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The recent discovery of ambient-pressure superconductivity in thin-film bilayer nickelates opens new possibilities for investigating electronic structures in this new class of high-transition temperature $T_C$ superconductors. Here, we…

The discovery of superconductivity in the infinite-layer nickelates has opened new perspectives in the context of quantum materials. We analyze, via first-principles calculations, the electronic properties of La$_2$NiO$_3$F -- the first…

Superconductivity · Physics 2021-06-10 F. Bernardini , A. Demourgues , A. Cano

The discovery of superconductivity in nickelates has generated significant interest in condensed matter physics. Nickelate superconductors, which are hole-doped within the layered structure of RNiO$_2$, share structural similarities with…

Recent discovery of superconductivity in the doped infinite-layer nickelates has renewed interest in understanding the nature of high-temperature superconductivity more generally. The low-energy electronic structure of the parent compound…

The discovery of superconductivity in thin films ($\sim$10 nm) of infinite-layer hole-doped NdNiO$_2$ has invigorated the field of high-temperature superconductivity research, reviving the debate over contrasting views that nickelates that…

Superconductivity · Physics 2022-02-15 Antia S. Botana , Kwan-Woo Lee , Michael R. Norman , Victor Pardo , Warren E. Pickett

Superconductivity with a remarkably high $T_c$ has recently been found in Sr-doped NdNiO$_2$ thin films. While this system bears strong similarities to the cuprates, some differences, such as a weaker antiferromagnetic exchange coupling and…

Strongly Correlated Electrons · Physics 2020-01-15 Philipp Werner , Shintaro Hoshino

Recent experiments have shown that the reduced multilayer rare-earth (RE) nickel oxides of form RE$_{p+1}$Ni$_p$O$_{2p+2}$ may belong to the novel family of superconducting lanthanide nickelates. Here, the correlated electronic structure of…

Strongly Correlated Electrons · Physics 2022-04-07 Frank Lechermann

The recent discovery of superconductivity in Sr-doped NdNiO$_2$ films grown on SrTiO$_3$ started a novel field within unconventional superconductivity. To understand the similarities and differences between nickelate and cuprate layers on…

Strongly Correlated Electrons · Physics 2020-11-13 Yang Zhang , Ling-Fang Lin , Wenjun Hu , Adriana Moreo , Shuai Dong , Elbio Dagotto

Infinite-layer nickelate superconductors are typically synthesized as thin films and thus include, besides the more bulk-like inner layers, distinct surface and interface layers in contact with the vacuum and substrate, respectively. Here,…

Strongly Correlated Electrons · Physics 2025-11-26 Leonard M. Verhoff , Liang Si , Karsten Held

Superconducting nickelates appear to be difficult to synthesize. Since the chemical reduction of ABO3 (A: rare earth; B transition metal) with CaH2 may result in both, ABO2 and ABO2H, we calculate the topotactic H binding energy by density…

Strongly Correlated Electrons · Physics 2020-04-28 Liang Si , Wen Xiao , Josef Kaufmann , Jan M. Tomczak , Yi Lu , Zhicheng Zhong , Karsten Held

Recently, superconductivity with a $T_c$ up to 78 K has been reported in bulk samples of the bilayer nickelate La$_3$Ni$_2$O$_7$ at pressures above 14 GPa. Important theoretical tasks are the formulation of relevant low-energy models and…

Strongly Correlated Electrons · Physics 2023-11-17 Viktor Christiansson , Francesco Petocchi , Philipp Werner

Motivated by the recent discovery of superconductivity in the Sr-doped layered nickelate NdNiO$_2$, we perform a systematic computational materials design of layered nickelates that are dynamically stable and whose electronic structure…

Superconductivity · Physics 2020-02-12 Motoaki Hirayama , Terumasa Tadano , Yusuke Nomura , Ryotaro Arita

Motivated by the recent experimental discovery of superconductivity in the infinite-layer nickelate Nd0.8Sr0.2NiO2 [Li et al., Nature 572, 624 (2019)], we study how the correlated Ni 3dx2-y2 electrons in the NiO2 layer interact with the…

The recent observation of superconductivity at relatively high temperatures in hole doped NdNiO$_2$ has generated considerable interest, particularly due to its similarity with the infinite layer cuprates. Building on the observation that…

Strongly Correlated Electrons · Physics 2020-05-06 Ya-Hui Zhang , Ashvin Vishwanath

The discovery of superconductivity in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ [1] introduced a new family of layered nickelate superconductors that has now been extended to include a range of Sr-doping [2, 3], Pr or La in place of Nd [4-6], and the…

The recent discovery of high-T$_{c}$ superconductivity (HTS) in Sr-doped NdNiO$_2$ has sparked a renewed interest in investigating nickelates as cuprate counterparts. Parent cuprates [Cu$^{2+}$: d$^9$] are antiferromagnetic charge-transfer…

Superconductivity · Physics 2021-01-04 Jyoti Krishna , Harrison LaBollita , Adolfo O. Fumega , Victor Pardo , Antia S. Botana

Motivated by recent core-level x-ray photoemission spectroscopy (XPS), x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) experiments for the newly-discovered superconducting infinite-layer nickelate, we…

Strongly Correlated Electrons · Physics 2023-02-17 Keisuke Higashi , Mathias Winder , Jan Kuneš , Atsushi Hariki

It has been recently shown that under pressure trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ (LNO) becomes superconducting below a critical temperature $\sim$20 K, in addition to the infinite-layer and bilayer systems. Motivated…

Strongly Correlated Electrons · Physics 2024-06-12 I. V. Leonov

Effective models are constructed for a newly discovered superconductor (Nd,Sr)NiO2, which has been considered as a possible nickelate analogue of the cuprates owing to the d9 electron configuration. Estimation of the effective interaction,…

Superconductivity · Physics 2020-08-14 Hirofumi Sakakibara , Hidetomo Usui , Katsuhiro Suzuki , Takao Kotani , Hideo Aoki , Kazuhiko Kuroki

We present electronic structure calculations on layered nickelate oxyfluorides derived from the Ruddlesden-Popper arisotype structure in search of unidentified materials that may host nickelate superconductivity. By performing anion…