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Exchange correlation plays an important role in double-ionization of complex atoms by ultrashort laser pulse. In this work, we investigate two-photon double inner-shell electron ionization of neon induced by an attosecond extreme…

Atomic Physics · Physics 2019-06-05 Jianpeng Liu , Yongqiang Li , Jianmin Yuan

Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…

Atomic Physics · Physics 2021-06-30 Saad Mehmood , Eva Lindroth , Luca Argenti

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

In a double-slit experiment with a bipartite system, the visibility of interference fringes depends on the availability of which-way information. Here, we report the formation of a Bell-like state of photoelectron and residual ion in the…

We review different attempts to show the decoherence process in double-slit-like experiments both for charged particles (electrons) and neutral particles with permanent dipole moments. Interference is studied when electrons or atomic…

Quantum Physics · Physics 2009-11-11 Fernando C. Lombardo , Paula I. Villar

Photoionization using attosecond pulses can lead to the formation of coherent superpositions of the electronic states of the parent ion. However, ultrafast electron ejection triggers not only electronic but also nuclear dynamics---leading…

Chemical Physics · Physics 2017-03-29 Caroline Arnold , Oriol Vendrell , Robin Santra

The two-photon decay in hydrogen-like ions is investigated within the framework of second order perturbation theory and Dirac's relativistic equation. Special attention is paid to the angular correlation of the emitted photons as well as to…

Atomic Physics · Physics 2014-10-23 P. Amaro , F. Fratini , S. Fritzsche , P. Indelicato , J. P. Santos , A. Surzhykov

Autoionization, which results from the interference between direct photoionization and photoexcitation to a discrete state decaying to the continuum by configuration interaction, is a well known example of the important role of electron…

We calculate the decoherence caused by photon emission for a charged particle travelling through an interferometer; the decoherence rate gives a quantitative measure of how much "which-path" quantum information is gained by the…

Quantum Physics · Physics 2024-05-17 Colby DeLisle , P. C. E. Stamp

We report a theoretical investigation of photoionization by a pair of coherent, ultrashort fundamental and second-harmonic extreme-ultraviolet pulses, where the photon energies are selected to yield the same photoelectron energy for…

Atomic Physics · Physics 2023-11-27 Kenichi L. Ishikawa , Kevin C. Prince , Kiyoshi Ueda

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

We study resonant two-color two-photon ionization of Helium via the 1s3p 1P1 state. The first color is the 15th harmonic of a tunable titanium sapphire laser, while the second color is the fundamental laser radiation. Our method uses…

Engineering and studying few-electron states in ballistic conductors is a key step towards understanding entanglement in quantum electronic systems. In this Letter, we introduce the intrinsic two-electron coherence of an electronic source…

Mesoscale and Nanoscale Physics · Physics 2016-02-17 E. Thibierge , D. Ferraro , B. Roussel , C. Cabart , A. Marguerite , G. Fève , P. Degiovanni

We study and experimentally implement a double-slit quantum eraser in the presence of a controlled decoherence mechanism. A two-photon state, produced in a spontaneous parametric down conversion process, is prepared in a maximally entangled…

Quantum Physics · Physics 2015-05-14 F. A. Torres-Ruiz , G. Lima , A. Delgado , S. Pádua , C. Saavedra

Classical physics is often a good approximation for quantum systems composed of many interacting particles, although wavepacket dispersion and scattering processes continuously induce delocalization and entanglement. According to…

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

Chemical Physics · Physics 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

We discuss the various manifestations of quantum decoherence in the forms of dephasing, entanglement with the environment, and revelation of "which-path" information. As a specific example, we consider an electron interference experiment.…

Quantum Physics · Physics 2015-05-13 Jen-Tsung Hsiang , L. H. Ford

A theoretical study of the polarization entanglement of two photons emitted in the decay of metastable ionic states is performed within the framework of density matrix theory and second-order perturbative approach. Particular attention is…

Ionization of atoms and molecules by absorption of a light pulse results in electron wavepackets carrying information on the atomic or molecular structure as well as on the dynamics of the ionization process. These wavepackets can be…

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

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