelativistic electron beam during photon emissions in a counterpropoagating ultrastrong focused laser pulse in the quantum radiation reaction regime are investigated. We employ a…

We devise an approach to measure the polarization of nuclear spins via conductance measurements. Specifically, we study the combined effect of external magnetic field, nuclear spin polarization, and Rashba spin-orbit interaction on the…

Mesoscale and Nanoscale Physics · Physics 2010-10-12 James A. Nesteroff , Yuriy V. Pershin , Vladimir Privman