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We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading…

Atomic Physics · Physics 2021-02-16 Michał Śmiałkowski , Michał Tomza

In this work we investigate the possibility to create cold Fr$\_2$, RbFr, and CsFr molecules through photoassociation of cold atoms. Potential curves, permanent and transition dipole moments for the Francium dimer and for the RbFr and RbCs…

Quantum Physics · Physics 2009-11-13 Mireille Aymar , Olivier Dulieu , Fernand Spiegelman

Deformed nuclei exhibit enhanced moments that violate time-reversal invariance ($T$) and parity ($P$). This paper focuses on the enhanced nuclear electric dipole moment (EDM) and Schiff moment present in nuclei with octupole deformation…

Nuclear Theory · Physics 2025-06-24 V. V. Flambaum , A. J. Mansour

The electric dipole moments (EDMs) of heavy nuclei, such as 199Hg, 225Ra and 211Rn, can be enhanced by the Schiff moments induced by the presence of nearby parity-doublet states. Working within the framework of the maximally CP-violating…

High Energy Physics - Phenomenology · Physics 2015-03-17 John Ellis , Jae Sik Lee , Apostolos Pilaftsis

Magnetic Feshbach resonances are an invaluable tool for controlling ultracold atoms and molecules. They can be used to tune atomic interactions and have been used extensively to explore few- and many-body phenomena. They can also be used…

Chemical reactions can be surprisingly efficient at ultracold temperatures ( < 1mK) due to the wave nature of atoms and molecules. The study of reactions in the ultracold regime is a new research frontier enabled by cooling and trapping…

Atomic Physics · Physics 2017-01-16 Lee R. Liu , Jessie T. Zhang , Yichao Yu , Nicholas R. Hutzler , Yu Liu , Till Rosenband , Kang-Kuen Ni

We report on the observation of ultracold heteronuclear Feshbach molecules. Starting with a $^{87}$Rb BEC and a cold atomic gas of $^{85}$Rb, we utilize previously unobserved interspecies Feshbach resonances to create up to 25,000…

Other Condensed Matter · Physics 2009-07-01 S. B. Papp , C. E. Wieman

Ultracold diatomic molecules find application in quantum studies ranging from controlled chemistry and precision measurement physics to quantum many-body simulation and potentially quantum computing. Accurate knowledge of molecular…

Atomic Physics · Physics 2024-05-14 Hela Ladjimi , Michał Tomza

We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of $^{40}$K and $^{87}$Rb atoms, where we can create as many as $7\times 10^4$ $^{40}$K$^{87}$Rb molecules with a conversion efficiency as high as 45%.…

Quantum Gases · Physics 2013-09-12 Tyler D. Cumby , Ruth A. Shewmon , Ming-Guang Hu , John D. Perreault , Deborah S. Jin

Parity and time invariance violating (${\cal P},{\cal T}$-odd) nuclear forces produce ${\cal P},{\cal T}$-odd nuclear moments, for example, the nuclear Schiff moment. In turn, this moment can induce electric dipole moments (EDMs) in atoms.…

Nuclear Theory · Physics 2009-08-18 V. V. Flambaum , V. G. Zelevinsky

Ultracold Feshbach molecules are a crucial intermediate step for the creation of quantum degenerate gases of strongly dipolar molecules. After coherent transfer to the rovibrational ground state, these dimers can realize stable dipolar…

Quantum Gases · Physics 2025-12-03 Sungjun Lee , Younghoon Lim , Jongyeol Kim , Jaeryeong Chang , Jee Woo Park

We report on the creation of ultracold heteronuclear molecules assembled from fermionic 40K and bosonic 87Rb atoms in a 3D optical lattice. Molecules are produced at a heteronuclear Feshbach resonance both on the attractive and the…

Statistical Mechanics · Physics 2007-05-23 C. Ospelkaus , S. Ospelkaus , L. Humbert , P. Ernst , K. Sengstock , K. Bongs

Photoassociation of ultracold atoms is a resonant light-assisted collision process, in which two colliding atoms absorb a photon and form an excited molecule. Since the first observation about three decades ago, the photoassociation of…

Atomic Physics · Physics 2024-03-19 Jin Cao , Bo-Yuan Wang , Huan Yang , Zhi-Jie Fan , Zhen Su , Jun Rui , Bo Zhao , Jian-Wei Pan

We report the comprehensive theoretical investigation of the Sr-SrOH system identifying it as a promising route to production of ultracold asymmetric top molecules. Combining high-level ab initio electronic structure calculations with…

Atomic Physics · Physics 2025-08-21 Maciej B. Kosicki , Mateusz Borkowski , Marcin Umiński , Piotr S. Żuchowski

Quantum gases of doubly-polar molecules represent appealing frameworks for a variety of cross-disciplinary applications, encompassing quantum simulation and computation, controlled quantum chemistry and precision measurements. Through a…

Optical Feshbach resonances [Phys. Rev. Lett. 94, 193001 (2005)] and pump-dump photoassociation with short laser pulses [Phys. Rev. A 73, 033408 (2006)] have been proposed as means to coherently form stable ultracold alkali dimer molecules.…

Atomic Physics · Physics 2009-01-05 Christiane P. Koch

Nuclear forces violating parity and time reversal invariance P,T-odd produce P,T-odd nuclear moments, for example, the nuclear Schiff moment. In turn, this moment can induce the electric dipole moment (EDM) in the atom. The contribution to…

Nuclear Theory · Physics 2007-05-23 A. F. Lisetskiy , V. V. Flambaum , V. G. Zelevinsky

We propose high-spin $\Sigma$-state polar molecules assembled from ultracold atoms to probe charge-parity violating physics beyond the Standard Model. We identify YbCr as a prime candidate to search for the electric dipole moment of the…

Quantum Gases · Physics 2026-03-16 Alessio Ciamei , Adam Koza , Marcin Gronowski , Michał Tomza

We propose a new method to produce an electric and magnetic dipolar gas of ultracold dysprosium atoms. The pair of nearly degenerate energy levels of opposite parity, at 17513.33 cm$^{-1}$ with electronic angular momentum $J=10$, and at…

Atomic Physics · Physics 2018-08-15 Maxence Lepers , Hui Li , Jean-François Wyart , Goulven Quéméner , Olivier Dulieu

A theoretical model is proposed for the formation of ultracold ground-state triatomic molecules in weakly bound energy levels. The process is driven by the electric component of a microwave field, which induces the association of an…

Atomic Physics · Physics 2026-01-16 Baraa Shammout , Leon Karpa , Silke Ospelkaus , Eberhard Tiemann , Olivier Dulieu