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A nonlinear interferometry scheme is described theoretically to induce and resolve electron wave- function beating on time scales shorter than the optical cycle of the time-delayed pump and probe pulses. By employing two moderately intense…

Chemical Physics · Physics 2017-08-23 Christian Ott , Philipp Raith , Thomas Pfeifer

We propose a novel quantum diffraction imaging technique whereby one photon of an entangled pair is diffracted off a sample and detected in coincidence with its twin. The image is obtained by scanning the photon that did not interact with…

Quantum Physics · Physics 2019-09-04 Shahaf Asban , Konstantin E. Dorfman , Shaul Mukamel

We investigate the intensity correlation properties of single photons emitted from an optically excited single semiconductor quantum dot. The second order temporal coherence function of the photons emitted at various wavelengths is measured…

Strongly Correlated Electrons · Physics 2009-11-07 D. V. Regelman , U. Mizrahi , D. Gershoni , E. Ehrenfreund , W. V. Schoenfeld , P. M. Petroff

Quantum light is increasingly recognized as a promising resource for developing optical measurement techniques. Particular attention has been paid to enhancing the precision of the measurements beyond classical techniques by using…

Chemical Physics · Physics 2023-10-03 Yuta Fujihashi , Kuniyuki Miwa , Masahiro Higashi , Akihito Ishizaki

We describe a method to probe the spectral fluctuations of a transition over broad ranges of frequencies and timescales with the high spectral resolution of Fourier spectroscopy, and a temporal resolution as high as the excited state…

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

We present a technique to completely characterise the spectral-temporal wave function of a broadband photon pair using spectral-shearing interferometry. Our method is fully self-referencing and is generalisable across a wide range of…

Quantum Physics · Physics 2018-09-12 Alex O. C. Davis , Valerian Thiel , Brian J. Smith

We describe and demonstrate a quantum state tomography for measuring the complex temporal waveform of narrowband biphotons. Through six sets of two-photon interference measurements projected in different polarization subspaces, we can…

Quantum Physics · Physics 2015-01-14 Peng Chen , Chi Shu , Xianxin Guo , M. M. T. Loy , Shengwang Du

Conventional optical synthesis, the manipulation of the phase and amplitude of spectral components to produce an optical pulse in different temporal modes, is revolutionizing ultrafast optical science and metrology. These technologies rely…

In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…

Quantum Physics · Physics 2026-04-24 Arunangshu Debnath , Shaul Mukamel

In this article we try to describe the physics of a standard optical interferometer fed by "quantum" photons in terms of primitive, nevertheless accurate formulation. We derive explicit interferene patterns and show how they vary depending…

Quantum Physics · Physics 2016-03-30 Fujio Shimizu

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

Atomic Physics · Physics 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

We show that quantum frequency conversion (QFC) can overcome the spectral distinguishability common to inhomogeneously broadened solid-state quantum emitters. QFC is implemented by combining single photons from an InAs quantum dot (QD) at…

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

Quantum sensing is highly attractive for accessing spectral regions in which the detection of photons is technically challenging: sample information is gained in the spectral region of interest and transferred via entanglement into another…

We explore the response of a quantum ring system coupled to a photon cavity with a single mode when excited by a classical dipole field. We find that the energy oscillates between the electronic and photonic components of the system. The…

Mesoscale and Nanoscale Physics · Physics 2014-12-16 Thorsten Arnold , Chi-Shung Tang , Andrei Manolescu , Vidar Gudmundsson

Multi-photon propagation in connected structures - a quantum walk - offers the potential for simulating complex physical systems and provides a route to universal quantum computation. Increasing the complexity of quantum photonic networks…

Quantum Physics · Physics 2016-03-21 Hugo Defienne , Marco Barbieri , Ian A. Walmsley , Brian J. Smith , Sylvain Gigan

A photon is the single excitation of a particular spatiotemporal mode of the electromagnetic field. A precise knowledge of the mode structure is therefore essential for its processing and detection, as well as for applying generic quantum…

Quantum entanglement and squeezing have significantly improved phase estimation and imaging in interferometric settings beyond the classical limits. However, for a wide class of non-interferometric phase imaging/retrieval methods vastly…