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We investigate quantum spectroscopy with undetected photons for protein detection in the mid-infrared spectral region. Classical Fourier-transform infrared spectroscopy of protein samples (bovine serum albumin and N-terminal pro-brain…

At the heart of recent breakthroughs in quantum imaging and spectroscopy utilizing undetected photons lies the quantum optical effect known as induced coherence without induced emission. This fundamental quantum interference effect has…

Quantum Physics · Physics 2025-10-24 Dong-Gil Im , Seung-Yeun Yoo , Chung-Hyun Lee , Jongheon Suh , Yoon-Ho Kim

We propose and demonstrate a method for measuring the joint spectrum of photon pairs via Fourier spectroscopy. The biphoton spectral intensity is computed from a two-dimensional interferogram of coincidence counts. The method has been…

We study a system of two interacting, non-indentical quantum emitters driven by a coherent field. We focus on the particular condition of two-photon resonance and obtain analytical expressions for the stationary density matrix of the system…

Quantum Physics · Physics 2021-08-18 Alejandro Vivas-Viaña , Carlos Sánchez Muñoz

We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto…

Quantum Physics · Physics 2013-05-24 J. Feist , S. Nagele , C. Ticknor , B. I. Schneider , L. A. Collins , J. Burgdörfer

Joint spectral measurements are a powerful tool for characterising biphoton spectral correlation, which is crucial for quantum information and communication technologies. In these applications, highly pure biphoton states are essential in…

We perform a high resolution Fourier Transform Spectroscopy of optical sources in the few-photon regime based on the phenomenon of two-photon interference in a beam splitter. From the heterodyne interferogram between test and reference…

We present a quantum interference phenomenon in which four-photon quantum states generated by two independent sources are used to create a two-photon interference pattern without detecting two of the photons. Contrary to the common…

Quantum Physics · Physics 2025-09-26 Chandler Tarrant , Mayukh Lahiri

It is demonstrated a two-photon interfering technique based on polarization-resolved measurements for the simultaneous estimation with the maximum sensitivity achievable in nature of multiple parameters associated with the polarization…

Quantum Physics · Physics 2025-02-11 L. Maggio , D. Triggiani , P. Facchi , V. Tamma

It is controversial what is the true role of entanglement in two-photon virtual-state spectroscopy [Saleh et al, Phys. Rev. Lett. 80, 3483, 1998], a two-photon absorption spectroscopic technique that can retrieve information about the…

Quantum Physics · Physics 2015-06-11 R. de J. León-Montiel , J. Svozilík , L. J. Salazar-Serrano , J. P. Torres

Two-dimensional spectroscopy is discussed for open quantum systems with multiple simultaneously measurable fluxes. In particular, we discuss a junction where optical measurements of photon flux are complemented with simultaneous transport…

Mesoscale and Nanoscale Physics · Physics 2025-02-28 Haoran Sun , Upendra Harbola , Shaul Mukamel , Michael Galperin

Two-mode squeezing is central to entangled-photon generation and nonlinear interferometry, yet standard perturbative low-gain treatments and Gaussian formalisms can obscure the interference of photon-number amplitudes, especially in…

Quantum Physics · Physics 2026-02-11 Xuemei Gu , Carlos Ruiz-Gonzalez , Mario Krenn

The study of entangled states has greatly improved the basic understanding about two-photon interferometry. Two-photon interference is not the interference of two photons but the result of superposition among indistinguishable two-photon…

Quantum Physics · Physics 2009-11-10 Giuliano Scarcelli , Alejandra Valencia , Yanhua Shih

We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor,…

Quantum Physics · Physics 2009-01-23 F. Zäh , M. Halder , T. Feurer

Multi-photon quantum interference is the underlying principle for optical quantum information processing protocols. Indistinguishability is the key to quantum interference. Therefore, the success of many protocols in optical quantum…

Quantum Physics · Physics 2020-09-23 Liang Cui , Jie Su , Jiamin Li , Yuhong Liu , Xiaoying Li , Z. Y. Ou

This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series of one- and two-dimensional nonlinear spectroscopic…

Quantum light spectroscopy, providing novel molecular information non-accessible by classical light, necessitates new computational tools when applied for complex molecular systems. We introduce two computational protocols for the molecular…

Chemical Physics · Physics 2021-09-14 Bing Gu , Daniel Keefer , Shaul Mukamel

We present ultra-fast quantum chemical methods for the calculation of infrared and ultraviolet-visible spectra designed to provide fingerprint information during autonomous and interactive explorations of molecular structures.…

Chemical Physics · Physics 2022-08-30 Francesco Bosia , Thomas Weymuth , Markus Reiher

Quantum phenomena such as entanglement can improve fundamental limits on the sensitivity of a measurement probe. In optical interferometry, a probe consisting of $N$ entangled photons provides up to a $\sqrt{N}$ enhancement in phase…

Two-photon interference, a quantum phenomenon arising from the principle of indistinguishability, is a powerful tool for quantum state engineering and plays a fundamental role in various quantum technologies. These technologies demand…