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We show that detuned optical pulse trains with a modest spectral width can polarize nuclear spins in InAs quantum dots. The pulse bandwidth is large enough to excite a coherent superposition of both electron spin eigenstates in these…

Quantum Physics · Physics 2015-05-27 S. G. Carter , Sophia E. Economou , A. Shabaev , A. S. Bracker

Most of dynamic nuclear polarization (DNP) has been requiring helium cryogenics and strong magnetic fields for a high degree of polarization. In this work, we instead demonstrate an optical hyperpolarization of naturally abundant $^{13}$C…

We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

A promising platform for quantum information processing is that of silicon impurities, where the quantum states are manipulated by magnetic resonance. Such systems, in abstraction, can be considered as a nucleus of arbitrary spin coupled to…

Quantum Physics · Physics 2013-05-07 M. H. Mohammady

We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…

Quantum Physics · Physics 2019-10-25 Jiwon Yun , Kiho Kim , Dohun Kim

The shaping of nuclear spin polarization profiles and the induction of nuclear resonances are demonstrated within a parabolic quantum well using an externally applied gate voltage. Voltage control of the electron and hole wave functions…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Poggio , G. M. Steeves , R. C. Myers , Y. Kato , A. C. Gossard , D. D. Awschalom

We describe a new approach to spin squeezing based on a double-pass Faraday interaction between an optical probe and an optically dense atomic sample. A quantum eraser is used to remove residual spin-probe entanglement, thereby realizing a…

Quantum Physics · Physics 2013-05-29 Collin M. Trail , Poul S. Jessen , Ivan H. Deutsch

Entanglement can improve the measurement precision of quantum sensors beyond the shot noise limit. Neutral atoms, the basis of some of the most precise and accurate optical clocks and interferometers, do not naturally exhibit all-to-all…

We introduce a method for non-destructive quantification of nuclear spin polarization, of relevance to hyperpolarized spin tracers widely used in magnetic resonance from spectroscopy to in vivo imaging. In a bias field of around 30 nT we…

Magnetic spin resonance is a key non-invasive sensing and imaging technique across the life-, material- and fundamental sciences with further medical and commercial applications. Recent advances using paramagnetic color centers enable…

Mesoscale and Nanoscale Physics · Physics 2018-07-24 Florestan Ziem , Marwa Garsi , Helmut Fedder , Jörg Wrachtrup

PulsePol is an elegantly designed pulse-sequence-based quantum control scheme that enables polarization transfer between electron and nuclear spins, for example, in nitrogen-vacancy (NV) centers. However, previous analyses of PulsePol…

Conduction electrons are used to optically polarize, detect and manipulate nuclear spin in a (110) GaAs quantum well. Using optical Larmor magnetometry, we find that nuclear spin can be polarized along or against the applied magnetic field,…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 G. Salis , D. T. Fuchs , J. M. Kikkawa , D. D. Awschalom , Y. Ohno , H. Ohno

We theoretically study the interplay of spin-orbit and hyperfine interactions in dynamical nuclear polarization in two-electron semiconductor double quantum dots near the singlet $(S)$ - triplet $(T_+)$ anticrossing. The goal of the scheme…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Marko J. Rančić , Guido Burkard

Magnetic resonance imaging at microtesla fields is a promising imaging method that combines the pre-polarization technique and broadband signal reception by SQUID sensors to enable in vivo MRI at microtesla-range magnetic fields. Despite…

Medical Physics · Physics 2010-10-18 V. S. Zotev , T. Owens , A. N. Matlashov , I. M. Savukov , J. J. Gomez , M. A. Espy

Polarization-dependent photon spectroscopy (dichroism) using signal-enhancing superchiral beams is shown to be sensitive to magnetic properties of the sample, whereas previous investigations explored charge-like electronic properties of…

Materials Science · Physics 2019-03-06 S. W. Lovesey , J. T. Collins , S. P. Collins

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

Chemical Physics · Physics 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

Hyperpolarized nuclear spins in molecules exhibit high magnetization that is unachievable by classical polarization techniques, making them widely used as sensors in physics, chemistry, and medicine. The state of a hyperpolarized material,…

Chemical Physics · Physics 2024-12-31 James Eills , Morgan W. Mitchell , Irene Marco Rius , Michael C. D. Tayler

Electron spin resonance (ESR) is a useful tool to investigate properties of materials in magnetic fields where high spin polarization of target electron spins is required in order to obtain high sensitivity. However, the smaller magnetic…

Quantum Physics · Physics 2022-02-09 Shingo Kukita , Hideaki Ookane , Yuichiro Matsuzaki , Yasushi Kondo

In solid_state hybrid electron_nuclear spin systems quantum entanglement plays vital role in allowing accessible transfer of information between subatomic particles, regardless of the host lattice coordination spatial geometry, revealing…

Quantum Physics · Physics 2013-11-25 Vesna Berec , J. S. Braunstein
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