Related papers: Quantum interferometric two-photon excitation spec…
We report a direct demonstration of quantum-enhanced sensing in the Fourier domain by comparing single- and two-photon interference in a fiber-based interferometer under strictly identical noise conditions. The simultaneous acquisition of…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…
Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…
Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the…
Quantum information science is driving progress in a vast number of scientific and technological areas that cover molecular spectroscopy and matter-light interactions in general. In these fields, the ability to generate quantum…
The spectral characterization of quantum emitter luminescence over broad wavelength ranges and fast timescales is important for applications ranging from biophysics to quantum technologies. Here we present the application of time-domain…
Coherent two-dimensional spectroscopy in IR or visible region is very effective for studying correlations, energy relaxation/transfer pathways in complex multi-chromophore or multi-mode systems. However it is usually restricted up to…
We consider how the conventional spectroscopic and interferometric schemes can be rearranged to serve for reconstructing quantum states of physical systems possessing SU(2) symmetry. The discussed systems include a collection of two-level…
The goal of this research is to determine and study a physical system that will enable a fast and intrinsically two-photon detector, which would be of interest for quantum information and metrology applications. We consider two types of…
Recent interest in the role of quantum mechanics in the primary events of photosynthetic energy transfer has led to a convergence of nonlinear optical spectroscopy and quantum optics on the topic of energy-transfer dynamics in…
Quantum-correlated interferometer is a newly emerging tool in quantum technology that offers classical-limit-breaking phase sensitivity. But to date, there exists a configurational bottleneck for its practicability due to the low…
We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to…
Attosecond nonlinear Fourier transform (NFT) pump probe spectroscopy is an experimental technique which allows investigation of the electronic excitation, ionization, and unimolecular dissociation processes. The NFT spectroscopy utilizes…
The ability to entangle distant quantum nodes is essential for the construction of quantum networks and for quantum information processing. For solid-state quantum emitters used as qubits, it can be achieved by photon interference. When the…
Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of…
Properties of quantum states have disclosed new and revolutionary technologies, ranging from quantum information to quantum imaging. This last field is addressed to overcome limits of classical imaging by exploiting specific properties of…
Entangled photons (biphotons) in the time-frequency degree of freedom play a crucial role in both foundational physics and advanced quantum technologies. Fully characterizing them poses a key scientific challenge. Here, we propose a…
The quest to have both which-path knowledge and interference fringes in a double-slit experiment dates back to the inception of quantum mechanics (QM) and to the famous Einstein-Bohr debates. In this paper we propose and discuss an…
In this chapter we review the use of semiconductor quantum dots as sources of quantum light. Principally, we focus on resonant two-photon excitation, which is a method that allows for on-demand generation of photon pairs. We explore the…