Related papers: Prospects for assembling ultracold radioactive mol…
The parameter $W_\mathrm{a}$, which characterizes nuclear spin-dependent parity violation effects within the effective molecular spin-rotational Hamiltonian, was computed for the electronic ground state of radium fluoride (RaF) and found to…
We investigate the presence of Feshbach resonances in ultracold alkali-dialkali reactive collisions. Quantum scattering calculations are performed on a new Na_3 quartet potential energy surface. An analysis of scattering features is…
It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…
We present measurements of the loss-rate coefficients K_am and K_mm caused by inelastic atom-molecule and molecule-molecule collisions. A thermal cloud of atomic 87Rb is prepared in an optical dipole trap. A magnetic field is ramped across…
We study collisions in an optically trapped, pure sample of ultracold Cs$_2$ molecules in various internal states. The molecular gas is created by Feshbach association from a near-degenerate atomic gas, with adjustable temperatures in the…
Reaching high densities is a key step towards cold-collision experiments with polyatomic molecules. We use a cryofuge to load up to 2$\times10^7$ CH$_3$F molecules into a box-like electric trap, achieving densities up to 10$^7$/cm$^3$ at…
Nuclear forces violating parity and time reversal invariance (${\cal P},{\cal T}$-odd) produce ${\cal P},{\cal T}$-odd nuclear moments, for example, the nuclear Schiff moment. In turn, this moment can induce the electric dipole moment in…
We describe the formation of fermionic NaLi Feshbach molecules from an ultracold mixture of bosonic 23Na and fermionic 6Li. Precise magnetic field sweeps across a narrow Feshbach resonance at 745 G result in a molecule conversion fraction…
We report on the observation of five Feshbach resonances in collisions between ultracold $^7$Li and $^{87}$Rb atoms in the absolute ground state mixture where both species are in their $|f,m_f>=|1,1>$ hyperfine states. The resonances appear…
Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecule…
We observe magnetically tuned collision resonances for ultracold Cs2 molecules stored in a CO2-laser trap. By magnetically levitating the molecules against gravity, we precisely measure their magnetic moment. We find an avoided level…
We have observed and located more than 60 magnetic field-induced Feshbach resonances in ultracold collisions of ground-state $^{133}$Cs atoms. These resonances are associated with molecular states with up to four units of rotational angular…
Ultracold dysprosium gases, with a magnetic moment ten times that of alkali atoms and equal only to terbium as the most magnetic atom, are expected to exhibit a multitude of fascinating collisional dynamics and quantum dipolar phases,…
The electronic structure of the (LiYb)$^+$ molecular ion is investigated with two variants of the coupled cluster method restricted to single, double, and noniterative or linear triple excitations. Potential energy curves for the ground and…
Ultracold polyatomic molecules offer intriguing new opportunities in cold chemistry, precision measurements, and quantum information processing, thanks to their rich internal structure. However, their increased complexity compared to…
We investigate the prospects of controlling charge-exchange in ultracold collisions of heteroisotopic combinations of atoms and ions of the same element. The treatment, readily applicable to alkali or alkanine-earth metals, is illustrated…
We investigate ultracold collisions in a novel mixture of $^6$Li and $^{53}$Cr fermionic atoms, discovering more than 50 interspecies Feshbach resonances via loss spectroscopy. Building a full coupled-channel model, we unambiguously…
We propose a new mechanism to produce ultracold polar molecules with microwave fields. The proposed mechanism converts trapped ultracold atoms of different species into vibrationally excited molecules by a single microwave transition and…
We report on the creation of heterospecies bosonic molecules, associated from an ultracold Bose-Bose mixture of 41K and 87Rb, by using a resonantly modulated magnetic field close to two Feshbach resonances. We measure the binding energy of…
Imaging the structure of molecules in transient excited states remains a challenge due to the extreme requirements for spatial and temporal resolution. Ultrafast electron diffraction from aligned molecules (UEDAM) provides atomic resolution…