Related papers: Macroscopic Hyperpolarization Enhanced with Quantu…
Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…
Pure, highly nuclear-spin-polarized molecules have only been produced with molecular beam-separation methods, with production rates up to ${\sim}3{\times}10^{12}$ s$^{-1}$. Here, we propose the production of spin-polarized molecular…
Nitrogen-vacancy (NV) center ensembles have the potential to improve a wide range of applications, including nuclear magnetic resonance spectroscopy at the microscale and nanoscale, wide-field magnetometry, and hyperpolarization of nuclear…
Noble-gas spins feature hours long coherence times owing to their great isolation from the environment, and find practical usage in various applications. However, this isolation leads to extremely slow preparation times, relying on weak…
The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…
Magnetic resonance spectroscopy is universally regarded as one of the most important tools in chemical and bio-medical research. However, sensitivity limitations typically restrict imaging resolution to length scales greater than 10 \mu m.…
Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…
The control of nuclear spins in quantum dots is essential to explore their many-body dynamics and exploit their prospects for quantum information processing. We present a unique combination of dynamic nuclear spin polarization and…
We demonstrate ionization of a molecule with the bias voltage of a Scanning Tunnelling Microscope (STM) resulting in a coexistence of a neutral and ionic molecules, i.e. radical (paramagnetic) and non-radical (diamagnetic) states. This…
Periodic excitation of electron spin polarization by consecutive laser pulses in phase with Larmor spin precession about a magnetic field results in resonant spin amplification (RSA). We observe a drastic modification of RSA in $n$-doped…
Magnetic resonance imaging with hyperpolarized contrast agents can provide unprecedented \textit{in-vivo} measurements of metabolism, but yields images that are lower resolution than that achieved with proton anatomical imaging. In order to…
Magnetic noise of atomic nuclear spins is a major problem for solid state spin qubits. Highly-polarized nuclei would not only overcome this obstacle, but also make nuclear spins a useful quantum information resource. However, achieving…
The possibility of realizing the regime of punctuated spin superradiance is advanced. In this regime, the number of superradiant pulses and the temporal intervals between them can be regulated. This makes it feasible to compose a kind of…
The root raised-cosine pulse commonly used in linear digital modulations yields exactly two intersymbol interference components from the preceding and the subsequent data symbols, provided that the roll-off factor is $100\%$ and the…
A model of dynamic orientation using optimized radiofrequency (RF) irradiation produced perpendicular to the holding field is developed for the spin-1 system required for tensor-polarized fixed-target experiments. The derivation applies to…
Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…
Dynamic nuclear polarization via contact with electronic spins has emerged as an attractive route to enhance the sensitivity of nuclear magnetic resonance (NMR) beyond the traditional limits imposed by magnetic field strength and…
We describe a new approach to precision NMR with hyperpolarized gases designed to mitigate NMR frequency shifts due to the alkali spin exchange field. The electronic spin polarization of optically pumped alkali atoms is square-wave…
It is proposed that nuclear (or electron) spins in a trapped molecule would be well isolated from the environment and the state of each spin can be measured by means of mechanical detection of magnetic resonance. Therefore molecular traps…
Multipass cells enable long optical path lengths in compact volumes and are central to quantum technologies such as atomic magnetometers and optical quantum memories. In optical magnetometry, multipass geometries enhance sensitivity by…