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Emergent flat-band physics in $d^{9-\delta}$ multilayer nickelates

Strongly Correlated Electrons 2022-04-07 v2 Materials Science Superconductivity

Abstract

Recent experiments have shown that the reduced multilayer rare-earth (RE) nickel oxides of form REp+1_{p+1}Nip_pO2p+2_{2p+2} may belong to the novel family of superconducting lanthanide nickelates. Here, the correlated electronic structure of Pr4_{4}Ni3_3O8_{8} and Nd6_{6}Ni5_5O12_{12} is studied by means of an advanced realistic many-body framework. It is revealed that the low-energy physics of both systems is dominated by an interplay of Ni-dx2y2d_{x^2-y^2} and Ni-dz2d_{z^2} degrees of freedom. Whilst the Ni-dx2y2d_{x^2-y^2} orbitals are always highly correlated near an (orbital-selective) Mott-insulating regime, the Ni-dz2d_{z^2} orbitals give rise to intriguing non-dispersive features. At low temperature, the Pr compound still displays QP-like Ni-dx2y2d_{x^2-y^2}-derived states at the Fermi level, but the interacting fermiology of the Nd compound is outshined by an emergent Ni-dz2d_{z^2}-controlling flat band. These findings translate well to the previous characterization of doped infinite-layer nickelates, and hence further make the case for a mechanism of unconventional superconductivity which is distinct from the one in high-TcT_{\rm c} cuprates.

Keywords

Cite

@article{arxiv.2201.08123,
  title  = {Emergent flat-band physics in $d^{9-\delta}$ multilayer nickelates},
  author = {Frank Lechermann},
  journal= {arXiv preprint arXiv:2201.08123},
  year   = {2022}
}

Comments

10 pages, 6 figures

R2 v1 2026-06-24T08:56:26.822Z