Related papers: Probing electronic decoherence with high-resolutio…
Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…
The performance of modern quantum devices in communication, metrology or microscopy relies on the quantum-classical interaction which is generally described by the theory of decoherence. Despite the high relevance for long coherence times…
We report on kinematically complete measurements and ab initio non-perturbative calculations of double ionization of He and H2 by a single 800 eV circularly polarized photon. We confirm the quasifree mechanism of photoionization for H2 and…
A two-particle interferometer is theoretically analyzed, to show how decoherence induced by interactions with the environment affects time correlations, a process we call time-correlation de-coherence. Specifically, on the basis of simple…
We measure the decoherence of a spatially separated atomic superposition due to spontaneous photon scattering. We observe a qualitative change in decoherence versus separation as the number of scattered photons increases, and verify…
The ionization of atoms with sequences of attosecond pulses gives rise to excited ionic states that are entangled with the emitted photoelectron. Still, the ionic ensemble preserves some coherence that can be controlled through the laser…
Complexity in strongly correlated electron systems is analyzed by considering decoherence process between the localized state, |L> and the itinerant state, |I>. The coherent superposition state of a|I> + b|L> decoheres to the pointer states…
We show that the complete photoemission dynamics in situations of electron-ion entanglement can be retrieved from photoelectron spectral measurements without information on the ion. To this end, we develop an energy-time analysis of the…
Quantum coherence between electronic states of a photoionized molecule and the resulting process of ultrafast electron-hole migration have been put forward as a possible quantum mechanism of charge-directed reactivity governing the…
We produce polarization entangled states with variable degree of entanglement for twin photons. Entanglement in polarization is coupled to entanglement in position that produces transverse coincidence interference fringes. We show both…
Electron microscopy relies on the spatial coherence of electron beams to generate atomic-scale images using interference and diffraction, which can be degraded by inelastic scattering processes that induce decoherence. Here, we present a…
The study of entangled states has greatly improved the basic understanding about two-photon interferometry. Two-photon interference is not the interference of two photons but the result of superposition among indistinguishable two-photon…
In a joint experimental and theoretical endeavour, photoionization of metastable C4+(1s 2s 3S1) ions via intermediate levels with hollow, double-K-vacancy configurations 2s2p, 2s3p, 2p3s, 2p3d, 2s4p, 2p4s and 2p4d has been investigated.…
Fano resonances are ubiquitous phenomena appearing in many fields of physics, e.g. atomic or molecular photoionization, or electron transport in quantum dots. Recently, attosecond interferometric techniques have been used to measure the…
We propose a scheme to explore two-photon high-dimensional entanglement associated with a transverse pattern by means of two-photon interference in a beamsplitter. We find that the topological symmetry of the angular spectrum of the…
Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…
We report on interferometric autocorrelation measurements of broadband supercontinuum light in the anomalous dispersion regime using two-photon absorption in a GaP photodetector. The method is simple, low-cost, and provides a direct measure…
The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…
A photofragmentation study of gas-phase indole (C$_8$H$_7$N) upon single-photon ionization at a photon energy of 420 eV is presented. Indole was primarily inner-shell ionized at its nitrogen and carbon $1s$ orbitals. Electrons and ions were…
We study theoretically single electron loss from helium-like highly charged ions involving excitation and decay of autoionizing states of the ion. Electron loss is caused by either photo absorption or the interaction with a fast atomic…