Related papers: Magnetotropic Response in Ruthenium Chloride
Materials manifesting the Kitaev model, characterized by bond-dependent interactions on a honeycomb lattice, can host exotic phenomena like quantum spin liquid states and topological magnetic excitations. However, finding such materials…
The present studies show that long-range magnetic order takes place in RuBr$_3$ at $\approx$ 34 K. The observations of clear oscillations in the muon time spectra demonstrate the presence of well-defined internal fields at the muon sites.…
Thermomagnetic and inelastic neutron scattering measurements on Na2PrO3 are reported. This material is an antiferromagnetic honeycomb magnet based on the tetravalent lanthanide Pr4+ and has been proposed to host dominant antiferromagnetic…
$\alpha$-RuCl$_3$ has attracted significant attention as a prime candidate for the spin-1/2 Kitaev spin liquid in two-dimensional honeycomb lattices. Although its ground state is magnetically ordered, the order is suppressed under a…
Hexagonal alpha-Ru trichloride single crystals exhibit a strong magnetic anisotropy and we show that upon applying fields up to 14 T in the honeycomb plane the successive magnetic order at T1 = 14 K and T2 = 8 K could be completely…
Anderson proposed structural topology in frustrated magnets hosting novel quantum spin liquids (QSLs). The QSL state is indeed exactly derived by fractionalizing the spin excitation into spinless Majorana fermions in a perfect two…
We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $\alpha$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a…
The Kitaev model is a rare example of an analytically solvable and physically instantiable Hamiltonian yielding a topological quantum spin liquid ground state. Here we report signatures of Kitaev spin liquid physics in the honeycomb magnet…
The exchange-driven contribution to the magnetoelectric susceptibility $\hat\alpha$ is formulated using a microscopic model Hamiltonian coupling the spin degrees of freedom to lattice displacements and electric field, which may be…
An effective low-energy Hamiltonian of itinerant electrons for iridium oxide Na2IrO3 is derived by an ab initio downfolding scheme. The model is then reduced to an effective spin model on a honeycomb lattice by the strong coupling…
The theoretical inception of the Kitaev honeycomb model has had defining influence on the experimental hunt for quantum spin liquids, bringing unprecedented focus onto the synthesis of materials with bond-directional interactions. Numerous…
The magnetism of Kitaev materials has been widely studied, but their charge properties and the coupling to other degrees of freedom are less known. Here we investigate the charge states of $\alpha$-RuCl$_3$, a promising Kitaev quantum spin…
The honeycomb $K-\Gamma$ model is known to have both deconfined spin liquid and confined phases. We study here a confinement transition between the Kitaev spin liquid and a dimerized phase in the limit of strong bond anisotropy. By…
We use an exact numerical diagonalization method to calculate the dynamical spin structure factors (DSFs) of three ab-initio models and one ab-initio-guided model for a honeycomb-lattice magnet $\alpha$-RuCl$_3$. We also use thermal pure…
The antiferromagnetic insulating cuprate Ba$_3$Cu$_2$O$_4$Cl$_2$ contains folded CuO$_2$ chains with four magnetic copper ions ($S=1/2$) per unit cell. An underlying multiorbital Hubbard model is formulated and the superexchange theory is…
Combining thermodynamic measurements with theoretical density functional and thermodynamic calculations we demonstrate that the honeycomb lattice iridates A2IrO3 (A = Na, Li) are magnetically ordered Mott insulators where the magnetism of…
We use a recently developed interpretable and unsupervised machine-learning method, the tensorial kernel support vector machine (TK-SVM), to investigate the low-temperature classical phase diagram of a generalized Heisenberg-Kitaev-$\Gamma$…
Single layer $\alpha$-ruthenium trichloride ($\rm\alpha-RuCl_3$) has been proposed as a potential quantum spin liquid. Graphene/$\rm RuCl_3$ heterobilayers have been extensively studied with a focus on the large interlayer electron transfer…
We study the effective spin-orbital model for honeycomb-layered transition metal compounds, applying the second-order perturbation theory to the three-orbital Hubbard model with the anisotropic hoppings. This model is reduced to the Kitaev…
Rare-earth materials hold promise to realize exotic magnetic states owing to synergy between electron correlations and spin-orbit coupling. Recently, quasi-two-dimensional honeycomb magnets $A_2$PrO$_3$ ($A$ = alkali metals) were predicted…