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We performed the detailed microscopic analysis of the inter-layer magnetic couplings for bilayer CrI$_3$. As the first step toward understanding the recent experimental observations and utilizing them for device applications, we estimated…

Materials Science · Physics 2019-04-10 Seung Woo Jang , Min Yong Jeong , Hongkee Yoon , Siheon Ryee , Myung Joon Han

Recently, two-dimensional (2D) bilayer magnetic systems have been widely studied. Their interlayer magnetic interactions play a vital role in the magnetic properties. In this paper, we theoretically studied the interlayer magnetic…

Materials Science · Physics 2025-09-10 Wenqi Yang , Xinlong Yang , Menglei Li , Lin Hu , Fawei Zheng

Diverse interlayer tunability of physical properties of two-dimensional layers mostly lies in the covalent-like quasi-bonding that is significant in electronic structures but rather weak for energetics. Such characteristics result in…

Materials Science · Physics 2019-04-03 Peiheng Jiang , Cong Wang , Dachuan Chen , Zhicheng Zhong , Zhe Yuan , Zhong-Yi Lu , Wei Ji

We address the interplay between stacking and interlayer exchange for ferromagnetically ordered CrI$_3$, both for bilayers and bulk. Whereas bulk CrI$_3$ is ferromagnetic, both magneto-optical and transport experiments show that interlayer…

Mesoscale and Nanoscale Physics · Physics 2019-08-29 D. Soriano , C. Cardoso , J. Fernández-Rossier

In twisted two-dimensional (2D) magnets, the stacking dependence of the magnetic exchange interaction can lead to regions of ferromagnetic and antiferromagnetic interlayer order, separated by non-collinear, skyrmion-like spin textures.…

We report the connection between the stacking order and magnetic properties of bilayer CrI$_3$ using first-principles calculations. We show that the stacking order defines the magnetic ground state. By changing the interlayer stacking order…

Materials Science · Physics 2018-11-19 Nikhil Sivadas , Satoshi Okamoto , Xiaodong Xu , Craig. J. Fennie , Di Xiao

A monolayer of CrI$_3$ is a two-dimensional crystal that in its equilibrium configuration is a ferromagnetic semiconductor, however, two coupled layers can be ferromagnetic or antiferromagnetic depending on the stacking. We study the…

Mesoscale and Nanoscale Physics · Physics 2020-04-07 Andrea Leon , J. W. González , J. Mejía-López , F. Crasto de Lima , E. Suárez Morell

The emergence of two-dimensional (2D) magnetic crystals and moir\'e engineering has opened the door for devising new magnetic ground states via competing interactions in moir\'e superlattices. Although a suite of interesting phenomena,…

Recently intrinsic ferromagnetism in two-dimensional(2D) van der Waals materials was discovered [1, 2, 3]. A monolayer of Chromiun triiodide(CrI3) is ferromagnetic while a bilayer structure was reported to be anti-ferro magnetic, moreover…

Materials Science · Physics 2018-11-30 E. Suarez Morell , Andrea León , R. Hiroki Miwa , P. Vargas

We present a comprehensive theory of the magnetic phases in twisted bilayer Cr-trihalides through a combination of first-principles calculations and atomistic simulations. We show that the stacking-dependent interlayer exchange leads to an…

Strongly Correlated Electrons · Physics 2021-08-13 Muhammad Akram , Harrison LaBollita , Dibyendu Dey , Jesse Kapeghian , Onur Erten , Antia S. Botana

Various noncollinear spin textures and magnetic phases have been predicted in twisted two-dimensional CrI$_3$ due to competing ferromagnetic (FM) and antiferromagnetic (AFM) interlayer exchange from moir\'e stacking - with potential…

The exploration of magnetism in two-dimensional layered materials has attracted extensive research interest. For the monoclinic phase CrI3 with interlayer antiferromagnetism, finding a static and robust way of realizing the intrinsic…

Materials Science · Physics 2022-11-30 Shiyang Sun , Xuyan Chen , Xuqi Li , Huihui Zhang , Haidan Sang , Shifei Qi , Zhenhua Qiao

The marked interplay between the crystalline, electronic, and magnetic structure of atomically thin magnets has been regarded as the key feature for designing next-generation magneto-optoelectronic devices. In this respect, a detailed…

Strongly Correlated Electrons · Physics 2020-05-25 Michele Pizzochero , Ravi Yadav , Oleg V. Yazyev

Bilayer CrI$_3$ attracted much attention owing to peculiar switching between the layered ferromagnetic and antiferromagnetic order upon stacking alternation. This finding pointed out the importance of the apparently small interlayer…

Materials Science · Physics 2024-06-19 Srdjan Stavrić , Paolo Barone , Silvia Picozzi

We use a first-principles calculations approach to reveal the electronic and magnetic properties of chromium diiodide (CrI$_2$) bilayers and establish a hierarchy of magnetic interactions across stable registries. The monolayer presents a…

Materials Science · Physics 2025-12-23 B. Valdés-Toro , I. Ferreira-Araya , R. A. Gallardo , J. W. González

The magnetic properties of two-dimensional VI3 bilayer are the focus of our first-principles analysis, highlighting the role of trigonal crystal-field effects and carried out in comparison with the CrI3 prototypical case, where the effects…

Materials Science · Physics 2021-07-21 Thi Phuong Thao Nguyen , Kunihiko Yamauchi , Tamio Oguchi , Danila Amoroso , Silvia Picozzi

The interfacial coupling between electrons and magnons in adjacent layers can mediate an attractive electron-electron interaction and induce superconductivity. We consider magic-angle twisted bilayer graphene sandwiched between two…

Superconductivity · Physics 2023-01-20 Bjørnulf Brekke , Asle Sudbø , Arne Brataas

Motivated by the recent experiment demonstration of stacking dependent interlayer magnetic interaction [T. Song et al., Nat. Mater. 18, 1298 (2019); T. Li et al., Nat. Mater. 18, 1303 (2019); W. Chen et al., Science 366, 983 (2019)], we…

Mesoscale and Nanoscale Physics · Physics 2021-03-22 Feiping Xiao , Keqiu Chen , Qingjun Tong

Motivated by the potential of atomically-thin magnets towards tunable high-frequency magnonics, we detail the spin-wave dispersion of bilayer CrI$_3$. We demonstrate that the magnonic behavior of the bilayer strongly depends on its stacking…

Materials Science · Physics 2023-03-01 M. Soenen , C. Bacaksiz , R. M. Menezes , M. V. Milosevic

Two-dimensional (2D) materials are being explored as a novel multiferroic platform. One of the most studied magnetoelectric multiferroic 2D materials are antiferromagnetically-coupled (AFM) CrI$_3$ bilayers. Neglecting magnetism, those…

Mesoscale and Nanoscale Physics · Physics 2023-05-16 Shiva P. Poudel , Juan M. Marmolejo-Tejada , Joseph E. Roll , Martín A. Mosquera , Salvador Barraza-Lopez
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